Nonlinear photoluminescence spectra from a quantum dot-cavity system: Direct evidence of pump-induced stimulated emission and anharmonic cavity-QED

We investigate the power-dependent photoluminescence spectra from a strongly coupled quantum dot-cavity system using a quantum master equation technique that accounts for incoherent pumping, pure dephasing, and fermion or boson statistics. Analytical spectra at the one-photon correlation level and the numerically exact multi-photon spectra for fermions are presented. We compare to recent experiments on a quantum dot-micropiller cavity system and show that an excellent fit to the data can be obtained by varying only the incoherent pump rates in direct correspondence with the experiments. Our theory and experiments together show a clear and systematic way of studying stimulated-emission induced broadening and anharmonic cavity-QED.Comment: We have reworked our previous arXiv paper and submitted this latest version for peer revie

A New Sampler for the Collection and Retrieval of Dry Dust Deposition

Atmospheric dust can influence biogeochemical cycles, accelerate snowmelt, and affect air, water quality, and human health. Yet, the bulk of atmospherically transported material remains poorly quantified in terms of total mass fluxes and composition. This lack of information stems in part from the challenges associated with measuring dust deposition. Here we report on the design and efficacy of a new dry deposition sampler (Dry Deposition Sampling Unit (DSU)) and method that quantifies the gravitational flux of dust particles. The sampler can be used alone or within existing networks such as those employed by the National Atmospheric Deposition Program (NADP). Because the samplers are deployed sterile and the use of water to remove trapped dust is not required, this method allows for the recovery of unaltered dry material suitable for subsequent chemical and microbiological analyses. The samplers were tested in the laboratory and at 15 field sites in the western United States. With respect to material retention, sampler performance far exceeded commonly used methods. Retrieval efficiency was \u3e97% in all trials and the sampler effectively preserved grain size distributions during wind exposure experiments. Field tests indicated favorable comparisons to dust-on-snow measurement across sites (r2 0.70, p \u3c 0.05) and within sites to co-located aerosol data (r2 0.57–0.99, p \u3c 0.05). The inclusion of dust deposition and composition monitoring into existing networks increases spatial and temporal understanding of the atmospheric transport on materials and substantively furthers knowledge of the effects of dust on terrestrial ecosystems and human exposure to dust and associated deleterious compounds

On-chip light detection using monolithically integrated quantum dot micropillars

This work was supported by the German Research Foundation (DFG) under Grants RE2974/9-1 and SCHN1376/1-1. The research leading to these results has received funding from the European Research Council under the European Union's Seventh Framework ERC Grant Agreement No. 615613.We demonstrate the on-chip detection of light using photosensitive detectors based on quantum dot (QD) micropillar cavities. These microscale detectors are applied exemplarily to probe the emission of a monolithically integrated, electrically pumped whispering gallery mode microlaser. Light is detected via the photocurrent induced in the electrically contacted micropillar detectors under reverse-bias. In order to demonstrate the high potential and applicability of the microdetector presented, we determine the threshold current of an integrated microlaser to be (54 ± 4) μA, in very good agreement with the value of (53 ± 4) μA inferred from optical data. Within this work we realize the monolithic integration of a laser and a detector in a single device operating in the regime of cavity-quantum electrodynamics. Our results thus advance the research on microscale sensor technology towards the few-photon quantum limit and pave the way for on-chip opto-electronic feedback experiments.PostprintPeer reviewe

An electrically driven cavity-enhanced source of indistinguishable photons with 61% overall efficiency

This work was financially supported by the German Research Foundation (DFG) under Grants RE2974/9-1 and SCHN1376/1-1 as well as the German Federal Ministry of Education and Research (BMBF) through the VIP-project “QSOURCE”.We report on an electrically driven efficient source of indistinguishable photons operated at pulse-repetition rates f up to 1.2 GHz. The quantum light source is based on a p-i-n-doped micropillar cavity with integrated self-organized quantum dots, which exploits cavity quantum electrodynamics effects in the weak coupling regime to enhance the emission of a single quantum emitter coupled to the cavity mode. We achieve an overall single-photon extraction efficiency of (61 ± 11) % for a device triggered electrically at f = 625 MHz. Analyzing the suppression of multi-photon emission events as a function of excitation repetition rate, we observe single-photon emission associated with g(2)HBT(0) values between 0.076 and 0.227 for f ranging from 373 MHz to 1.2 GHz. Hong-Ou-Mandel-type two-photon interference experiments under pulsed current injection at 487 MHz reveal a photon-indistinguishability of (41.1 ± 9.5) % at a single-photon emission rate of (92 ± 23) MHz.Publisher PDFPeer reviewe

Minimum Fluidization Velocity and Gas Holdup in Fluidized Beds with Side Port Air

ABSTRACT Fluidized beds can be used to gasify biomass in the production of producer gas, a flammable gas that can replace natural gas in process heating. Knowing how the fluidized bed hydrodynamics vary as reactor dimensions are scaled up is vital for improving reactor efficiency. This study utilizes 10.2 cm and 15.2 cm diameter fluidized beds with added side port air injection to investigate column diameter effects on fluidized bed hydrodynamics. Both inert (glass beads) and biomass (ground walnut shell and ground corncob) bed materials are used and the hydrodynamic differences with side port air injection are recorded. Minimum fluidization velocity is determined through pressure drop measurements. Timeaveraged local and global gas holdup are recorded using X-ray computed tomography imaging. Results show that by varying the side port air flow rate as a percentage of the minimum fluidization flow rate, partial and complete fluidization is observed in both fluidized beds. Local gas holdup trends are also similar in both fluidized beds. These results will be used in future studies to validate computational fluid dynamics models of fluidized beds

13th Meeting of the Scientific Group on Methodologies for the Safety Evaluation of Chemicals (SGOMSEC): alternative testing methodologies for organ toxicity.

In the past decade in vitro tests have been developed that represent a range of anatomic structure from perfused whole organs to subcellular fractions. To assess the use of in vitro tests for toxicity testing, we describe and evaluate the current status of organotypic cultures for the major target organs of toxic agents. This includes liver, kidney, neural tissue, the hematopoietic system, the immune system, reproductive organs, and the endocrine system. The second part of this report reviews the application of in vitro culture systems to organ specific toxicity and evaluates the application of these systems both in industry for safety assessment and in government for regulatory purposes. Members of the working group (WG) felt that access to high-quality human material is essential for better use of in vitro organ and tissue cultures in the risk assessment process. Therefore, research should focus on improving culture techniques that will allow better preservation of human material. The WG felt that it is also important to develop and make available relevant reference compounds for toxicity assessment in each organ system, to organize and make available via the Internet complete in vivo toxicity data, including human data, containing dose, end points, and toxicokinetics. The WG also recommended that research should be supported to identify and to validate biological end points for target organ toxicity to be used in alternative toxicity testing strategies