190 research outputs found
Unusual temperature dependence of band dispersion in Ba(Fe(1-x)Ru(x))2As2 and its consequences for antiferromagnetic ordering
We have performed detailed studies of the temperature evolution of the
electronic structure in Ba(Fe(1-x)Ru(x))2As2 using Angle Resolved Photoemission
Spectroscopy (ARPES). Surprisingly, we find that the binding energy of both
hole and electron bands changes significantly with temperature in pure and Ru
substituted samples. The hole and electron pockets are well nested at low
temperature in unsubstituted (BaFe2As2) samples, which likely drives the spin
density wave (SDW) and resulting antiferromagnetic order. Upon warming, this
nesting is degraded as the hole pocket shrinks and the electron pocket expands.
Our results demonstrate that the temperature dependent nesting may play an
important role in driving the antiferromagnetic/paramagnetic phase transition.Comment: 5 pages, 6 figure
Evolution from a nodeless gap to d(x2-y2) form in underdoped La(2-x)SrxCuO4
Using angle-resolved photoemission (ARPES), it is revealed that the
low-energy electronic excitation spectra of highly underdoped superconducting
and non-superconducting La(2-x)SrxCuO4 cuprates are gapped along the entire
underlying Fermi surface at low temperatures. We show how the gap function
evolves to a d(x2-y2) form as increasing temperature or doping, consistent with
the vast majority of ARPES studies of cuprates. Our results provide essential
information for uncovering the symmetry of the order parameter(s) in strongly
underdoped cuprates, which is a prerequisite for understanding the pairing
mechanism and how superconductivity emerges from a Mott insulator.Comment: 5 pages, 4 figure
Possible nodal superconducting gap emerging at the Lifshitz transition in heavily hole-doped Ba0.1K0.9Fe2As2
We performed a high energy resolution ARPES investigation of over-doped
Ba0.1K0.9Fe2As2 with T_c= 9 K. The Fermi surface topology of this material is
similar to that of KFe2As2 and differs from that of slightly less doped
Ba0.3K0.7Fe2As2, implying that a Lifshitz transition occurred between x=0.7 and
x=0.9. Albeit for a vertical node found at the tip of the emerging
off-M-centered Fermi surface pocket lobes, the superconducting gap structure is
similar to that of Ba0.3K0.7Fe2As2, suggesting that the paring interaction is
not driven by the Fermi surface topology.Comment: 5 pages, 4 figure
Disorder Induced Stripes in d-Wave Superconductors
Stripe phases are observed experimentally in several copper-based high-Tc
superconductors near 1/8 hole doping. However, the specific characteristics may
vary depending on the degree of dopant disorder and the presence or absence of
a low- temperature tetragonal phase. On the basis of a Hartree-Fock decoupling
scheme for the t-J model we discuss the diverse behavior of stripe phases. In
particular the effect of inhomogeneities is investigated in two distinctly
different parameter regimes which are characterized by the strength of the
interaction. We observe that small concen- trations of impurities or vortices
pin the unidirectional density waves, and dopant disorder is capable to
stabilize a stripe phase in parameter regimes where homogeneous phases are
typically favored in clean systems. The momentum-space results exhibit
universal features for all coexisting density-wave solutions, nearly unchanged
even in strongly disordered systems. These coexisting solutions feature
generically a full energy gap and a particle-hole asymmetry in the density of
states.Comment: 28 pages, 8 figure
Bulk electronic structure of superconducting LaRu2P2 single crystals measured by soft x-ray angle-resolved photoemission spectroscopy
We present a soft X-ray angle-resolved photoemission spectroscopy (SX-ARPES)
study of the stoichiometric pnictide superconductor LaRu2P2. The observed
electronic structure is in good agreement with density functional theory (DFT)
calculations. However, it is significantly different from its counterpart in
high-temperature superconducting Fe-pnictides. In particular the bandwidth
renormalization present in the Fe-pnictides (~2 - 3) is negligible in LaRu2P2
even though the mass enhancement is similar in both systems. Our results
suggest that the superconductivity in LaRu2P2 has a different origin with
respect to the iron pnictides. Finally we demonstrate that the increased
probing depth of SX-ARPES, compared to the widely used ultraviolet ARPES, is
essential in determining the bulk electronic structure in the experiment.Comment: 4 pages, 4 figures, 1 supplemental material. Accepted for publication
in Physical Review Letter
Emergence of pseudogap from short-range spin-correlations in electron doped cuprates
Electron interactions are pivotal for defining the electronic structure of
quantum materials. In particular, the strong electron Coulomb repulsion is
considered the keystone for describing the emergence of exotic and/or ordered
phases of quantum matter as disparate as high-temperature superconductivity and
charge- or magnetic-order. However, a comprehensive understanding of
fundamental electronic properties of quantum materials is often complicated by
the appearance of an enigmatic partial suppression of low-energy electronic
states, known as the pseudogap. Here we take advantage of ultrafast
angle-resolved photoemission spectroscopy to unveil the temperature evolution
of the low-energy density of states in the electron-doped cuprate
NdCeCuO, an emblematic system where
the pseudogap intertwines with magnetic degrees of freedom. By photoexciting
the electronic system across the pseudogap onset temperature T*, we report the
direct relation between the momentum-resolved pseudogap spectral features and
the spin-correlation length with an unprecedented sensitivity. This transient
approach, corroborated by mean field model calculations, allows us to establish
the pseudogap in electron-doped cuprates as a precursor to the incipient
antiferromagnetic order even when long-range antiferromagnetic correlations are
not established, as in the case of optimal doping.Comment: 17 pages, 3 figure
Spectroscopic evidence for preformed Cooper pairs in the pseudogap phase of cuprates
Angle-resolved photoemission on underdoped LaSrCuO
reveals that in the pseudogap phase, the dispersion has two branches located
above and below the Fermi level with a minimum at the Fermi momentum. This is
characteristic of the Bogoliubov dispersion in the superconducting state. We
also observe that the superconducting and pseudogaps have the same d-wave form
with the same amplitude. Our observations provide direct evidence for preformed
Cooper pairs, implying that the pseudogap phase is a precursor to
superconductivity
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