65 research outputs found
Detection of the Vortex Dynamic Regimes in MgB2 by Third Harmonic AC Susceptibility Measurements
In a type-II superconductor the generation of higher harmonics in the
magnetic response to an alternating magnetic field is a consequence of the
non-linearity in the I-V relationship. The shape of the current-voltage (I-V)
curve is determined by the current dependence of the thermal activation energy
U(J) and is thus related to the dynamical regimes governing the vortex motion.
In order to investigate the vortex dynamics in MgB2 bulk superconductors we
have studied the fundamental (chi1) and third (chi3) harmonics of the ac
magnetic susceptibility. Measurements have been performed as a function of the
temperature and the dc magnetic field, up to 9 T, for various frequencies and
amplitudes of the ac field. We show that the analysis of the behaviour in
frequency of chi3(T) and chi3(B) curves can provide clear information about the
non-linearity in different regions of the I-V characteristic. By comparing the
experimental curves with numerical simulations of the non-linear diffusion
equation for the magnetic field we are able to resolve the crossover between a
dissipative regime governed by flux creep and one dominated by flux flow
phenomena.Comment: to be published in "Horizons in Superconductivity Research" (Nova
Science Publishers, Inc., NY, 2003
Vortex pinning in Au-irradiated FeSe0.4Te0.6 crystals from the static limit to gigahertz frequencies
Fe(Se,Te) is one of the simplest compounds of iron-based superconductors, but it shows a variety of vortex pinning phenomena both in thin-film and single-crystal forms. These properties are particularly important in light of its potential for applications ranging from the development of coated conductors for high-field magnets to topological quantum computation exploiting the Majorana particles found in the superconducting vortex cores. In this paper, we characterize the pinning properties of
FeSe
0.4
Te
0.6
single crystals, both pristine and Au-irradiated, with a set of characterization techniques ranging from the static limit to the GHz frequency range by using dc magnetometry, ac susceptibility measurements of both the fundamental and the third harmonic signals, and by microwave coplanar waveguide resonator measurements of London and Campbell penetration depths. We observed signatures of single vortex pinning that can be modeled by a parabolic pinning potential, dissipation caused by flux creep, and a general enhancement of the critical current density after 320 MeV Au ion irradiation
Chemically exfoliated graphene detects NO2 at the ppb level
Abstract The high sensitivity of graphene to the adsorption/desorption of gas molecule, is at the very beginning of its exploitation. This sensitivity relies on the two-dimensional nature of graphene allowing a total exposure of all its atoms to the adsorbing gas molecules, thus providing the greatest sensor area per unit volume. Indeed several technological limits weigh on the synthesis and manipulation of the material for the device fabrication. Herein a simple approach to fabricate conductometric sensors based on chemically exfoliated natural graphite is presented. The devices were tested upon sub-ppm concentrations of NO 2 in environmental conditions and show the ability to detect this toxic gas down to few ppb at room temperature
Study of coupling loss on bi-columnar BSCCO/Ag tapes by a.c. susceptibility measurements
Coupling losses were studied in composite tapes containing superconducting
material in the form of two separate stacks of densely packed filaments
embedded in a metallic matrix of Ag or Ag alloy. This kind of sample geometry
is quite favorable for studying the coupling currents and in particular the
role of superconducting bridges between filaments. By using a.c. susceptibility
technique, the electromagnetic losses as function of a.c. magnetic field
amplitude and frequency were measured at the temperature T = 77 K for two tapes
with different matrix composition. The length of samples was varied by
subsequent cutting in order to investigate its influence on the dynamics of
magnetic flux penetration. The geometrical factor which takes into
account the demagnetizing effects was established from a.c. susceptibility data
at low amplitudes. Losses vs frequency dependencies have been found to agree
nicely with the theoretical model developed for round multifilamentary wires.
Applying this model, the effective resistivity of the matrix was determined for
each tape, by using only measured quantities. For the tape with pure silver
matrix its value was found to be larger than what predicted by the theory for
given metal resistivity and filamentary architecture. On the contrary, in the
sample with a Ag/Mg alloy matrix, an effective resistivity much lower than
expected was determined. We explain these discrepancies by taking into account
the properties of the electrical contact of the interface between the
superconducting filaments and the normal matrix. In the case of soft matrix of
pure Ag, this is of poor quality, while the properties of alloy matrix seem to
provoke an extensive creation of intergrowths which can be actually observed in
this kind of samples.Comment: 20 pages 11 figure, submitted to Superconductor Science and
Technolog
Magneto-Optical and Multiferroic Properties of Transition-Metal (Fe, Co, or Ni)-Doped ZnO Layers Deposited by ALD
ZnO doped with transition metals (Co, Fe, or Ni) that have non-compensated electron spins attracts particular interest as it can induce various magnetic phenomena and behaviors. The advanced atomic layer deposition (ALD) technique makes it possible to obtain very thin layers of doped ZnO with controllable thicknesses and compositions that are compatible with the main microelectronic technologies, which further boosts the interest. The present study provides an extended analysis of the magneto optical MO Kerr effect and the dielectric properties of (Co, Fe, or Ni)-doped ZnO films prepared by ALD. The structural, magneto optical, and dielectric properties were considered in relation to the technological details of the ALD process and the corresponding dopant effects. All doped samples show a strong MO Kerr behavior with a substantial magnetization response and very high values of the Kerr polarization angle, especially in the case of ZnO/Fe. In addition, the results give evidence that Fe-doped ZnO also demonstrates a ferroelectric behavior. In this context, the observed rich and versatile physical nature and functionality open up new prospects for the application of these nanostructured materials in advanced electronic, spintronic, and optical devices
Vortex dynamics and pinning properties analysis of MgB2 bulk samples by ac susceptibility measurements
The flux lines dynamics have been investigated on MgB2 bulk superconductors
obtained by reactive liquid infiltration by measuring the ac magnetic
susceptibility. The fundamental and third harmonics have been studied as a
function of temperature, dc magnetic field, ac field amplitude and frequency.
In order to determine the dynamical regimes governing the vortex motion, the
experimental results have been compared with susceptibility curves obtained by
numerical calculations of the non-linear diffusion equation for the magnetic
field. The frequency behaviour of the third harmonic response, that cannot be
explained by frequency dependent critical state models, has been related to the
current dependence of the flux creep activation energy U(J) in the diffusion
coefficient. In this way we have shown that the measured curves are correctly
interpreted within the framework of a vortex glass description.Comment: 12 pages, 4 figures, Proceedings of Boromag worksho
Enhancement of the high-field critical current density of superconducting MgB2 by proton irradiation
A relatively high critical temperature, Tc, approaching 40 K, places the
recently-discovered superconductor magnesium diboride (MgB2) intermediate
between the families of low- and copper-oxide-based high-temperature
superconductors (HTS). Supercurrent flow in MgB2 is unhindered by grain
boundaries, unlike the HTS materials. Thus, long polycrystalline MgB2
conductors may be easier to fabricate, and so could fill a potentially
important niche of applications in the 20 to 30 K temperature range. However,
one disadvantage of MgB2 is that in bulk material the critical current density,
Jc, appears to drop more rapidly with increasing magnetic field than it does in
the HTS phases. The magnitude and field dependence of Jc are related to the
presence of structural defects that can "pin" the quantised magnetic vortices
that permeate the material, and prevent them from moving under the action of
the Lorentz force. Vortex studies suggest that it is the paucity of suitable
defects in MgB2 that causes the rapid decay of Jc with field. Here we show that
modest levels of atomic disorder, induced by proton irradiation, enhance the
pinning, and so increase Jc significantly at high fields. We anticipate that
chemical doping or mechanical processing should be capable of generating
similar levels of disorder, and so achieve technologically-attractive
performance in MgB2 by economically-viable routes.Comment: 5 pages, 4 figures, to be published in Nature (in press
A modified flux-creep picture
We study the creep problem in type-II superconducting materials for which the characteristic pinning center dimension I is larger than the coherence length xi. The average value of the escape time of flux quanta from these pinning centers is calculated by adopting an appropriate expression for the pinning potential U. The attempt frequency v in the Arrhenius formula is seen to depend explicitly on the current density J and the electric field E-creep due to flux-creep, calculated by this approach, qualitatively agrees with the experimental E - J curves
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