2,804 research outputs found
Fine structure of the isoscalar giant quadrupole resonance in 40Ca due to Landau damping?
The fragmentation of the Isoscalar Giant Quadrupole Resonance (ISGQR) in 40Ca
has been investigated in high energy-resolution experiments using proton
inelastic scattering at E_p = 200 MeV. Fine structure is observed in the region
of the ISGQR and its characteristic energy scales are extracted from the
experimental data by means of a wavelet analysis. The experimental scales are
well described by Random Phase Approximation (RPA) and second-RPA calculations
with an effective interaction derived from a realistic nucleon-nucleon
interaction by the Unitary Correlation Operator Method (UCOM). In these results
characteristic scales are already present at the mean-field level pointing to
their origination in Landau damping, in contrast to the findings in heavier
nuclei and also to SRPA calculations for 40Ca based on phenomenological
effective interactions, where fine structure is explained by the coupling to
two-particle two-hole (2p-2h) states.Comment: Phys. Lett. B, in pres
Spin and orbital frustration in MnSc_2S_4 and FeSc_2S_4
Crystal structure, magnetic susceptibility, and specific heat were measured
in the normal cubic spinel compounds MnSc_2S_4 and FeSc_2S_4. Down to the
lowest temperatures, both compounds remain cubic and reveal strong magnetic
frustration. Specifically the Fe compound is characterized by a Curie-Weiss
temperature \Theta_{CW}= -45 K and does not show any indications of order down
to 50 mK. In addition, the Jahn-Teller ion Fe^{2+} is orbitally frustrated.
Hence, FeSc_2S_4 belongs to the rare class of spin-orbital liquids. MnSc_2S_4
is a spin liquid for temperatures T > T_N \approx 2 K.Comment: 4 pages, to be published in Physical Review Letter
Spin Frustration and Magnetic Exchange in Cobalt Aluminum Oxide Spinels
We report on x-ray diffraction, magnetic susceptibility, electron- spin
resonance and heat- capacity studies of Co[Al_1-xCo_x]_2O_4 for Co
concentrations 0<x<1. In this spinel system only the A-site Co^2+ cation is
magnetic, while the non-magnetic B-site Al^3+ is substituted by the low-spin
non-magnetic Co^3+, and it is possible to investigate the complete phase
diagram from Co^2+Al^3+_2O_4 to Co^2+Co^3+_2O_4. All samples reveal large
negative Curie-Weiss temperatures Theta_CW of the order of -110 K independent
of concentration, which is attributed to a high multiplicity of the
superexchange interactions between the A-site Co^2+ cations. A pure
antiferromagnetic state is found for x = 1.0 and 0.9 with Neel temperatures T_N
= 29.5 K and 21.2 K, respectively, as evidenced by lambda-like anomalies in the
specific heat. Compositions with 0.3<x<0.75 show smeared out strongly reduced
magnetic ordering temperatures. At low temperatures, a T^2.5 dependence of the
specific heat is indicative of a spin-liquid state. For x < 0.2 a T^2
dependence of the specific heat and a spin-glass like behavior of the
susceptibility below T_f = 4.7 K are observed. The high value of the
frustration parameter f = |Theta_CW|/T_f > 10 indicates the presence of strong
spin frustration at least for x < 0.6. The frustration mechanism is attributed
to competing nearest neighbor and next-nearest neighbor superexchange
interactions between the A-site Co^2+ ions.Comment: 19 pages, 9 figures, 46 reference
Spin Wave Instability of Itinerant Ferromagnet
We show variationally that instability of the ferromagnetic state in the
Hubbard model is largely controlled by softening of a long-wavelength spin-wave
excitation, except in the over-doped strong-coupling region where the
individual-particle excitation becomes unstable first. A similar conclusion is
drawn also for the double exchange ferromagnet. Generally the spin-wave
instability may be regarded as a precursor of the metal-insulator transition.Comment: 11 pages, 8 figure
Unification of dynamic density functional theory for colloidal fluids to include inertia and hydrodynamic interactions: derivation and numerical experiments.
Starting from the Kramers equation for the phase-space dynamics of the N-body probability distribution, we derive a dynamical density functional theory (DDFT) for colloidal fluids including the effects of inertia and hydrodynamic interactions (HI). We compare the resulting theory to extensive Langevin dynamics simulations for both hard rod systems and three-dimensional hard sphere systems with radially symmetric external potentials. As well as demonstrating the accuracy of the new DDFT, by comparing with previous DDFTs which neglect inertia, HI, or both, we also scrutinize the significance of including these effects. Close to local equilibrium we derive a continuum equation from the microscopic dynamics which is a generalized NavierâStokes-like equation with additional non-local terms governing the effects of HI. For the overdamped limit we recover analogues of existing configuration-space DDFTs but with a novel diffusion tensor
STITCH 3: zooming in on proteinâchemical interactions
To facilitate the study of interactions between proteins and chemicals, we have created STITCH, an aggregated database of interactions connecting over 300â000 chemicals and 2.6 million proteins from 1133 organisms. Compared to the previous version, the number of chemicals with interactions and the number of high-confidence interactions both increase 4-fold. The database can be accessed interactively through a web interface, displaying interactions in an integrated network view. It is also available for computational studies through downloadable files and an API. As an extension in the current version, we offer the option to switch between two levels of detail, namely whether stereoisomers of a given compound are shown as a merged entity or as separate entities. Separate display of stereoisomers is necessary, for example, for carbohydrates and chiral drugs. Combining the isomers increases the coverage, as interaction databases and publications found through text mining will often refer to compounds without specifying the stereoisomer. The database is accessible at http://stitch.embl.de/
Effective forces in colloidal mixtures: from depletion attraction to accumulation repulsion
Computer simulations and theory are used to systematically investigate how
the effective force between two big colloidal spheres in a sea of small spheres
depends on the basic (big-small and small-small) interactions. The latter are
modeled as hard-core pair potentials with a Yukawa tail which can be both
repulsive or attractive. For a repulsive small-small interaction, the effective
force follows the trends as predicted by a mapping onto an effective
non-additive hard-core mixture: both a depletion attraction and an accumulation
repulsion caused by small spheres adsorbing onto the big ones can be obtained
depending on the sign of the big-small interaction. For repulsive big-small
interactions, the effect of adding a small-small attraction also follows the
trends predicted by the mapping. But a more subtle ``repulsion through
attraction'' effect arises when both big-small and small-small attractions
occur: upon increasing the strength of the small-small interaction, the
effective potential becomes more repulsive. We have further tested several
theoretical methods against our computer simulations: The superposition
approximation works best for an added big-small repulsion, and breaks down for
a strong big-small attraction, while density functional theory is very accurate
for any big-small interaction when the small particles are pure hard-spheres.
The theoretical methods perform most poorly for small-small attractions.Comment: submitted to PRE; New version includes an important quantitative
correction to several of the simulations. The main conclusions remain
unchanged thoug
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