853 research outputs found

    Short note on magnetic impurities in SmFeAsO1x_{1-x}Fx_x (x=0, 0.07) compounds revealed by zero-field 75^{75}As NMR

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    We have performed zero-field 75^{75}As nuclear magnetic resonance study of SmFeAsO1x_{1-x}Fx_x (x=0, 0.07) polycrystals in a wide frequency range at various temperatures. 75^{75}As resonance line was found at around 265 MHz revealing the formation of the intermetallic FeAs clusters in the new layered superconductors. We have also demonstrated that NMR is a sensitive tool for probing the quality of these materials.Comment: Revised authorshi

    Tetragonal to orthorhombic phase transition in SmFeAsO: a synchrotron powder diffraction investigation

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    The crystal structure of SmFeAsO has been investigated by means of Rietveld refinement of high resolution synchrotron powder diffraction data collected at 300 K and 100 K. The compound crystallizes in the tetragonal P4/nmm space group at 300 K and in the orthorhombic Cmma space group at 100 K; attempts to refine the low temperature data in the monoclinic P112/n space group diverged. On the basis of both resistive and magnetic analyses the tetragonal to orthorhombic phase transition can be located at T about 140 K.Comment: Submitted to: Superconductor Science and Technology PACS: 61.05.cp, 61.66.Fn, 74.10.+v, 74.62.Dh, 74.70.D

    Role of Dirac cones in magnetotransport properties of REFeAsO (RE=rare earth) oxypnictides

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    In this work we study the effect of the rare earth element in iron oxypnictides of composition REFeAsO (RE=rare earth). On one hand we carry out Density Functional Theory calculations of the band structure, which evidence the multiband character of these compounds and the presence of Dirac cones along the Y-{\Gamma} and Z-R directions of the reciprocal space. On the other hand, we explore transport behavior by means of resistivity, Hall resistance and magnetoresistance measurements, which confirm the dominant role of Dirac cones. By combining our theoretical and experimental approaches, we extract information on effective masses, scattering rates and Fermi velocities for different rare earth elements.Comment: 13 pages, 5 figures accepted for publication on European Journal of Physics

    Coupling between 4f and itinerant electrons in SmFeAsO1-xFx (0.15 < x < 0.2) superconductors: an NMR study

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    19^{19}F NMR measurements in SmFeAsO1x_{1-x}Fx_x, for 0.15x0.20.15\leq x\leq 0.2, are presented. The nuclear spin-lattice relaxation rate 1/T11/T_1 increases upon cooling with a trend analogous to the one already observed in CeCu5.2_{5.2}Au0.8_{0.8}, a quasi two-dimensional heavy-fermion intermetallic compound with an antiferromagnetic ground-state. In particular, the behaviour of the relaxation rate either in SmFeAsO1x_{1-x}Fx_x or in CeCu5.2_{5.2}Au0.8_{0.8} can be described in the framework of the self-consistent renormalization theory for weakly itinerant electron systems. Remarkably, no effect of the superconducting transition on 19^{19}F 1/T11/T_1 is detected, a phenomenon which can hardly be explained within a single band model.Comment: 4 figure

    Theoretical search for superconductivity in Sc3XB perovskites and weak ferromagnetism in Sc3X (X = Tl, In, Ga, Al)

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    A possibility for a new family of intermetallic perovskite superconductors Sc3XB, with X = Tl, In, Ga and Al, is presented as a result of KKR electronic structure and pseudopotential phonon calculations. The large values of computed McMillan--Hopfield parameters on scandium suggest appearance of superconductivity in Sc3XB compounds. On the other hand, the possibility of weak itinerant ferromagnetic behavior of Sc3X systems is indicated by the small magnetic moment on Sc atoms in two cases of X =~ l and In. Also the electronic structure and resulting superconducting parameters for more realistic case of boron--deficient systems Sc3XB_x are computed using KKR--CPA method, by replacing boron atom with a vacancy. The comparison of the calculated McMillan--Hopfield parameters of the Sc3XB series with corresponding values in MgCNi3 and YRh3B superconductors is given, finding the favorable trends for superconductivity.Comment: 13 pages, 13 figures. v3 - revise

    Angular dependence of magnetoresistivity in c-oriented MgB2 thin film

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    The anisotropy of MgB2 is still under debate: its value, strongly dependent on the sample and on the measuring method, ranges between 1.2 and 13. In this work we present our results on a MgB2 c-oriented superconducting thin film. To evaluate the anisotropy, we followed two different approaches. Firstly, magnetoresistivity was measured as a function of temperature at selected magnetic fields applied both parallel and perpendicular to the c-axis; secondly, we measured magnetoresistivity at selected temperatures and magnetic fields, varying the angle q between the magnetic field and the c-axis. The anisotropy estimated from the ratio between the upper critical fields parallel and perpendicular to the c-axis and the one obtained in the framework of the scaling approach within the anisotropic Ginzburg-Landau theory are different but show a similar trend in the temperature dependence. The obtained results are compared and discussed in the light of the two-band nature of MgB2. A comparison between critical fields in thin films and single crystal is also performed.Comment: 13 pages, 4 figures, European Physical Journal B in pres

    Experimental confirmation of the low B isotope coefficient in MgB2

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    Recent investigations have shown that the first proposed explanations of the disagreement between experimental and theoretical value of isotope coefficient in MgB2 need to be reconsidered. Considering that in samples with residual resistivity of few mu-Ohm cm critical temperature variations produced by disorder effects can be comparable with variations due to the isotopic effect, we adopt a procedure in evaluating the B isotope coefficient which take account of these effects, obtaining a value which is in agreement with previous results and then confirming that there is something still unclear in the physics of MgB2.Comment: 8 pages, 3 figures Title has been changed A statement has been added in page 7 of the pdf file "Finally we would..." Reference 21 has been added Figure 1 anf Figure 2 have been change

    Critical Field of MGB2 : Crossover from Clean to Dirty Regimes

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    We have studied the upper critical field, Bc2, in poly-crystalline MgB2 samples in which disorder was varied in a controlled way to carry selectively p and s bands from clean to dirty limit. We have found that the clean regime survives when p bands are dirty and s bands are midway between clean and dirty. In this framework we can explain the anomalous behaviour of Al doped samples, in which Bc2 decreases as doping increases.Comment: 11 pages, 2 figure
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