31,685 research outputs found
Construction of nested space-filling designs
New types of designs called nested space-filling designs have been proposed
for conducting multiple computer experiments with different levels of accuracy.
In this article, we develop several approaches to constructing such designs.
The development of these methods also leads to the introduction of several new
discrete mathematics concepts, including nested orthogonal arrays and nested
difference matrices.Comment: Published in at http://dx.doi.org/10.1214/09-AOS690 the Annals of
Statistics (http://www.imstat.org/aos/) by the Institute of Mathematical
Statistics (http://www.imstat.org
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Polyisoprene Captured Sulfur Nanocomposite Materials for High-Areal-Capacity Lithium Sulfur Battery
A polyisoprene-sulfur (PIPS) copolymer and nano sulfur composite material (90 wt % sulfur) is synthesized through inverse vulcanization of PIP polymer with micrometer-sized sulfur particles for high-areal-capacity lithium sulfur batteries. The polycrystalline structure and nanodomain nature of the copolymer are revealed through high-resolution transmission electron microscopy (HRTEM). PIP polymer is also used as binders for the electrode to further capture the dissovlved polysulfides. A high areal capacity of ca. 7.0 mAh/cm2 and stable cycling are achieved based on the PIPS nanosulfur composite with a PIP binder, crucial to commercialization of lithium sulfur batteries. The chemical confinement both at material and electrode level alleviates the diffusion of polysulfides and the shuttle effect. The sulfur electrodes, both fresh and cycled, are analyzed through scanning electron microscopy (SEM). This approach enables scalable material production and high sulfur utilization at the cell level
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Experimental and Numerical Investigation on Progressive Collapse Resistance of Post-tensioned Precast Concrete Beam-Column Sub-assemblages
In this paper, four 1/2 scaled precast concrete (PC) beam-column sub-assemblages with high performance connection were tested under push-down loading procedure to study the load resisting mechanism of PC frames subjected to different column removal scenarios. The parameters investigated include the location of column removal and effective prestress in tendons. The test results indicated that the failure modes of unbonded post-tensioned precast concrete (PTPC) frames were different from that of reinforced concrete (RC) frames: no cracks formed in the beams and wide opening formed near the beam to column interfaces. For specimens without overhanging beams, the failure of side column was eccentric compression failure. Moreover, the load resisting mechanisms in PC frames were significantly different from that of RC frames: the compressive arch action (CAA) developed in concrete during column removal was mainly due to actively applied pre-compressive stress in the concrete; CAA will not vanish when severe crush in concrete occurred. Thus, it may provide negative contribution for load resistance when the displacement exceeds one-beam depth; the tensile force developed in the tendons could provide catenary action from the beginning of the test. Moreover, to deeper understand the behavior of tested specimens, numerical analyses were carried out. The effects of concrete strength, axial compression ratio at side columns, and loading approaches on the behavior of the sub-assemblages were also investigated based on validated numerical analysis
Prompt Iron Enrichment, Two r-Process Components, and Abundances in Very Metal-Poor Stars
We present a model to explain the wide range of abundances for heavy
r-process elements (mass number A > 130) at low [Fe/H]. This model requires
rapid star formation and/or an initial population of supermassive stars in the
earliest condensed clots of matter to provide a prompt or initial Fe inventory.
Subsequent Fe and r-process enrichment was provided by two types of supernovae:
one producing heavy r-elements with no Fe on a rather short timescale and the
other producing light r-elements (A < or = 130) with Fe on a much longer
timescale.Comment: 5 pages, 2 postscript figures, to appear in ApJ
Achieving ground-state polar molecular condensates by chainwise atom-molecule adiabatic passage
We generalize the idea of chainwise stimulated Raman adiabatic passage
(STIRAP) [Kuznetsova \textit{et al.} Phys. Rev. A \textbf{78}, 021402(R)
(2008)] to a photoassociation-based chainwise atom-molecule system, with the
goal of directly converting two-species atomic Bose-Einstein condensates (BEC)
into a ground polar molecular BEC. We pay particular attention to the
intermediate Raman laser fields, a control knob inaccessible to the usual
three-level model. We find that an appropriate exploration of both the
intermediate laser fields and the stability property of the atom-molecule
STIRAP can greatly reduce the power demand on the photoassociation laser, a key
concern for STIRAPs starting from free atoms due to the small Franck-Condon
factor in the free-bound transition.Comment: 8 pages, 2 figures, to appear in Phy. Rev.
Relationship between Thermodynamic Driving Force and One-Way Fluxes in Reversible Chemical Reactions
Chemical reaction systems operating in nonequilibrium open-system states
arise in a great number of contexts, including the study of living organisms,
in which chemical reactions, in general, are far from equilibrium. Here we
introduce a theorem that relates forward and re-verse fluxes and free energy
for any chemical process operating in a steady state. This rela-tionship, which
is a generalization of equilibrium conditions to the case of a chemical process
occurring in a nonequilibrium steady state, provides a novel equivalent
definition for chemical reaction free energy. In addition, it is shown that
previously unrelated theories introduced by Ussing and Hodgkin and Huxley for
transport of ions across membranes, Hill for catalytic cycle fluxes, and Crooks
for entropy production in microscopically reversible systems, are united in a
common framework based on this relationship.Comment: 11 page
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