470 research outputs found
Frenkel and charge transfer excitons in C60
We have studied the low energy electronic excitations of C60 using momentum
dependent electron energy-loss spectroscopy in transmission. The momentum
dependent intensity of the gap excitation allows the first direct experimental
determination of the energy of the 1Hg excitation and thus also of the total
width of the multiplet resulting from the gap transition. In addition, we could
elucidate the nature of the following excitations - as either Frenkel or charge
transfer excitons.Comment: RevTEX, 3 Figures, to appear in Phys. Rev.
Fungal Planet description sheets: 92–106
Novel species of microfungi described in the present study include the following from Australia: Diaporthe ceratozamiae on Ceratozamia robusta, Seiridium banksiae on Banksia marginata, Phyllosticta hymenocallidicola on Hymenocallis littoralis, Phlogicylindrium uniforme on Eucalyptus cypellocarpa, Exosporium livistonae on Livistona benthamii and Coleophoma eucalyptorum on Eucalyptus piperita. Several species are also described from South Africa, namely: Phoma proteae, Pyrenochaeta protearum and Leptosphaeria proteicola on Protea spp., Phaeomoniella niveniae on Nivenia stokoei, Toxicocladosporium leucadendri on Leucadendron sp. and Scorias leucadendri on Leucadendron muirii. Other species include Myrmecridium phragmitis on Phragmites australis (Netherlands) and Camarographium carpini on Carpinus betulus (Russia). Furthermore, Pseudoidriella syzygii on Syzygium sp. represents a novel genus of hyphomycetes collected in Australia. Morphological and culture characteristics along with ITS DNA barcodes are provided for all taxa
Strong correlation effects in the doped Hubbard model in infinite dimensions
The density of states and the optical conductivity of the doped Hubbard model
on a Bethe lattice with infinite connectivities have been studied using an
analytic variant of the Lanczos continued fraction method. The spectral weight
of the gap states and the position of the chemical potential upon hole or
electron doping have been studied. We argue that the strong correlation effects
such as gap states and midinfrared band shown in two dimensions also appear in
infinite dimensions.Comment: 9 pages, revtex, 3 figures upon reques
Theory for Dynamical Short Range Order and Fermi Surface Volume in Strongly Correlated Systems
Using the fluctuation exchange approximation of the one band Hubbard model,
we discuss the origin of the changing Fermi surface volume in underdoped
cuprate systems due to the transfer of occupied states from the Fermi surface
to its shadow, resulting from the strong dynamical antiferromagnetic short
range correlations. The momentum and temperature dependence of the quasi
particle scattering rate shows unusual deviations from the conventional Fermi
liquid like behavior. Their consequences for the changing Fermi surface volume
are discussed. Here, we investigate in detail which scattering processes
might be responsible for a violation of the Luttinger theorem. Finally, we
discuss the formation of hole pockets near half filling.Comment: 5 pages, Revtex, 4 postscript figure
Magnetic Properties of YBa_2Cu_3O_{7-\delta} in a self-consistent approach: Comparison with Quantum-Monte-Carlo Simulations and Experiments
We analyze single-particle electronic and two-particle magnetic properties of
the Hubbard model in the underdoped and optimally-doped regime of \YBCO by
means of a modified version of the fluctuation-exchange approximation, which
only includes particle-hole fluctuations. Comparison of our results with
Quantum-Monte Carlo (QMC) calculations at relatively high temperatures () suggests to introduce a temperature renormalization in order to
improve the agreement between the two methods at intermediate and large values
of the interaction .
We evaluate the temperature dependence of the spin-lattice relaxation time
and of the spin-echo decay time and compare it with the results
of NMR measurements on an underdoped and an optimally doped \YBCO sample. For
it is possible to consistently adjust the parameters of the Hubbard
model in order to have a good {\it semi-quantitative} description of this
temperature dependence for temperatures larger than the spin gap as obtained
from NMR measurements. We also discuss the case , which is more
appropriate to describe magnetic and single-particle properties close to
half-filling. However, for this larger value of the agreement with QMC as
well as with experiments at finite doping is less satisfactory.Comment: Final version, to appear in Phys. Rev. B (sched. Feb. 99
Superconductivity in the two dimensional Hubbard Model.
Quasiparticle bands of the two-dimensional Hubbard model are calculated using
the Roth two-pole approximation to the one particle Green's function. Excellent
agreement is obtained with recent Monte Carlo calculations, including an
anomalous volume of the Fermi surface near half-filling, which can possibly be
explained in terms of a breakdown of Fermi liquid theory. The calculated bands
are very flat around the (pi,0) points of the Brillouin zone in agreement with
photoemission measurements of cuprate superconductors. With doping there is a
shift in spectral weight from the upper band to the lower band. The Roth method
is extended to deal with superconductivity within a four-pole approximation
allowing electron-hole mixing. It is shown that triplet p-wave pairing never
occurs. Singlet d_{x^2-y^2}-wave pairing is strongly favoured and optimal
doping occurs when the van Hove singularity, corresponding to the flat band
part, lies at the Fermi level. Nearest neighbour antiferromagnetic correlations
play an important role in flattening the bands near the Fermi level and in
favouring superconductivity. However the mechanism for superconductivity is a
local one, in contrast to spin fluctuation exchange models. For reasonable
values of the hopping parameter the transition temperature T_c is in the range
10-100K. The optimum doping delta_c lies between 0.14 and 0.25, depending on
the ratio U/t. The gap equation has a BCS-like form and (2*Delta_{max})/(kT_c)
~ 4.Comment: REVTeX, 35 pages, including 19 PostScript figures numbered 1a to 11.
Uses epsf.sty (included). Everything in uuencoded gz-compressed .tar file,
(self-unpacking, see header). Submitted to Phys. Rev. B (24-2-95
Parameters of the Effective Singlet-Triplet Model for Band Structure of High- Cuprates by Different Approaches
The present paper covers the problem of parameters determination for
High- superconductive copper oxides. Different approaches, {\it ab initio}
LDA and LDA+U calculations and Generalized Tight-Binding (GTB) method for
strongly correlated electron systems, are used to calculate hopping and
exchange parameters of the effective singlet-triplet model for -layer.
The resulting parameters are in remarkably good agreement with each other and
with parameters extracted from experiment. This set of parameters is proposed
for proper quantitative description of physics of hole doped High-
cuprates in the framework of effective models.Comment: PACS 74.72.h; 74.20.z; 74.25.Jb; 31.15.A
Correlated local distortions of the TlO layers in TlBaCuO: An x-ray absorption study
We have used the XAFS (x-ray-absorption fine structure) technique to
investigate the local structure about the Cu, Ba, and Tl atoms in orthorhombic
Tl-2201 with a superconducting transition temperature T=60 K. Our results
clearly show that the O(1), O(2), Cu, and Ba atoms are at their ideal sites as
given by the diffraction measurements, while the Tl and O(3) atoms are more
disordered than suggested by the average crystal structure. The Tl-Tl distance
at 3.5 \AA{ } between the TlO layers does not change, but the Tl-Tl distance at
3.9 \AA{ } within the TlO layer is not observed and the Tl-Ba and Ba-Tl peaks
are very broad. The shorter Tl-O(3) distance in the TlO layer is about 2.33
\AA, significantly shorter than the distance calculated with both the Tl and
O(3) atoms at their ideal sites ( 0 or ). A model based
on these results shows that the Tl atom is displaced along the
directions from its ideal site by about 0.11 \AA; the displacements of
neighboring Tl atoms are correlated. The O(3) atom is shifted from the $4e$
site by about 0.53 \AA{ } roughly along the directions. A comparison of
the Tl L-edge XAFS spectra from three samples, with T=60 K, 76 K,
and 89 K, shows that the O environment around the Tl atom is sensitive to T
while the Tl local displacement is insensitive to T and the structural
symmetry. These conclusions are compared with other experimental results and
the implications for charge transfer and superconductivity are discussed. This
paper has been submitted to Phys. Rev. B.Comment: 20 pages plus 14 ps figures, REVTEX 3.
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Reprogramming human T cell function and specificity with non-viral genome targeting.
Decades of work have aimed to genetically reprogram T cells for therapeutic purposes1,2 using recombinant viral vectors, which do not target transgenes to specific genomic sites3,4. The need for viral vectors has slowed down research and clinical use as their manufacturing and testing is lengthy and expensive. Genome editing brought the promise of specific and efficient insertion of large transgenes into target cells using homology-directed repair5,6. Here we developed a CRISPR-Cas9 genome-targeting system that does not require viral vectors, allowing rapid and efficient insertion of large DNA sequences (greater than one kilobase) at specific sites in the genomes of primary human T cells, while preserving cell viability and function. This permits individual or multiplexed modification of endogenous genes. First, we applied this strategy to correct a pathogenic IL2RA mutation in cells from patients with monogenic autoimmune disease, and demonstrate improved signalling function. Second, we replaced the endogenous T cell receptor (TCR) locus with a new TCR that redirected T cells to a cancer antigen. The resulting TCR-engineered T cells specifically recognized tumour antigens and mounted productive anti-tumour cell responses in vitro and in vivo. Together, these studies provide preclinical evidence that non-viral genome targeting can enable rapid and flexible experimental manipulation and therapeutic engineering of primary human immune cells
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