1,420 research outputs found
-Electron Ferromagnetism in Metal Free Carbon Probed by Soft X-Ray Dichroism
Elemental carbon represents a fundamental building block of matter and the
possibility of ferromagnetic order in carbon attracted widespread attention.
However, the origin of magnetic order in such a light element is only poorly
understood and has puzzled researchers. We present a spectromicroscopy study at
room temperature of proton irradiated metal free carbon using the elemental and
chemical specificity of x-ray magnetic circular dichroism (XMCD). We
demonstrate that the magnetic order in the investigated system originates only
from the carbon -electron system.Comment: 10 pages 3 color figure
The role of hydrogen in room-temperature ferromagnetism at graphite surfaces
We present a x-ray dichroism study of graphite surfaces that addresses the
origin and magnitude of ferromagnetism in metal-free carbon. We find that, in
addition to carbon states, also hydrogen-mediated electronic states
exhibit a net spin polarization with significant magnetic remanence at room
temperature. The observed magnetism is restricted to the top 10 nm of
the irradiated sample where the actual magnetization reaches emu/g
at room temperature. We prove that the ferromagnetism found in metal-free
untreated graphite is intrinsic and has a similar origin as the one found in
proton bombarded graphite.Comment: 10 pages, 5 figures, 1 table, submitted to New Journal of Physic
Magnetic phase diagram of the Hubbard model with next-nearest-neighbour hopping
We calculate the magnetic phase diagram of the Hubbard model for a Bethe
lattice with nearest neighbour (NN) hopping and next nearest neighbour
(NNN) hopping in the limit of infinite coordination. We use the amplitude
of the NNN hopping to tune the density of states (DOS) of the
non-interacting system from a situation with particle-hole symmetry to an
asymmetric one with van-Hove singularities at the lower ()
respectively upper () band edge for large enough . For
this strongly asymmetric situation we find rather extended parameter regions
with ferromagnetic states and regions with antiferromagnetic states.Comment: 13 pages, 7 figure
Atomic and itinerant effects at the transition metal x-ray absorption K-pre-edge exemplified in the case of VO
X-ray absorption spectroscopy is a well established tool for obtaining
information about orbital and spin degrees of freedom in transition metal- and
rare earth-compounds. For this purpose usually the dipole transitions of the L-
(2p to 3d) and M- (3d to 4f) edges are employed, whereas higher order
transitions such as quadrupolar 1s to 3d in the K-edge are rarely studied in
that respect. This is due to the fact that usually such quadrupolar transitions
are overshadowed by dipole allowed 1s to 4p transitions and, hence, are visible
only as minor features in the pre-edge region. Nonetheless, these features
carry a lot of valuable information, similar to the dipole L-edge transition,
which is not accessible in experiments under pressure due to the absorption of
the diamond anvil pressurecell. We recently performed a theoretical and
experimental analysis of such a situation for the metal insulator transition of
(V(1-x)Crx)2O3. Since the importance of the orbital degrees of freedom in this
transition is widely accepted, a thorough understanding of quadrupole
transitions of the vanadium K-pre-edge provides crucial information about the
underlying physics. Moreover, the lack of inversion symetry at the vanadium
site leads to onsite mixing of vanadium 3d- and 4p- states and related quantum
mechanical interferences between dipole and quadrupole transitions. Here we
present a theoretical analysis of experimental high resolution x-ray absorption
spectroscopy at the V pre-K edge measured in partial fluorescence yield mode
for single crystals. We carried out density functional as well as configuration
interaction calculations in order to capture effects coming from both,
itinerant and atomic limits
On rationality of the intersection points of a line with a plane quartic
We study the rationality of the intersection points of certain lines and
smooth plane quartics C defined over F_q. For q \geq 127, we prove the
existence of a line such that the intersection points with C are all rational.
Using another approach, we further prove the existence of a tangent line with
the same property as soon as the characteristic of F_q is different from 2 and
q \geq 66^2+1. Finally, we study the probability of the existence of a rational
flex on C and exhibit a curious behavior when the characteristic of F_q is
equal to 3.Comment: 17 pages. Theorem 2 now includes the characteristic 2 case;
Conjecture 1 from the previous version is proved wron
Are the renormalized band widths in TTF-TCNQ of structural or electronic origin? - An angular dependent NEXAFS study
We have performed angle-dependent near-edge x-ray absorption fine structure
measurements in the Auger electron yield mode on the correlated
quasi-one-dimensional organic conductor TTF-TCNQ in order to determine the
orientation of the molecules in the topmost surface layer. We find that the
tilt angles of the molecules with respect to the one-dimensional axis are
essentially the same as in the bulk. Thus we can rule out surface relaxation as
the origin of the renormalized band widths which were inferred from the
analysis of photoemission data within the one-dimensional Hubbard model.
Thereby recent theoretical results are corroborated which invoke long-range
Coulomb repulsion as alternative explanation to understand the spectral
dispersions of TTF-TCNQ quantitatively within an extended Hubbard model.Comment: 6 pages, 5 figure
Trichostatin A-induced histone acetylation causes decondensation of interphase chromatin
The effect of trichostatin A (TSA)-induced histone acetylation on the interphase chromatin structure was visualized in vivo with a HeLa cell line stably expressing histone H2A, which was fused to enhanced yellow fluorescent protein. The globally increased histone acetylation caused a reversible decondensation of dense chromatin regions and led to a more homogeneous distribution. These structural changes were quantified by image correlation spectroscopy and by spatially resolved scaling analysis. The image analysis revealed that a chromatin reorganization on a length scale from 200 nm to >1 μm was induced consistent with the opening of condensed chromatin domains containing several Mb of DNA. The observed conformation changes could be assigned to the folding of chromatin during G1 phase by characterizing the effect of TSA on cell cycle progression and developing a protocol that allowed the identification of G1 phase cells on microscope coverslips. An analysis by flow cytometry showed that the addition of TSA led to a significant arrest of cells in S phase and induced apoptosis. The concentration dependence of both processes was studied
Via-Less Microstrip to Rectangular Waveguide Transition on InP
Indium-Phosphide (InP) is one of the most common materials used for realizing active devices working in the millimeter frequency range. The isotropic etching profile of InP substrates limits the realization of passive devices, thus requiring an expensive and lossy hybrid platform. This paper presents a via-less, cost-effective and efficient solution for InP substrate. By using the proposed planar solution, it is demonstrated that rectangular waveguides can be realized on InP by fabricating a bed of nails structure which acts as a reflecting boundary for an impinging millimeter wave. As a proof of concept, a transition from microstrip to rectangular waveguide structure is realized within H-band (220-320 GHz) with a return loss of -18dB over a bandwidth of 30 GHz
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