333 research outputs found
Magneto-transport characteristics of La1.4Ca1.6Mn2O7 thin film deposited by spray pyrolysis
Polycrystalline thin films of double layer manganite La_1.4Ca_1.6Mn_2O_7
(DLCMO) have been deposited by nebulized spray pyrolysis on single crystal
LaAlO_3 substrates. These single phase films having grain size in the range
70-100 nm exhibit ferromagnetic transition at T_C ~ 107K. The short range
ferromagnetic ordering due to in plane spin coherence is evidenced to occur at
a higher temperature around 225 K. Insulator/semiconductor to metal transition
occurs at a lower temperature T_P ~ 55K. The transport mechanism above T_C is
of Mott`s variable range hopping type. Below T_C the current-voltage
characteristics show non-linear behaviour that becomes stronger with decreasing
temperature. At low temperatures below T_CA ~ 30K a magnetically frustrated
spin canted state is observed. The DLCMO films exhibit resonable low field
magnetoresistance and at 77K the magnetoresistance ratio is ~ 5% at 0.6 kOe and
\~ 13% at 3 kOe.Comment: 14 pages, 7 figure
The Skyrme model predictions for the mass spectrum and the - mass splittings
The -plet mass spectrum and the - mass splittings are computed in the framework of the minimal SU(3)
extended Skyrme model. As functions of the Skyrme charge and the SU(3)
symmetry breaking parameters the predictions are presented in tabular form. The
predicted mass splitting - is the smallest among
all SU(3) baryonic multiplets.Comment: 4 pages, 2 tables, version to appear in Phys. Rev.
Relation between crystal and magnetic structures of the layered manganites La2-2xSr1+2xMn2O7 (0.30 =< x =< 0.50)
Comprehensive neutron-powder diffraction and Rietveld analyses were carried
out to clarify the relation between the crystal and magnetic structures of
La2-2xSr1+2xMn2O7 (0.30 =< x =< 0.50). The Jahn-Teller (JT) distortion of Mn-O6
octahedra, i.e., the ratio of the averaged apical Mn-O bond length to the
equatorial Mn-O bond length, is Delta_JT=1.042(5) at x=0.30, where the magnetic
easy-axis at low temperature is parallel to the c axis. As the JT distortion
becomes suppressed with increasing x, a planar ferromagnetic structure appears
at x =< 0.32, which is followed by a canted antiferromagnetic (AFM) structure
at x =< 0.39. The canting angle between neighboring planes continuously
increases from 0 deg (planar ferromagnet: 0.32 =< x < 0.39) to 180 deg (A-type
AFM: x=0.48 where Delta_JT=1.013(5)). Dominance of the A-type AF structure with
decrease of JT distortion can be ascribed to the change in the eg orbital state
from d3z^2-r^2 to dx^2-y^2
Optical Studies of a Layered Manganite La_{1.2}Sr_{1.8}Mn_2O_7 : Polaron Correlation Effect
Optical conductivity spectra of a cleaved ab-plane of a
La_{1.2}Sr_{1.8}Mn_2O_7 single crystal exhibit a small polaron absorption band
in the mid-infrared region at overall temperatures. With decreasing temperature
(T) to Curie temperature (T_C), the center frequency of the small polaron band
moves to a higher frequency, resulting in a gap-like feature, and that it
collapses to a lower frequency below T_C. Interestingly, with decreasing T, the
stretching phonon mode hardens above T_C and softens below T_C. These
concurring changes of lattice and electronic structure indicate that short
range polaron correlation exist above T_C but disappear with a magnetic
ordering.Comment: 4 pages including 5 figures. submitted to Phys. Rev.
On the interpretation of spin-polarized electron energy loss spectra
We study the origin of the structure in the spin-polarized electron energy
loss spectroscopy (SPEELS) spectra of ferromagnetic crystals. Our study is
based on a 3d tight-binding Fe model, with constant onsite Coulomb repulsion U
between electrons of opposite spin. We find it is not the total density of
Stoner states as a function of energy loss which determines the response of the
system in the Stoner region, as usually thought, but the densities of Stoner
states for only a few interband transitions. Which transitions are important
depends ultimately on how strongly umklapp processes couple the corresponding
bands. This allows us to show, in particular, that the Stoner peak in SPEELS
spectra does not necessarily indicate the value of the exchange splitting
energy. Thus, the common assumption that this peak allows us to estimate the
magnetic moment through its correlation with exchange splitting should be
reconsidered, both in bulk and surface studies. Furthermore, we are able to
show that the above mechanism is one of the main causes for the typical
broadness of experimental spectra. Finally, our model predicts that optical
spin waves should be excited in SPEELS experiments.Comment: 11 pages, 7 eps figures, REVTeX fil
Surface and lightning sources of nitrogen oxides over the United States: Magnitudes, chemical evolution, and outflow
We use observations from two aircraft during the ICARTT campaign over the eastern United States and North Atlantic during summer 2004, interpreted with a global 3-D model of tropospheric chemistry (GEOS-Chem) to test current understanding of regional sources, chemical evolution, and export of NOx. The boundary layer NOx data provide top-down verification of a 50% decrease in power plant and industry NOx emissions over the eastern United States between 1999 and 2004. Observed NOx concentrations at 8–12 km altitude were 0.55 ± 0.36 ppbv, much larger than in previous U.S. aircraft campaigns (ELCHEM, SUCCESS, SONEX) though consistent with data from the NOXAR program aboard commercial aircraft. We show that regional lightning is the dominant source of this upper tropospheric NOx and increases upper tropospheric ozone by 10 ppbv. Simulating ICARTT upper tropospheric NOx observations with GEOS-Chem requires a factor of 4 increase in modeled NOx yield per flash (to 500 mol/ flash). Observed OH concentrations were a factor of 2 lower than can be explained from current photochemical models, for reasons that are unclear. A NOy-CO correlation analysis of the fraction f of North American NOx emissions vented to the free troposphere as NOy (sum of NOx and its oxidation products) shows observed f = 16 ± 10% and modeled f = 14 ± 9%, consistent with previous studies. Export to the lower free troposphere is mostly HNO3 but at higher altitudes is mostly PAN. The model successfully simulates NOy export efficiency and speciation, supporting previous model estimates of a large U.S. anthropogenic contribution to global tropospheric ozone through PAN export
Theory of anomalous magnon softening in ferromagnetic manganites
In metallic manganites with low Curie temperatures, a peculiar softening of
the magnon spectrum close to the magnetic zone boundary has experimentally been
observed. Here we present a theory of the renormalization of the magnetic
excitation spectrum in colossal magnetoresistance compounds. The theory is
based on the modulation of magnetic exchange bonds by the orbital degree of
freedom of double-degenerate e_g electrons. The model considered is an
orbitally degenerate double-exchange system coupled to Jahn-Teller active
phonons which we treat in the limit of strong onsite repulsions. Charge and
coupled orbital-lattice fluctuations are identified as the main origin of the
unusual softening of the magnetic spectrum
Observation of two time scales in the ferromagnetic manganite La(1-x)Ca(x)MnO(3), x = 0.3
We report new zero-field muon spin relaxation and neutron spin echo
measurements in ferromagnetic (FM) (La,Ca)MnO3 which taken together suggest two
spatially separated regions in close proximity possessing very different Mn-ion
spin dynamics. One region corresponds to an extended cluster which displays
'critical slowing down' near Tc and an increasing volume fraction below Tc. The
second region possesses more slowly fluctuating spins and a decreasing volume
fraction below Tc. These data are discussed in terms of the growth of small
polarons into overlapping regions of correlated spins below Tc, resulting in a
microscopically inhomogeneous FM transition.Comment: 10 pages, 3 figure
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