1,281 research outputs found
Commensurate Fluctuations in the Pseudogap and Incommensurate spin-Peierls Phases of TiOCl
X-ray scattering measurements on single crystals of TiOCl reveal the presence
of commensurate dimerization peaks within both the incommensurate spin-Peierls
phase and the so-called pseudogap phase above T_c2. This scattering is
relatively narrow in Q-space indicating long correlation lengths exceeding ~
100 A below T* ~ 130 K. It is also slightly shifted in Q relative to that of
the commensurate long range ordered state at the lowest temperatures, and it
coexists with the incommensurate Bragg peaks below T_c2. The integrated
scattering over both commensurate and incommensurate positions evolves
continuously with decreasing temperature for all temperatures below T* ~ 130 K.Comment: To appear in Physical Review B: Rapid Communications. 5 page
Critical X-ray Scattering Studies of Jahn-Teller Phase Transitions in TbVAsO
The critical behaviour associated with cooperative Jahn-Teller phase
transitions in TbVAsO (where \textit{x} = 0, 0.17, 1)
single crystals have been studied using high resolution x-ray scattering. These
materials undergo continuous tetragonal orthorhombic structural phase
transitions driven by Jahn-Teller physics at T = 33.26(2) K, 30.32(2) K and
27.30(2) K for \textit{x} = 0, 0.17 and 1 respectively. The orthorhombic strain
was measured close to the phase transition and is shown to display mean field
behavior in all three samples. Pronounced fluctuation effects are manifest in
the longitudinal width of the Bragg scattering, which diverges as a power law,
with an exponent given by , on approaching the transition from
either above or below. All samples exhibited twinning; however the disordered x
= 0.17 sample showed a broad distribution of twins which were stable to
relatively low temperatures, well below T. This indicates that while the
orthorhombic strain continues to develop in a conventional mean field manner in
the presence of disorder, twin domains are easily pinned by the quenched
impurities and their associated random strains.Comment: 8 pages, 6 figure
Suppression of the commensurate spin-Peierls state in Sc-doped TiOCl
We have performed x-ray scattering measurements on single crystals of the
doped spin-Peierls compound Ti(1-x)Sc(x)OCl (x = 0, 0.01, 0.03). These
measurements reveal that the presence of non-magnetic dopants has a profound
effect on the unconventional spin-Peierls behavior of this system, even at
concentrations as low as 1%. Sc-doping suppresses commensurate fluctuations in
the pseudogap and incommensurate spin-Peierls phases of TiOCl, and prevents the
formation of a long-range ordered spin-Peierls state. Broad incommensurate
scattering develops in the doped compounds near Tc2 ~ 93 K, and persists down
to base temperature (~ 7 K) with no evidence of a lock-in transition. The width
of the incommensurate dimerization peaks indicates short correlation lengths on
the order of ~ 12 angstroms below Tc2. The intensity of the incommensurate
scattering is significantly reduced at higher Sc concentrations, indicating
that the size of the associated lattice displacement decreases rapidly as a
function of doping.Comment: 7 pages, 5 figure
Design, Construction, and Qualification of a Microscale Heater Array for Use in Boiling Heat Transfer
Boiling heat transfer is an efficient means of heat transfer because a large amount of heat can be removed from a surface using a relatively small temperature difference between the surface and the bulk liquid. However, the mechanisms that govern boiling heat transfer are not well understood. Measurements of wall temperature and heat flux near the wall would add to the database of knowledge which is necessary to understand the mechanisms of nucleate boiling. A heater array has been developed which contains 96 heater elements within a 2.5 mm square area. The temperature of each heater element is held constant by an electronic control system similar to a hot-wire anemometer. The voltage that is being applied to each heater element can be measured and digitized using a high-speed A/D converter, and this digital information can be compiled into a series of heat-flux maps. Information for up to 10,000 heat flux maps can be obtained each second. The heater control system, the A/D system and the heater array construction are described in detail. Results are presented which show that this is an effective method of measuring the local heat flux during nucleate and transition boiling. Heat flux maps are obtained for pool boiling in FC-72 on a horizontal surface. Local heat flux variations are shown to be three to six times larger than variations in the spatially averaged heat flux
Structural Fluctuations in the Spin Liquid State of Tb2Ti2O7
High resolution X-ray scattering measurements on single crystal Tb2Ti2O7
reveal finite structural correlations at low temperatures. This geometrically
frustrated pyrochlore is known to exhibit a spin liquid, or cooperative
paramagnetic state, at temperatures below ~ 20 K. Parametric studies of
structural Bragg peaks appropriate to the Fdm space group of Tb2Ti2O7
reveal substantial broadening and peak intensity reduction in the temperature
regime 20 K to 300 mK. We also observe a small, anomalous lattice expansion on
cooling below a density maximum at ~ 18 K. These measurements are consistent
with the development of fluctuations above a cooperative Jahn-Teller,
cubic-tetragonal phase transition at very low temperatures.Comment: 5 pages, 4 figures, submitted for publicatio
Nature of the spin dynamics and 1/3 magnetization plateau in azurite
We present a specific heat and inelastic neutron scattering study in magnetic
fields up into the 1/3 magnetization plateau phase of the diamond chain
compound azurite Cu(CO)(OH). We establish that the
magnetization plateau is a dimer-monomer state, {\it i.e.}, consisting of a
chain of monomers, which are separated by dimers on the
diamond chain backbone. The effective spin couplings K
and K are derived from the monomer and dimer
dispersions. They are associated to microscopic couplings K,
K and a ferromagnetic K, possibly as
result of orbitals in the Cu-O bonds providing the superexchange
pathways.Comment: 5 pages, 4 figure
phase i ii first in human trial with m7583 a bruton s tyrosine kinase inhibitor btki in patients with b cell malignancies
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Magnetoelastic and structural properties of azurite Cu3(CO3)2(OH)2 from neutron scattering and muon spin rotation
Azurite, Cu3(CO3)2(OH)2, has been considered an ideal example of a
one-dimensional (1D) diamond chain antiferromagnet. Early studies of this
material imply the presence of an ordered antiferromagnetic phase below K while magnetization measurements have revealed a 1/3 magnetization
plateau. Until now, no corroborating neutron scattering results have been
published to confirm the ordered magnetic moment structure. We present recent
neutron diffraction results which reveal the presence of commensurate magnetic
order in azurite which coexists with significant magnetoelastic strain. The
latter of these effects may indicate the presence of spin frustration in zero
applied magnetic field. Muon spin rotation, SR, reveals an onset of
short-range order below 3K and confirms long-range order below .Comment: 5 pages, 4 figures, PHYSICAL REVIEW B 81, 140406(R) (2010
The association between benign prostatic hyperplasia and chronic kidney disease in community-dwelling men
The association between benign prostatic hyperplasia and chronic kidney disease in community-dwelling men.BackgroundBenign prostatic hyperplasia (BPH) and chronic kidney disease are important public health problems in older men. Previous referral-based studies disagree on whether BPH is associated with chronic kidney disease. The objective of this study was to determine the community-based association between clinical measures of BPH and chronic kidney disease.MethodsA community-based sample of 2115 white men (ages 40–79 years) was randomly selected from the Olmsted County, Minnesota population (55% participation rate) in 1990. A random subsample (N = 476) had a detailed clinical evaluation. This evaluation included a questionnaire with similar queries to the International Prostate Symptom Score (IPSS), peak urinary flow rates (uroflowmeter), postvoid residual urine volume (ultrasound), prostate volume (ultrasound), serum prostate specific antigen (PSA), and serum creatinine.ResultsAfter adjustment for age, hypertension, diabetes, leukocyte esterase positive (possible urinary tract infection), and smoking, chronic kidney disease [serum creatinine ≥133 μmol/L (1.5 mg/dL)] was associated with diminished peak urinary flow rate (<15 mL/sec) by an odds ratio (OR) = 2.96 (95% CI 1.30–7.01), moderate-severe lower urinary tract symptoms (IPSS >7) by an OR = 2.91 (95% CI 1.32–6.62), and chronic urinary retention (postvoid residual >100 mL) by an OR = 2.28 (95% CI 0.66–6.68). There was no association with a prostate volume >30 mL by an OR = 0.56 (95% CI 0.22–1.37) or PSA >1.4 ng/mL by an OR = 1.17 (95% CI 0.47–2.81).ConclusionThere was a cross-sectional association between signs and symptoms of bladder outlet obstruction and chronic kidney disease in community-dwelling men. Prostatic enlargement was not associated with chronic kidney disease
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