11 research outputs found

    Calculating the O3 Instantaneous Longwave Radiative Impact from Satellite Observations

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    Ozone is a key atmospheric substance for both chemistry and climate. Being a secondary species, its concentration is controlled by a number of different factors, such as precursors’ emission, sunlight and oxidizing agents. Its impact on atmospheric chemistry and radiative balance differs with altitude: in the lower troposphere ozone acts as a toxic pollutant, in the upper troposphere as a greenhouse gas (GHG) and finally in the stratosphere as a protection against harmful ultraviolet (UV) radiation. Ozone is in general a radiatively active gas for both solar (shortwave, SW) and terrestrial (longwave, LW) radiation [14], therefore it’s very important to acquire and understand its radiative impact for climate related studies.info:eu-repo/semantics/publishe

    Is there a stratospheric radiative feedback in global warming simulations?

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    The radiative impacts of the stratosphere in global warming simulations are investigated using abrupt CO2 quadrupling experiments of the Coupled Model Inter-comparison Project phase 5 (CMIP5), with a focus on stratospheric temperature and water vapor. It is found that the stratospheric temperature change has a robust bullhorn-like zonal-mean pattern due to a strengthening of the stratospheric overturning circulation. This temperature change modifies the zonal mean top-of-the-atmosphere energy balance, but the compensation of the regional effects leads to an insignificant global-mean radiative feedback (-0.02 +/- 0.04 W m(-2) K-1). The stratospheric water vapor concentration generally increases, which leads to a weak positive global-mean radiative feedback (0.02 +/- 0.01 W m(-2) K-1). The stratospheric moistening is related to mixing of elevated upper-tropospheric humidity, and, to a lesser extent, to change in tropical tropopause temperature. Our results indicate that the strength of the stratospheric water vapor feedback is noticeably larger in high-top models than in low-top ones. The results here indicate that although its radiative impact as a forcing adjustment is significant, the stratosphere makes a minor contribution to the overall climate feedback in CMIP5 models.National Science and Engineering Research Council of Canada [RGPIN418305-13]; Fonds de recherche du Quebec-Nature et technologies; National Natural Science Foundation of China [41025018]; National Basic Research Program of China (973 Program) [2010CB428606]; Korea Ministry of EnvironmentSCI(E)[email protected]
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