72 research outputs found
Anomalous Self-Energy Effects of the B_1g Phonon in Y_{1-x}(Pr,Ca)_xBa_2Cu_3O_7 Films
In Raman spectra of cuprate superconductors the gap shows up both directly,
via a redistribution of the electronic background, the so-called "2Delta
peaks", and indirectly, e.g. via the renormalization of phononic excitations.
We use a model that allows us to study the redistribution and the related
phonon self-energy effects simultaneously. We apply this model to the B_1g
phonon of Y_{1-x}(Pr,Ca)_xBa_2Cu_3O_7 films, where Pr or Ca substitution
enables us to investigate under- and overdoped samples. While various
self-energy effects can be explained by the strength and energy of the 2\Delta
peaks, anomalies remain. We discuss possible origins of these anomalies.Comment: 6 pages including 4 figure
Raman scattering studies of temperature- and field-induced melting of charge order in (La,Pr,Ca)MnO
We present Raman scattering studies of the structural and magnetic phases
that accompany temperature- and field-dependent melting of charge- and
orbital-order (COO) in La0.5Ca0.5MnO3 and La0.25Pr0.375Ca0.375MnO3. Our results
show that thermal and field-induced COO melting in La0.5Ca0.5MnO3 exhibits
three stages in a heterogeneous melting process associated with a structural
change: a long-range, strongly JT distorted/COO regime; a coexistence regime;
and weakly JT distorted/PM or FM phase. We provide a complete structural phase
diagram of La0.5Ca0.5MnO3 for the temperature and field ranges 6<=T<=170 K and
0<=H<=9 T. We also investigate thermal and field-induced melting in
La0.25Pr0.375Ca0.375MnO3 to elucidate the role of disorder in melting of COO.
We find that while thermal melting of COO in La0.25Pr0.375Ca0.375MnO3 is quite
similar to that in La0.5Ca0.5MnO3, the field-induced transition from the COO
phase to the weakly JT-distorted/FM phase in La0.25Pr0.375Ca0.375MnO3 is very
abrupt, and occurs at significantly lower fields (H~2 T at T~0 K) than in
La0.5Ca0.5MnO3 (H~30 T at T=0 K). Moreover, the critical field H_c increases
with increasing temperature in La0.25Pr0.375Ca0.375MnO3 in contrast to
La0.5Ca0.5MnO3. To explain these differences, we propose that field-induced
melting of COO in La0.25Pr0.375Ca0.375MnO3 is best described as the
field-induced percolation of FM domains, and we suggest that Griffiths phase
physics may be an appropriate theoretical model for describing the unusual
temperature- and field- dependent transitions observed in
La0.25Pr0.375Ca0.375MnO3.Comment: 14 pages, 8 figures, to be published in PR
Relation between the superconducting gap energy and the two-magnon Raman peak energy in Bi2Sr2Ca{1-x}YxCu2O{8+\delta}
The relation between the electronic excitation and the magnetic excitation
for the superconductivity in Bi2Sr2Ca{1-x}YxCu2O{8+\delta} was investigated by
wide-energy Raman spectroscopy. In the underdoping region the B1g scattering
intensity is depleted below the two-magnon peak energy due to the "hot spots"
effects. The depleted region decreases according to the decrease of the
two-magnon peak energy, as the carrier concentration ncreases. This two-magnon
peak energy also determines the B1g superconducting gap energy as
from under to overdoping hole concentration.Comment: 10 pages, 4 figure
Conductance-strain behavior in silver-nanowire composites: network properties of a tunable strain sensor
Highly flexible and conductive nano-composite materials are promising candidates for stretchable and flexible electronics. We report on the strain–resistance relation of a silver-nanowire photopolymer composite during repetitive stretching. Resistance measurements reveal a gradual change of the hysteretic resistance curves towards a linear and non-hysteretic behavior. Furthermore, a decrease in resistance and an increase in electrical sensitivity to strain over the first five stretching cycles can be observed. Sensitivity gauge factors between 10 and 500 at 23% strain were found depending on the nanowire concentration and stretching cycle. We model the electrical behavior of the investigated silver nanowire composites upon repetitive stretching considering the strain induced changes in the local force distribution within the polymer matrix and the tunnel resistance between the nanowires by using a Monte Carlo method
Emerging giant resonant exciton induced by Ta-substitution in anatase TiO: a tunable correlation effect
Titanium dioxide (TiO) has rich physical properties with potential
implications in both fundamental physics and new applications. Up-to-date, the
main focus of applied research is to tune its optical properties, which is
usually done via doping and/or nano-engineering. However, understanding the
role of -electrons in materials and possible functionalization of
-electron properties are still major challenges. Herewith, within a
combination of an innovative experimental technique, high energy optical
conductivity, and of the state-of-the-art {\it ab initio} electronic structure
calculations, we report an emerging, novel resonant exciton in the deep
ultraviolet region of the optical response. The resonant exciton evolves upon
low concentration Ta-substitution in anatase TiO films. It is
surprisingly robust and related to strong electron-electron and electron-hole
interactions. The - and - orbitals localization, due to Ta-substitution,
plays an unexpected role, activating strong electronic correlations and
dominating the optical response under photoexcitation. Our results shed light
on a new optical phenomenon in anatase TiO films and on the possibility
of tuning electronic properties by Ta substitution
Electrical and network properties of flexible silver-nanowire composite electrodes under mechanical strain
Flexible and conductive silver-nanowire photopolymer composites are fabricated and studied under mechanical strain. The initial resistances of the unstretched flexible composites are between 0.27 Ω mm−1 and 1.2 Ω mm−1 for silver-nanowire concentrations between 120 μg cm−2 and 40 μg cm−2. Stretching of the samples leads to an increased resistance by a factor of between 72 for 120 μg cm−2 and 343 for 40 μg cm−2 at elongations of 23%. In order to correlate network morphology and electrical properties, micrographs are recorded during stretching. The Fiber Image Network Evaluation (FINE) algorithm determines morphological silver-nanowire network properties under stretching. For unstretched and stretched samples, an isotropic nanowire network is found with only small changes in fiber orientation. Monte-Carlo simulations on 2D percolation networks of 1D conductive wires and the corresponding network resistance due to tunneling of electrons at nanowire junctions confirm that the elastic polymer matrix under strain exhibits forces in agreement with Hooke's law. By variation of a critical force distribution the resistance curves are accurately reproduced. This results in a model that is dominated by quantum-mechanical tunneling at nanowire junctions explaining the electrical behavior and the sensitivity of nanowire-composites with different filler concentrations under mechanical strain
Raman scattering in a two-dimensional electron gas: Boltzmann equation approach
The inelastic light scattering in a 2-d electron gas is studied theoretically
using the Boltzmann equation techniques. Electron-hole excitations produce the
Raman spectrum essentially different from the one predicted for the 3-d case.
In the clean limit it has the form of a strong non-symmetric resonance due to
the square root singularity at the electron-hole frequency while
in the opposite dirty limit the usual Lorentzian shape of the cross section is
reestablished. The effects of electromagnetic field are considered
self-consistently and the contribution from collective plasmon modes is found.
It is shown that unlike 3-d metals where plasmon excitations are unobservable
(because of very large required transfered frequencies), the two-dimensional
electron system gives rise to a low-frequency ()
plasmon peak. A measurement of the width of this peak can provide data on the
magnitude of the electron scattering rate.Comment: 4 pages, 3 figures. to appear in Phys. Rev. B 59 (1999
Raman scattering study of anomalous charge-, spin-, and lattice-dynamics in the charge-ordered phase of ()
We report an inelastic light scattering study of the effects of
charge-ordering on the spin-, charge-, and lattice-dynamics in . We find that charge-ordering
results in anomalous phonon behavior, such as the appearance of `activated'
modes. More significantly, however, the transition to the CO phase results in
the appearance of a quasielastic scattering response with the symmetry of the
spin chirality operator (); this scattering response is thus indicative
of magnetic or chiral spin fluctuations in the AFM charge-ordered phase.Comment: to be published in Phys. Rev. Lett. (Oct. 2000
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