244 research outputs found
Spectral properties and infrared absorption in manganites
Within a recently proposed variational approach it has been shown that, in
perovskites with , near the metal-insulator
transition, the combined effect of the magnetic and electron-phonon
interactions pushes the system toward a regime of two coexisting phases: a low
electron density one made by itinerant large polarons forming ferromagnetic
domains and a high electron density one made by localized small polarons giving
rise to paramagnetic or antiferromagnetic domains depending on temperature.
Employing the above-mentioned variational scheme, in this paper spectral and
optical properties of manganites are derived for at different
temperatures. It is found that the phase separation regime induces a robust
pseudogap in the excitation spectrum of the system. Then the conductivity
spectra are characterized by a transfer of spectral weight from high to low
energies, as the temperature decreases. In the metallic ferromagnetic
phase, at low two types of infrared absorption come out: a Drude term and a
broad absorption band due respectively to the coherent and incoherent motion of
large polarons. The obtained results turn out in good agreement with
experiments.Comment: 9 figure
Ballistic transport in one-dimensional loops with Rashba and Dresselhaus spin-orbit coupling
We discuss the combined effect of Rashba and Dresselhaus spin-orbit
interactions in polygonal loops formed by quantum wires, when the electron are
injected in a node and collected at the opposite one. The conditions that allow
perfect localization are found. Furthermore, we investigate the suppression of
the Al'tshuler--Aronov--Spivak oscillations that appear, in presence of a
magnetic flux, when the electrons are injected and collected at the same node.
Finally, we point out that a recent realization of a ballistic spin
interferometer can be used to obtain a reliable estimate of the magnitude ratio
of the two spin-orbit interactions.\bigskipComment: 6 figure
Ground state features of the Frohlich model
Following the ideas behind the Feynman approach, a variational wave function
is proposed for the Fr\"ohlich model. It is shown that it provides, for any
value of the electron-phonon coupling constant, an estimate of the polaron
ground state energy better than the Feynman method based on path integrals. The
mean number of phonons, the average electronic kinetic and interaction
energies, the ground state spectral weight and the electron-lattice correlation
function are calculated and successfully compared with the best available
results.Comment: 6 figure
Interplay between electron-phonon couplings and disorder strength on the transport properties of organic semiconductors
The combined effect of bulk and interface electron-phonon couplings on the
transport properties is investigated in a model for organic semiconductors
gated with polarizable dielectrics. While the bulk electron-phonon interaction
affects the behavior of mobility in the coherent regime below room temperature,
the interface coupling is dominant for the activated high contribution of
localized polarons. In order to improve the description of the transport
properties, the presence of disorder is needed in addition to electron-phonon
couplings. The effects of a weak disorder largely enhance the activation
energies of mobility and induce the small polaron formation at lower values of
electron-phonon couplings in the experimentally relevant window . The results are discussed in connection with experimental data of rubrene
organic field-effect transistors.Comment: 4 pages, 3 figure
Effects of electron coupling to intra- and inter-molecular vibrational modes on the transport properties of single crystal organic semiconductors
Electron coupling to intra- and inter-molecular vibrational modes is
investigated in models appropriate to single crystal organic semiconductors,
such as oligoacenes. Focus is on spectral and transport properties of these
systems beyond perturbative approaches. The interplay between different
couplings strongly affects the temperature band renormalization that is the
result of a subtle equilibrium between opposite tendencies: band narrowing due
to interaction with local modes, band widening due to electron coupling to non
local modes. The model provides an accurate description of the mobility as
function of temperature: indeed, it has the correct order of magnitude, at low
temperatures, it scales as a power-law with the exponent
larger than unity, and, at high temperatures, shows an hopping behavior with a
small activation energy.Comment: 3 Figures, Submitte
Exact Diagonalization Dynamical Mean Field Theory for Multi-Band Materials: Effect of Coulomb correlations on the Fermi surface of Na_0.3CoO_2
Dynamical mean field theory combined with finite-temperature exact
diagonalization is shown to be a suitable method to study local Coulomb
correlations in realistic multi-band materials. By making use of the sparseness
of the impurity Hamiltonian, exact eigenstates can be evaluated for
significantly larger clusters than in schemes based on full diagonalization.
Since finite-size effects are greatly reduced this approach allows the study of
three-band systems down to very low temperatures, for strong local Coulomb
interactions and full Hund exchange. It is also shown that exact
diagonalization yields smooth subband quasi-particle spectra and self-energies
at real frequencies. As a first application the correlation induced charge
transfer between t2g bands in Na_0.3CoO_2 is investigated. For both Hund and
Ising exchange the small eg' Fermi surface hole pockets are found to be
slightly enlarged compared to the non-interacting limit, in agreement with
previous Quantum Monte Carlo dynamical mean field calculations for Ising
exchange, but in conflict with photoemission data.Comment: 9 pages, 7 figure
Electronic transport within a quasi two-dimensional model for rubrene single-crystal field effect transistors
Spectral and transport properties of the quasi two-dimensional adiabatic
Su-Schrieffer-Heeger model are studied adjusting the parameters in order to
model rubrene single-crystal field effect transistors with small but finite
density of injected charge carriers. We show that, with increasing temperature
, the chemical potential moves into the tail of the density of states
corresponding to localized states, but this is not enough to drive the system
into an insulating state. The mobility along different crystallographic
directions is calculated including vertex corrections which give rise to a
transport lifetime one order of magnitude smaller than spectral lifetime of the
states involved in the transport mechanism. With increasing temperature, the
transport properties reach the Ioffe-Regel limit which is ascribed to less and
less appreciable contribution of itinerant states to the conduction process.
The model provides features of the mobility in close agreement with
experiments: right order of magnitude, scaling as a power law ,
with close or larger than two, and correct anisotropy ratio between
different in-plane directions. Due to a realistic high dimensional model, the
results are not biased by uncontrolled approximations.Comment: 10 pages, 9 figures, Submitte
Spectral, optical and transport properties of the adiabatic anisotropic Holstein model: Application to slightly doped organic semiconductors
Spectral, optical and transport properties of an anisotropic
three-dimensional Holstein model are studied within the adiabatic
approximation. The parameter regime is appropriate for organic semiconductors
used in single crystal based field effect transistors. Different approaches
have been used to solve the model: self-consistent Born approximation valid for
weak electron-phonon coupling, coherent potential approximation exact for
infinite dimensions, and numerical diagonalization for finite lattices. With
increasing temperature, the width of the spectral functions gets larger and
larger making the approximation of quasi-particle less accurate. On the
contrary, their peak positions are never strongly renormalized in comparison
with the bare ones. As expected, the density of states is characterized by an
exponential tail corresponding to localized states at low temperature. For weak
electron-lattice coupling, the optical conductivity follows a Drude behavior,
while, for intermediate electron-lattice coupling, a temperature dependent peak
is present at low frequency. For high temperatures and low particle densities,
the mobility always exhibits a power-law behavior as function of temperature.
With decreasing the particle density, at low temperature, the mobility shows a
transition from metallic to insulating behavior. Results are discussed in
connection with available experimental data.Comment: 9 pages, 7 figures, submitted to Phys. Rev.
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