15 research outputs found
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Gap-mode Plasmonic Nanocavity
Here we describe the fabrication and characterization of a plasmonic nanocavity formed in the narrow gap between a Ag nanowire and a flat Ag substrate. The fluorescence spectrum of nanocrystals within the gap was strongly modified by the cavity modes, showing peaks of position and width (Q ∼ 30–60) in quantitative agreement with numerical calculations. At gap spacings of ∼ 15 nm, the noncavity background fluorescence is largely quenched by the Ag substrate, while the modal fluorescence remains strong, indicating that gap-type structures are more robust to fluorescence quenching.Engineering and Applied Science
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Controlled mode tuning in 1-D ‘RIM’ plasmonic crystal trench cavities probed with coupled optical emitters
We present a design of plasmonic cavities that consists of two sets of 1-D plasmonic crystal reflectors on a plasmonic trench waveguide. A 'reverse image mold' (RIM) technique was developed to pattern high-resolution silver trenches and to embed emitters at the cavity field maximum, and FDTD simulations were performed to analyze the frequency response of the fabricated devices. Distinct cavity modes were observed from the photoluminescence spectra of the organic dye embedded within these cavities. The cavity geometry facilitates tuning of the modes through a change in cavity dimensions. Both the design and the fabrication technique presented could be extended to making trench waveguide-based plasmonic devices and circuits.Engineering and Applied Science
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Weak Localization and Mobility in ZnO Nanostructures
We conduct a comprehensive investigation into the electronic and magnetotransport properties of ZnO nanoplates grown concurrently with ZnO nanowires by the vapor-liquid-solid method. We present magnetoresistance data showing weak localization in our nanoplates and probe its dependence on temperature and carrier concentration. We measure phase coherence lengths of 50–100 nm at 1.9 K and, because we do not observe spin-orbit scattering through antilocalization, suggest that ZnO nanostructures may be promising for further spintronic study. We then proceed to study the effect of weak localization on electron mobility using four-terminal van der Pauw resistivity and Hall measurements versus temperature and carrier concentration. We report an electron mobility of ∼100 cm2/V s at 275 K, comparable to what is observed in ZnO thin films. We compare Hall mobility to field-effect mobility, which is more commonly reported in studies on ZnO nanowires and find that field-effect mobility tends to overestimate Hall mobility by a factor of 2 in our devices. Finally, we comment on temperature-dependent hysteresis observed during transconductance measurements and its relationship to mobile, positively charged Zn interstitial impurities.Engineering and Applied Science
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Growth of ZnO Nanowires Catalyzed by Size-Dependent Melting of Au Nanoparticles
We present a general approach to growing ZnO nanowires on arbitrary, high melting point (above 970 °C) substrates using the vapor–liquid–solid (VLS) growth mechanism. Our approach utilizes the melting point reduction of sufficiently small (5 nm diameter) Au particles to provide a liquid catalyst without substrate interaction. Using this size-dependent melting effect, we demonstrate catalytic VLS growth of ZnO nanowires on both Ti and Mo foil substrates with aspect ratios in excess of 1000:1. Transmission electron microscopy shows the nanowires to be single-crystalline, and photoluminescence spectra show high-quality optical properties. We believe this growth technique to be widely applicable to a variety of substrates and material systems.Engineering and Applied Science
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Narrow Band Defect Luminescence from AI-doped ZnO Probed by Scanning Tunneling Cathodoluminescence
We present an investigation of optically active near-surface defects in sputtered Al-doped ZnO films using scanning tunneling microscope cathodoluminescence (STM-CL). STM-CL maps suggest that the optically active sites are distributed randomly across the surface and do not correlate with the granular topography. In stark contrast to photoluminescence results, STM-CL spectra show a series of sharp, discrete emissions that characterize the dominant optically active defect, which we propose is an oxygen vacancy. Our results highlight the ability of STM-CL to spectrally fingerprint individual defects and contribute to understanding the optical properties of near-surface defects in an important transparent conductor.Engineering and Applied Science
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Direct Injection Tunnel Spectroscopy of a p-n Junction
We demonstrate spectroscopic measurements on an InGaAs p-n junction using direct tunnel injection of electrons. In contrast to the metal-base transistor design of conventional ballistic electron emission spectroscopy (BEES), the base layer of our device is comprised of a thin, heavily doped p-type region. By tunneling directly into the semiconductor, we observe a significant increase in collector current compared to conventional BEES measurements. This could enable the study of systems and processes that have thus far been difficult to probe with the low-electron collection efficiency of conventional BEES, such as luminescence from single-buried quantum dots.Engineering and Applied Science
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Dislocation Density-Dependent Quality Factors in InGaN Quantum Dot Containing Microdisks
Microdisks incorporating InGaN quantum dots were fabricated using SiO2 microspheres as a hard mask in conjunction with a photoelectrochemical etch step from a structure containing a sacrificial InGaN/InGaN superlattice. Formation of microdisks from two near-identical structures with differing dislocation densities was carried out and investigated using microphotoluminescence. This confirmed the existence of quantum dots through the presence of resolution limited spectral lines and showed a clear correlation between the resulting modes quality factors and the dislocation densities within the disks. The disks with higher dislocation densities showed up to 80% lower quality factors than the low dislocation density disks.Engineering and Applied Science
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Scattering-Assisted Tunneling: Energy Dependence, Magnetic Field Dependence, and Use as an External Probe of Two-Dimensional Transport
For more than three decades, research on tunneling through planar barriers has focused principally on processes that conserve momentum parallel to the barrier. Here we investigate transport in which scattering destroys lateral momentum conservation and greatly enhances the tunneling probability. We have measured its energy dependence using capacitance spectroscopy, and we show that for electrons confined in a quantum well, the scattering enhancement can be quenched in an applied magnetic field, enabling this mechanism to function as an external probe of the origin of the quantum Hall effect.Engineering and Applied Science
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Magnetoresistance in an Asymmetric GaMnAs Resonant Tunneling Diode
In a GaMnAs/AlGaAs resonant tunneling diode (RTD) structure, we observe that both the magnitude and polarity of magnetoresistance are bias dependent when tunneling from a three-dimensional GaMnAs layer through a two-dimensional GaMnAs quantum well. This magnetoresistance behavior results from a shift of negative differential resistance features to higher bias as the relative alignment of the GaMnAs layer magnetizations is changed from parallel to antiparallel. Our observations agree with recent predictions from a theoretical analysis of a similar n-type structure by Ertler and Fabian, and our results suggest that further investigation into ferromagnetic RTD structures may result in significantly enhanced magnetoresistance.Engineering and Applied Science
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Low threshold, room-temperature microdisk lasers in the blue spectral range
InGaN-based active layers within microcavity resonators offer the potential of low threshold lasers in the blue spectral range. Here, we demonstrate optically pumped, room temperature lasing in high quality factor GaN microdisk cavities, containing InGaN quantum dots (QDs) with thresholds as low as . The demonstration of lasing action from GaN microdisk cavities with QDs in the active layer, provides a critical step for the nitrides in realizing low threshold photonic devices with efficient coupling between QDs and an optical cavity.Engineering and Applied Science