25 research outputs found
Electrode Polarization Effects in Broadband Dielectric Spectroscopy
In the present work, we provide broadband dielectric spectra showing strong
electrode polarization effects for various materials, belonging to very
different material classes. This includes both ionic and electronic conductors
as, e.g., salt solutions, ionic liquids, human blood, and
colossal-dielectric-constant materials. These data are intended to provide a
broad data base enabling a critical test of the validity of phenomenological
and microscopic models for electrode polarization. In the present work, the
results are analyzed using a simple phenomenological equivalent-circuit
description, involving a distributed parallel RC circuit element for the
modeling of the weakly conducting regions close to the electrodes. Excellent
fits of the experimental data are achieved in this way, demonstrating the
universal applicability of this approach. In the investigated ionically
conducting materials, we find the universal appearance of a second dispersion
region due to electrode polarization, which is only revealed if measuring down
to sufficiently low frequencies. This indicates the presence of a second
charge-transport process in ionic conductors with blocking electrodes.Comment: 9 pages, 6 figures, experimental data are provided in electronic form
(see "Data Conservancy"
Factorization of integrals, defining the beta-function, into integrals of total derivatives in N=1 SQED, regularized by higher derivatives
Some calculations in supersymmetric theories, made with the higher derivative
regularization, show that the beta-function is given by integrals of total
derivatives. This is qualitatively explained for the N=1 supersymmetric
electrodynamics in all orders.Comment: 14 page
Colossal dielectric constants in transition-metal oxides
Many transition-metal oxides show very large ("colossal") magnitudes of the
dielectric constant and thus have immense potential for applications in modern
microelectronics and for the development of new capacitance-based
energy-storage devices. In the present work, we thoroughly discuss the
mechanisms that can lead to colossal values of the dielectric constant,
especially emphasising effects generated by external and internal interfaces,
including electronic phase separation. In addition, we provide a detailed
overview and discussion of the dielectric properties of CaCu3Ti4O12 and related
systems, which is today's most investigated material with colossal dielectric
constant. Also a variety of further transition-metal oxides with large
dielectric constants are treated in detail, among them the system La2-xSrxNiO4
where electronic phase separation may play a role in the generation of a
colossal dielectric constant.Comment: 31 pages, 18 figures, submitted to Eur. Phys. J. for publication in
the Special Topics volume "Cooperative Phenomena in Solids: Metal-Insulator
Transitions and Ordering of Microscopic Degrees of Freedom
The influence of underdense polymer target with/without high-Z nanoparticles on laser radiation absorption and energy transport
Fabrication methods for low-density fine-structure (cell
size 1 m) 3-D networks of cellulose triacetate (TAC) are developed.
Target densities ranged 4-20 mg/cc, similar polymer structures were produced
both with no load and with high-Z cluster dopant with concentration up to
30%. Foams of varying density down to 0.25 plasma critical density at the
third harmonic of iodine laser wavelength are supplied for laser shots.
Experiments with underdense foam targets with and without clusters
irradiated on the PALS laser facility are analyzed preliminary, showing
strong influence of target structure on process of laser light absorption.
Heat and radiation transport in such targets are considered