Length-dependent oscillations of the conductance through atomic chains: The importance of electronic correlations

We calculate the conductance of atomic chains as a function of their length. Using the Density Matrix Renormalization Group algorithm for a many-body model which takes into account electron-electron interactions and the shape of the contacts between the chain and the leads, we show that length-dependent oscillations of the conductance whose period depends on the electron density in the chain can result from electron-electron scattering alone. The amplitude of these oscillations can increase with the length of the chain, in contrast to the result from approaches which neglect the interactions.Comment: 7 pages, 4 figure

Spin blockade in ground state resonance of a quantum dot

We present measurements on spin blockade in a laterally integrated quantum dot. The dot is tuned into the regime of strong Coulomb blockade, confining ~ 50 electrons. At certain electronic states we find an additional mechanism suppressing electron transport. This we identify as spin blockade at zero bias, possibly accompanied by a change in orbital momentum in subsequent dot ground states. We support this by probing the bias, magnetic field and temperature dependence of the transport spectrum. Weak violation of the blockade is modelled by detailed calculations of non-linear transport taking into account forbidden transitions.Comment: 4 pages, 4 figure

Influence of nano-mechanical properties on single electron tunneling: A vibrating Single-Electron Transistor

We describe single electron tunneling through molecular structures under the influence of nano-mechanical excitations. We develop a full quantum mechanical model, which includes charging effects and dissipation, and apply it to the vibrating C$_{60}$ single electron transistor experiment by Park {\em et al.} {[Nature {\bf 407}, 57 (2000)].} We find good agreement and argue vibrations to be essential to molecular electronic systems. We propose a mechanism to realize negative differential conductance using local bosonic excitations.Comment: 7 pages, 6 figure

Electron Transport through Disordered Domain Walls: Coherent and Incoherent Regimes

We study electron transport through a domain wall in a ferromagnetic nanowire subject to spin-dependent scattering. A scattering matrix formalism is developed to address both coherent and incoherent transport properties. The coherent case corresponds to elastic scattering by static defects, which is dominant at low temperatures, while the incoherent case provides a phenomenological description of the inelastic scattering present in real physical systems at room temperature. It is found that disorder scattering increases the amount of spin-mixing of transmitted electrons, reducing the adiabaticity. This leads, in the incoherent case, to a reduction of conductance through the domain wall as compared to a uniformly magnetized region which is similar to the giant magnetoresistance effect. In the coherent case, a reduction of weak localization, together with a suppression of spin-reversing scattering amplitudes, leads to an enhancement of conductance due to the domain wall in the regime of strong disorder. The total effect of a domain wall on the conductance of a nanowire is studied by incorporating the disordered regions on either side of the wall. It is found that spin-dependent scattering in these regions increases the domain wall magnetoconductance as compared to the effect found by considering only the scattering inside the wall. This increase is most dramatic in the narrow wall limit, but remains significant for wide walls.Comment: 23 pages, 12 figure

Groups of Galaxies in the Two Micron All-Sky Redshift Survey

We present the results of applying a percolation algorithm to the initial release of the Two Micron All-Sky Survey Extended Source Catalog, using subsequently measured redshifts for almost all of the galaxies with K < 11.25 mag. This group catalog is based on the first near-IR all-sky flux-limited survey that is complete to |b| = 5 deg. We explore the dependence of the clustering on the length and velocity scales involved. The paper describes a group catalog, complete to a limiting redshift of 10,000 km/s, created by maximizing the number of groups containing 3 or more members. A second catalog is also presented, created by requiring a minimum density contrast of 80 to identify groups. We identify known nearby clusters in the catalogs and contrast the groups identified in the two catalogs. We examine and compare the properties of the determined groups and verify that the results are consistent with the UZC-SSRS2 and northern CfA redshift survey group catalogs. The all-sky nature of the catalog will allow the development of a flow-field model based on the density field inferred from the estimated cluster masses.Comment: Accepted for publication in ApJ (29 pages including 13 figures). A version with high-resolution figures is available at http://www.cfa.harvard.edu/~acrook/preprints

Level Statistics and Localization for Two Interacting Particles in a Random Potential

We consider two particles with a local interaction $U$ in a random potential at a scale $L_1$ (the one particle localization length). A simplified description is provided by a Gaussian matrix ensemble with a preferential basis. We define the symmetry breaking parameter $\mu \propto U^{-2}$ associated to the statistical invariance under change of basis. We show that the Wigner-Dyson rigidity of the energy levels is maintained up to an energy $E_{\mu}$. We find that $E_{\mu} \propto 1/\sqrt{\mu}$ when $\Gamma$ (the inverse lifetime of the states of the preferential basis) is smaller than $\Delta_2$ (the level spacing), and $E_{\mu} \propto 1/\mu$ when $\Gamma > \Delta_2$. This implies that the two-particle localization length $L_2$ first increases as $|U|$ before eventually behaving as $U^2$.Comment: 4 pages REVTEX, 4 Figures EPS, UUENCODE

Spin-Blockade in Single and Double Quantum Dots in Magnetic Fields: a Correlation Effect

The total spin of correlated electrons in a quantum dot changes with magnetic field and this effect is generally linked to the change in the total angular momentum from one magic number to another, which can be understood in terms of an `electron molecule' picture for strong fields. Here we propose to exploit this fact to realize a spin blockade, i.e., electrons are prohibited to tunnel at specific values of the magnetic field. The spin-blockade regions have been obtained by calculating both the ground and excited states. In double dots the spin-blockade condition is found to be less stringent than in single dots.Comment: 4pages, to be published in Phys. Rev. B (Rapid Communication

Nuclear spin relaxation probed by a single quantum dot

We present measurements on nuclear spin relaxation probed by a single quantum dot in a high-mobility electron gas. Current passing through the dot leads to a spin transfer from the electronic to the nuclear spin system. Applying electron spin resonance the transfer mechanism can directly be tuned. Additionally, the dependence of nuclear spin relaxation on the dot gate voltage is observed. We find electron-nuclear relaxation times of the order of 10 minutes

Residual conductance of correlated one-dimensional nanosystems: A numerical approach

We study a method to determine the residual conductance of a correlated system by means of the ground-state properties of a large ring composed of the system itself and a long non-interacting lead. The transmission probability through the interacting region and thus its residual conductance is deduced from the persistent current induced by a flux threading the ring. Density Matrix Renormalization Group techniques are employed to obtain numerical results for one-dimensional systems of interacting spinless fermions. As the flux dependence of the persistent current for such a system demonstrates, the interacting system coupled to an infinite non-interacting lead behaves as a non-interacting scatterer, but with an interaction dependent elastic transmission coefficient. The scaling to large lead sizes is discussed in detail as it constitutes a crucial step in determining the conductance. Furthermore, the method, which so far had been used at half filling, is extended to arbitrary filling and also applied to disordered interacting systems, where it is found that repulsive interaction can favor transport.Comment: 14 pages, 10 EPS figure

Tc-Glutathione Complex (Tc -GSH) : Labelling, Chemical Characterization and Biodistribution in Rats

The chemical structure of 99mTc-GSH has been estabilished using the 99Tc isotope. Labeling of glutathione with technetium in the presence of stanous chloride gave a high yield result. In a comparative study between 99Tc and 99Tc glutathione, the Tc-GSH complex obtained was purified and characterized by uv, visible spectroscopy, HPLC, Biogel chromatography, mass and NMR spectroscopy. Stoichiometric analysis showed a 2 : 1 molar ratio of GSH/Tc for the reaction. The molecular mass assessed by mass spectroscopy was 727 Da corresponding to an oxo(bis) glutathione technetate. NMR studies demonstrated that each glutathione molecule was coordinated to technetium via cysteinyl sulfur and nitrogen atoms. The biodistribution of the complex was studied in normal rats. Blood clearance was rapid during the first hour involving a biexponential curve ( t1/2 (1) : 50 min, t1/2 (2) : 400 min ). No radioactive accumulation was found in any specific organ except kidney and bladder. All the activity excreted was found unchanged in urine. In conclusion, Tc-GSH displayed an anionic dimer form as GSH-Tc-GSH. We assume that the complex is a tetradentate (2N,2S) complex containing a pentavalent technetium coordinated by two thiol and nitrogen atoms of both GSH ligands, and an apical oxo group