85 research outputs found
Multiband tight-binding theory of disordered ABC semiconductor quantum dots: Application to the optical properties of alloyed CdZnSe nanocrystals
Zero-dimensional nanocrystals, as obtained by chemical synthesis, offer a
broad range of applications, as their spectrum and thus their excitation gap
can be tailored by variation of their size. Additionally, nanocrystals of the
type ABC can be realized by alloying of two pure compound semiconductor
materials AC and BC, which allows for a continuous tuning of their absorption
and emission spectrum with the concentration x. We use the single-particle
energies and wave functions calculated from a multiband sp^3 empirical
tight-binding model in combination with the configuration interaction scheme to
calculate the optical properties of CdZnSe nanocrystals with a spherical shape.
In contrast to common mean-field approaches like the virtual crystal
approximation (VCA), we treat the disorder on a microscopic level by taking
into account a finite number of realizations for each size and concentration.
We then compare the results for the optical properties with recent experimental
data and calculate the optical bowing coefficient for further sizes
Resonant electron tunneling through semiconducting nanocrystals in a symmetrical and an asymmetrical junction
A single-electron transistor made from a cadmium selenide nanocrystal
The techniques of colloidal chemistry permit the routine creation of
semiconductor nanocrystals, whose dimensions are much smaller than those that
can be realized using lithographic techniques. The sizes of such nanocrystals
can be varied systematically to study quantum size effects or to make novel
electronic or optical materials with tailored properties. Preliminary studies
of both the electrical and optical properties of individual nanocrystals have
been performed recently. These studies show clearly that a single excess charge
on a nanocrystal can markedly influence its properties. Here we present
measurements of electrical transport in a single-electron transistor made from
a colloidal nanocrystal of cadmium selenide. This device structure enables the
number of charge carriers on the nanocrystal to be tuned directly, and so
permits the measurement of the energy required for adding successive charge
carriers. Such measurements are invaluable in understanding the energy-level
spectra of small electronic systems, as has been shown by similar studies of
lithographically patterned quantum dots and small metallic grains.Comment: 3 pages, PDF forma
A Spatial Distribution Study of Faunal Remains from Two Lower Magdalenian Occupation Levels in El MirĂłn Cave, Cantabria, Spain
Abstract: Human behaviour can be reconstructed by analysing specific activities and campsite organization using spatial analysis. The dense occupation layers of the Lower Cantabrian Magdalenian in the Northern Spain reveal varied aspects of Upper Palaeolithic lifeways, including evidence of specific localized activities. The outer vestibule of El Mirón cave has a particularly rich and intact Lower Magdalenian occupation horizon, Levels 15–17. The excavations in the outer vestibule “Cabin” area of the site revealed excellent bone preservation. Artefacts and faunal remains were individually recorded and sediments water-screened to yield a large sample of archaeological finds and spatial data. Zooarchaeological analysis provided the taxonomic, anatomic and taphonomic determination of the faunal individual finds. Smaller animal remains were categorized and counted; special attention was given to the identification of anthropogenic modifications such as burnt bones or bone flakes. These small refuse items are considered to be useful, in situ indicators of localized activities. The spatial distribution analysis of this dense and complex palimpsest of El Mirón Lower Cantabrian Magdalenian layers required GIS based methods including density analysis, heatmaps and cluster analysis. Based on the spatial distribution of Level 15 and 16 faunal remains, different activity areas were identified comprising hearth, working and dropping zones. These results imply the deliberately segregated use of space within the Lower Cantabrian Magdalenian site area, in which bone-processing activities played a central rol
Intercalation of Inorganic Fullerene-like Structures Yields Photosensitive Films and New Tips for Scanning Probe Microscopy
Evaluating the intensity of fire at the Acheulian site of Gesher Benot Ya'aqov—Spatial and thermoluminescence analyses
Microstratigraphic evidence of in situ fire in the Acheulean strata of Wonderwerk Cave, Northern Cape province, South Africa
The ability to control fire was a crucial turning point in human evolution, but the question when hominins first developed this ability still remains. Here we show that micromorphological and Fourier transform infrared microspectroscopy (mFTIR) analyses of intact sediments at the site of Wonderwerk Cave, Northern Cape province, South Africa, provide unambiguous evidence—in the form of burned bone and ashed plant remains—that burning took place in the cave during the early Acheulean occupation, approximately 1.0 Ma. To the best of our knowledge, this is the earliest secure evidence for burning in an archaeological context
Physical Fitness, Body Image, and Locus of Control in College Women Dancers and Nondancers
- …