358 research outputs found
Critical chain length and superconductivity emergence in oxygen-equalized pairs of YBa2Cu3O6.30
The oxygen-order dependent emergence of superconductivity in YBa2Cu3O6+x is
studied, for the first time in a comparative way, on pair samples having the
same oxygen content and thermal history, but different Cu(1)Ox chain
arrangements deriving from their intercalated and deintercalated nature.
Structural and electronic non-equivalence of pairs samples is detected in the
critical region and found to be related, on microscopic scale, to a different
average chain length, which, on being experimentally determined by nuclear
quadrupole resonance (NQR), sheds new light on the concept of critical chain
length for hole doping efficiency.Comment: 7 RevTex pages, 2 Postscript figures. Submitted to Phys. Rev.
Modification of magnetic and transport properties of manganite layers in Au/La_0.67Sr_0.33MnO_3/SrTiO_3 interfaces
The effect of gold capping on magnetic and transport properties of optimally
doped manganite thin films is studied. An extraordinary suppression of
conductivity and magnetic properties occurs in epitaxial (001)
La_0.67Sr_0.33MnO_3 (LSMO) films grown on SrTiO_3 upon deposition of 2 nm of
Au: in the case of ultrathin films of LSMO (4 nm thick) the resistivity
increases by four orders of magnitude while the Curie temperature decreases by
180 K. Zero-field 55Mn nuclear magnetic resonance reveals a significant
reduction of ferromagnetic double-exchange mechanism in manganite films upon
the gold capping. We find evidence for the formation of a 1.9-nm thick magnetic
"dead-layer" at the Au/LSMO interface, associated with the creation of
interfacial non double-exchange insulating phases.Comment: 4 figure
Influence of Nd on the magnetic properties of Nd1-xCaxMnO3
The role played by the Nd ions in the magnetic properties of Nd0.5Ca0.5MnO3
and Nd0.7Ca0.3MnO3 is studied using static magnetization, neutron diffraction
and high frequency (9.4-475GHz) Electron Spin Resonance. We show that the Nd
ions are weakly coupled to the Mn ions via ferromagnetic exchange and are
responsible for the peculiar ferromagnetic resonance observed in the FM phase
of both compounds (ground state below 120K for x=0.3, high field state for
x=0.5). We then use ESR to look for magnetic phase separation in the low field,
CO phase of Nd0.5Ca0.5MnO3. We show that there is no trace of the FM phase
imbedded in the CO phase, contrary to what is observed in La0.5Ca0.5MnO3 or
Pr0.5Sr0.5MnO3.Comment: to be published in phys.Rev.B as a Rapid Com
Field-induced segregation of ferromagnetic nano-domains in PrSrMnO, detected by Mn NMR
The antiferromagnetic manganite PrSrMnO was investigated
at low temperature by means of magnetometry and Mn NMR. A field-induced
transition to a ferromagnetic state is detected by magnetization measurements
at a threshold field of a few tesla. NMR shows that the ferromagnetic phase
develops from zero field by the nucleation of microscopic ferromagnetic
domains, consisting of an inhomogeneous mixture of tilted and fully aligned
parts. At the threshold the NMR spectrum changes discontinuously into that of a
homogeneous, fully aligned, ferromagnetic state, suggesting a percolative
origin for the ferromagnetic transition.Comment: Latex 2.09 language. 4 pages, 3 figures, 23 references. Submitted to
physical Review
Correlated trends of coexisting magnetism and superconductivity in optimally electron-doped oxy-pnictides
We report on the recovery of the short-range static magnetic order and on the
concomitant degradation of the superconducting state in optimally F-doped
SmFe_(1-x)Ru_(x)AsO_0.85F_0.15 for 0.1< x<0.6. The two reduced order parameters
coexist within nanometer-size domains in the FeAs layers and finally disappear
around a common critical threshold x_c=0.6. Superconductivity and magnetism are
shown to be closely related to two distinct well-defined local electronic
environments of the FeAs layers. The two transition temperatures, controlled by
the isoelectronic and diamagnetic Ru substitution, scale with the volume
fraction of the corresponding environments. This fact indicates that
superconductivity is assisted by magnetic fluctuations, which are frozen
whenever a short-range static order appears, and totally vanish above the
magnetic dilution threshold x_c.Comment: Approved for publication in Phys. Rev. Letter
Singling out the effect of quenched disorder in the phase diagram of cuprates
We investigate the specific influence of structural disorder on the
suppression of antiferromagnetic order and on the emergence of cuprate
superconductivity. We single out pure disorder, by focusing on a series of
YEuBaCuO samples at fixed oxygen content
, in the range . The gradual Y/Eu isovalent substitution
smoothly drives the system through the Mott-insulator to superconductor
transition from a full antiferromagnet with N\'eel transition K at
to a bulk superconductor with superconducting critical temperature
K at , YBaCuO. The electronic properties are
finely tuned by gradual lattice deformations induced by the different cationic
radii of the two lanthanides, inducing a continuous change of the basal Cu(1)-O
chain length, as well as a controlled amount of disorder in the active
Cu(2)O bilayers. We check that internal charge transfer from the basal to
the active plane is entirely responsible for the doping of the latter and we
show that superconductivity emerges with orthorhombicity. By comparing
transition temperatures with those of the isoelectronic clean system we
deterime the influence of pure structural disorder connected with the Y/Eu
alloy.Comment: 10 pages 11 figures, submitted to Journal of Physics: Condensed
Matter, Special Issue in memory of Prof. Sandro Massid
Effect of two gaps on the flux lattice internal field distribution: evidence of two length scales from muSR in Mg1-xAlxB2
We have measured the transverse field muon spin precession in the flux
lattice (FL) state of the two gap superconductor MgB2 and of the electron doped
compounds Mg1-xAlxB2 in magnetic fields up to 2.8T. We show the effect of the
two gaps on the internal field distribution in the FL, from which we determine
two coherence length parameters and the doping dependence of the London
penetration depth. This is an independent determination of the complex vortex
structure already suggested by the STM observation of large vortices in a MgB2
single crystal. Our data agrees quantitatively with STM and we thus validate a
new phenomenological model for the internal fields.Comment: now in press Phys. Rev. Lett., small modifications required by the
edito
Fast recovery of the stripe magnetic order by Mn/Fe substitution in F-doped LaFeAsO superconductors
As Nuclear Magnetic (NMR) and Quadrupolar (NQR) Resonance were used,
together with M\"{o}ssbauer spectroscopy, to investigate the magnetic state
induced by Mn for Fe substitutions in F-doped LaFeMnAsO
superconductors. The results show that % of Mn doping is enough to
suppress the superconducting transition temperature from 27 K to zero and
to recover the magnetic structure observed in the parent undoped LaFeAsO. Also
the tetragonal to orthorhombic transition of the parent compound is recovered
by introducing Mn, as evidenced by a sharp drop of the NQR frequency. The NQR
spectra also show that a charge localization process is at play in the system.
Theoretical calculations using a realistic five-band model show that
correlation-enhanced RKKY exchange interactions between nearby Mn ions
stabilize the observed magnetic order, dominated by and
ordering vectors. These results give compelling evidence that
F-doped LaFeAsO is a strongly correlated electron system at the verge of an
electronic instability.Comment: 5 pages, 5 figures and 4 pages of supplemental materia
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