30 research outputs found
Weak ferromagnetism and field-induced spin reorientation in K2V3O8
Magnetization and neutron diffraction measurements indicate long-range
antiferromagnetic ordering below TN=4 K in the 2D, S=1/2 Heisenberg
antiferromagnet K2V3O8. The ordered state exhibits ``weak ferromagnetism'' and
novel, field-induced spin reorientations. These experimental observations are
well described by a classical, two-spin Heisenberg model incorporating
Dzyaloshinskii-Moriya interactions and an additional c-axis anisotropy. This
additional anisotropy can be accounted for by inclusion of the symmetric
anisotropy term recently described by Kaplan, Shekhtman, Entin-Wohlman, and
Aharony. This suggests that K2V3O8 may be a very unique system where the
qualitative behavior relies on the presence of this symmetric anisotropy.Comment: 5 pages, 4 ps figures, REVTEX, submitted to PR
Dynamical properties of the spin-Peierls compound \alpha'--NaV2O5
Dynamical properties of the novel inorganic spin-Peierls compound
\alpha'--NaV2O5 are investigated using a one-dimensional dimerized Heisenberg
model. By exact diagonalizations of chains with up to 28 sites, supplemented by
a finite-size scaling analysis, the dimerization parameter \delta is determined
by requiring that the model reproduces the experimentally observed spin gap
\Delta. The dynamical and static spin structure factors are calculated. As for
CuGeO3, the existence of a low energy magnon branch separated from the
continuum is predicted. The present calculations also suggest that a large
magnetic Raman scattering intensity should appear above an energy threshold of
1.9 \Delta. The predicted photoemission spectrum is qualitatively similar to
results for an undimerized chain due to the presence of sizable short-range
antiferromagnetic correlations.Comment: 4 pages, latex, minor misprints corrected and a few references adde
Interference of a first-order transition with the formation of a spin-Peierls state in alpha'-NaV2O5?
We present results of high-resolution thermal-expansion and specific-heat
measurements on single crystalline alpha'-NaV2O5. We find clear evidence for
two almost degenerate phase transitions associated with the formation of the
dimerized state around 33K: A sharp first-order transition at T1=(33+-0.1)K
slightly below the onset of a second-order transition at T2onset around
(34+-0.1)K. The latter is accompanied by pronounced spontaneous strains. Our
results are consistent with a structural transformation at T1 induced by the
incipient spin-Peierls (SP) order parameter above T2=TSP.Comment: 5 pages, 7 figure
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Priority research directions for in situ data management: Enabling scientific discovery from diverse data sources
In January 2019, the US Department of Energy, Office of Science program in Advanced Scientific Computing Research, convened a workshop to identify priority research directions (PRDs) for in situ data management (ISDM). A fundamental finding of this workshop is that the methodologies used to manage data among a variety of tasks in situ can be used to facilitate scientific discovery from many different data sourcesâsimulation, experiment, and sensors, for exampleâand that being able to do so at numerous computing scales will benefit real-time decision-making, design optimization, and data-driven scientific discovery. This article describes six PRDs identified by the workshop, which highlight the components and capabilities needed for ISDM to be successful for a wide variety of applicationsâmaking ISDM capabilities more pervasive, controllable, composable, and transparent, with a focus on greater coordination with the software stack and a diversity of fundamentally new data algorithms
Electrochemical oxidation and reduction of La4Ni3O10 in alkaline media
In this work we used electrochemical polarization for oxidizing and reducing, in a controlled way, the Ruddlesden-Popper phase La4Ni3O10. With a careful choice of electrochemical parameters, we were able to obtain samples of La4Ni3O10±delta never obtained before..
Real-space pairing through charge transfer excitons in High-Tc cuprates
While approaching a MottâHubbard transition by hole doping of the pristine La2CuO4 cuprate, excitons are created because of excitonâexciton and exciton-doping hole stabilizing interactions. Here, excitons are of charge-transfer Frenkel-type, with effective Cu+Oâ electrical dipoles that solvate the doping charges. Assuming a moderate screening by charge carriers, we show that mobile exciton-solvated doping holes should be associated in pairs either by a deep energy well or as thermodynamically stable pairs that can glide in the [100] or [010] direction after Bose condensation. Excitonâexciton dipolar interactions constitute thus the âpairing glueâ in this model, which is based on instantaneous interactions and intrinsically differs from the previous excitonic models, in which BCS virtual phonons were replaced by virtual excitons