5 research outputs found
Enhanced generation of VUV radiation by four-wave mixing in mercury using pulsed laser vaporization
The efficiency of a coherent VUV source at 125 nm, based on 2-photon resonant
four-wave mixing in mercury vapor, has been enhanced by up to 2 orders of
magnitude. This enhancement was obtained by locally heating a liquid Hg surface
with a pulsed excimer laser, resulting in a high density vapor plume in which
the nonlinear interaction occurred. Energies up to 5 μJ (1 kW peak power)
have been achieved while keeping the overall Hg cell at room temperature,
avoiding the use of a complex heat pipe. We have observed a strong saturation
of the VUV yield when peak power densities of the fundamental beams exceed the
GW/cm2 range, as well as a large intensity-dependant broadening (up to ~30
cm-1) of the two-photon resonance. The source has potential applications for
high resolution interference lithography and photochemistry