158 research outputs found

    Metal-organic framework-derived Ni 2 P/nitrogen-doped carbon porous spheres for enhanced lithium storage

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    Transition metal phosphides (TMPs)/carbonaceous matrices have gradually attracted attention in the field of energy storage. In this study, we presented nickel phosphide (Ni2P) nanoparticles anchored to nitrogen-doped carbon porous spheres (Ni2P/NC) by using metal-organic framework-Ni as the template. The comprehensive encapsulation architecture provides closer contact among the Ni2P nanoparticles and greatly improves the structural integrity as well as the electronic conductivity, resulting in excellent lithium storage performance. The reversible specific capacity of 286.4 mA h g−1 has been obtained even at a high current density of 3.0 A g−1 and 450.4 mA h g−1 is obtained after 800 cycles at 0.5 A g−1. Furthermore, full batteries based on LiNi1/3Co1/3Mn1/3O2||Ni2P/NC exhibit both good rate capability and cycling life. This study provides a powerful and in-depth insight on new advanced electrodes in high-performance energy storage devices

    The impact of long-term care insurance in China on beneficiaries and caregivers: A systematic review

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    Background China’s long-term care insurance (LTCI) policy has been minimally evaluated. This systematic review aimed to assess the impact of China’s LTCI pilot on beneficiaries and their caregivers. Methods This review is based on a search of peer-reviewed studies in English (Embase, MEDLINE, Web of Science) and Chinese (China National Knowledge Infrastructure [CNKI], VIP, Wanfang) databases from January 2016 through July 2020, with all studies published in English or Chinese included. We included quantitative analyses of beneficiary-level data that assessed the impact of LTCI on beneficiaries and their caregivers, with no restriction placed on the outcomes studied. Results Nine studies met our inclusion criteria. One study was a randomised trial and two used quasi-experimental approaches. Four studies examined LTCI’s effect on beneficiaries’ quality of life, physical pain, and health service utilisation; one study reported the effect on beneficiaries’ healthcare expenditures; and one study evaluated the impact on caregivers’ care tasks. These studies generally found LTCI to be associated with an improvement in patients’ quality of life (including decreased physical pain), a reduction in the number of outpatient visits and hospitalisations, decreased patient-level health expenditures (e.g. one study reported a reduction in the length of stay, inpatient expenditures, and health insurance expenditures in tertiary hospitals by 41.0%, 17.7%, and 11.4%, respectively), and reduced informal care tasks for caregivers. In addition, four out of four studies that evaluated this outcome found that beneficiaries’ overall satisfaction with LTCI was high. Conclusion The current evidence base for the effects of LTCI in China on beneficiaries and their caregivers is sparse. Nonetheless, the existing studies suggest that LTCI has positive effects on beneficiaries and their caregivers. Further rigorous research on the impacts of LTCI in China is needed to inform the future expansion of the program

    Different wildfire types promoted two-step terrestrial plant community change across the Triassic-Jurassic transition

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    Frequent wildfires associated with emplacement of the Central Atlantic Magmatic Province (CAMP) are thought to have been important drivers of two significant changes in terrestrial plant communities and diversity during the Triassic-Jurassic Mass Extinction (TJME, ca. 201.51 Ma). ​However, it remains to be investigated whether these two changes are potentially related to different wildfire types. To better understand this relationship, we used a new method to reanalyze fossil pollen and spores across the Triassic-Jurassic transition in the Jiyuan Basin from the North China Plate. Results show that two peaks in wildfire frequency experienced different types of wildfires, with each linked to significant changes in plant communities and diversity losses. In the first wildfire peak, canopy fires dominated and are accompanied by significant losses of canopy forming plants, while in the second wildfire peak, ground cover fires dominated accompanied by significant losses of ground cover plants. ​Changes in atmospheric humidity conditions were an important control on the two different wildfire peaks. Relatively humid climatic conditions corresponded to the prevalence of canopy fires and hindered the spread and development of ground cover fires in wet surface conditions. Conversely, relatively arid climatic conditions corresponded with the prevalence of ground cover fires in dry surface environments. Our results provide a potential relationship between terrestrial plant communities and wildfire types, which is important to further understanding of terrestrial environmental and floral changes driven by Large Igneous Provinces

    Different wildfire types promoted two-step terrestrial plant community change across the Triassic-Jurassic transition

    Get PDF
    Frequent wildfires associated with emplacement of the Central Atlantic Magmatic Province (CAMP) are thought to have been important drivers of two significant changes in terrestrial plant communities and diversity during the Triassic-Jurassic Mass Extinction (TJME, ca. 201.51 Ma). ​However, it remains to be investigated whether these two changes are potentially related to different wildfire types. To better understand this relationship, we used a new method to reanalyze fossil pollen and spores across the Triassic-Jurassic transition in the Jiyuan Basin from the North China Plate. Results show that two peaks in wildfire frequency experienced different types of wildfires, with each linked to significant changes in plant communities and diversity losses. In the first wildfire peak, canopy fires dominated and are accompanied by significant losses of canopy forming plants, while in the second wildfire peak, ground cover fires dominated accompanied by significant losses of ground cover plants. ​Changes in atmospheric humidity conditions were an important control on the two different wildfire peaks. Relatively humid climatic conditions corresponded to the prevalence of canopy fires and hindered the spread and development of ground cover fires in wet surface conditions. Conversely, relatively arid climatic conditions corresponded with the prevalence of ground cover fires in dry surface environments. Our results provide a potential relationship between terrestrial plant communities and wildfire types, which is important to further understanding of terrestrial environmental and floral changes driven by Large Igneous Provinces

    Floral response to the Late Triassic Carnian Pluvial Episode

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    The Late Triassic Carnian Pluvial Episode (CPE; ca. 234–232 Ma) was characterized by dramatic global temperature and humidity increases, which in many terrestrial settings was accompanied by changes from arid to humid vegetation types. This study reviews current evidence of terrestrial floral composition and distribution during the CPE and analyzes spatial and temporal variation with relation to potential environmental driving mechanisms. Available evidence suggests the CPE was a globally significant event that triggered significant increases in the abundance of ferns and hygrophytes in terrestrial floras and freshwater algae in fluvial and lacustrine settings. These changes ended a long interval of relatively arid terrestrial climatic conditions since the early Triassic and are linked temporally with eruptions of the oceanic plateau Wrangellia Large Igneous Province (LIP). The massive release of greenhouse gasses including isotopically light CO2 during 3–4 distinct pulses of Wrangellia volcanism appears to have been the main driver of CPE climate change. Each pulse enhanced global atmospheric circulation and the hydrological cycle and resulted in changes from arid to humid conditions that affected floral abundance and composition. Higher terrestrial primary productivity in humid phases facilitated increased burial of terrestrial organic carbon and led to the recommencement of peat accumulation, ending the coal gap that had persisted since the earliest Triassic times. Enhanced movement of carbon from the atmosphere through the biosphere into the geosphere may have counteracted the warming effects of Wrangellia volcanic greenhouse gas emissions and ultimately led to the return of a steady climate state that terminated the warm and humid conditions of the CPE

    Observation of the Anomalous Hall Effect in a Collinear Antiferromagnet

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    Time-reversal symmetry breaking is the basic physics concept underpinning many magnetic topological phenomena such as the anomalous Hall effect (AHE) and its quantized variant. The AHE has been primarily accompanied by a ferromagnetic dipole moment, which hinders the topological quantum states and limits data density in memory devices, or by a delicate noncollinear magnetic order with strong spin decoherence, both limiting their applicability. A potential breakthrough is the recent theoretical prediction of the AHE arising from collinear antiferromagnetism in an anisotropic crystal environment. This new mechanism does not require magnetic dipolar or noncollinear fields. However, it has not been experimentally observed to date. Here we demonstrate this unconventional mechanism by measuring the AHE in an epilayer of a rutile collinear antiferromagnet RuO2_2. The observed anomalous Hall conductivity is large, exceeding 300 S/cm, and is in agreement with the Berry phase topological transport contribution. Our results open a new unexplored chapter of time-reversal symmetry breaking phenomena in the abundant class of collinear antiferromagnetic materials.Comment: 33 pages, 14 figures, 2 table

    Nanopore-Based Direct RNA-Sequencing Reveals a High-Resolution Transcriptional Landscape of Porcine Reproductive and Respiratory Syndrome Virus

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    The TRS-mediated discontinuous transcription process is a hallmark of Arteriviruses. Precise assessment of the intricate sub genomic RNA (sg mRNA) populations is required to understand the kinetics of viral transcription. It is difficult to reconstruct and comprehensively quantify splicing events using short-read sequencing, making the identification of transcription-regulatory sequences (TRS) particularly problematic. Here, we applied long-read direct RNA sequencing to characterize the recombined RNA molecules produced in porcine alveolar macrophages during early passage infection of porcine reproductive and respiratory syndrome virus (PRRSV). Based on sequencing two PRRSV isolates, namely XM-2020 and GD, we revealed a high-resolution and diverse transcriptional landscape in PRRSV. The data revealed intriguing differences in sub genomic recombination types between the two PRRSVs while also demonstrating TRS-independent heterogeneous subpopulation not previously observed in Arteriviruses. We find that TRS usage is a regulated process and share the common preferred TRS in both strains. This study also identified a substantial number of TRSmediated transcript variants, including alternative-sg mRNAs encoding the same annotated ORF, as well as putative sg mRNAs encoded nested internal ORFs, implying that the genetic information encoded in PRRSV may be more intensively expressed. Epigenetic modifications have emerged as an essential regulatory layer in gene expression. Here, we gained a deeper understanding of m5C modification in poly(A) RNA, elucidating a potential link between methylation and transcriptional regulation. Collectively, our findings provided meaningful insights for redefining the transcriptome complexity of PRRSV. This will assist in filling the research gaps and developing strategies for better control of the PRRS

    A NADC30-like PRRSV causes serious intestinal infections and tropism in piglets

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    Porcine reproductive and respiratory syndrome virus (PRRSV) causes huge economic loss to China's swine industry. Currently, a novel type 2 PRRSV, called the NADC30-like strain, is epidemic in numerous provinces of China. In this study, a NADC30-Like PRRSV strain was isolated in primary alveolar macrophage (PAM) cells from fecal samples collected from a local pig farm, which suffered severe diarrhea. A pathogenicity comparison study was conducted in 6–week‐old piglets by inoculating highly pathogenic HP-PRRSV and NADC30-Like PRRSV isolates. RT-qPCR revealed detection of NADC30-Like PRRSV but not the HP-PRRSV in the intestine. PRRSV infection-related lesions were observed in the intestine were further confirmed by histopathological and immunohistochemically examination (IHC). In addition, severe virus infections were also detected by RT-qPCR. Based on clinical observation and pathogenicity experiments, we confirmed that NADC30-Like PRRSV gained more tissue tropism, especially in the small intestine. This may be the one reason explaining why NADC-Like 30 PRRSV become a major epidemic strain in China since the first outbreak in 2013

    Publisher Correction: An anomalous Hall effect in altermagnetic ruthenium dioxide

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    In the version of this article initially published, square brackets and parentheses were incorrect in Fig. 1g and throughout Fig. 2 (excepting lower labels in Fig. 2d–f). Further, in the second paragraph of the “Consistency with theoretical prediction” subsection of the main article, in the text now reading “the reorientation-field scale, namely, HC = (H2 AE − H2 d) /Hd,” the term “H2 AE” wasn’t shown as squared. The changes have been made in the HTML and PDF versions of the article
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