1,690 research outputs found
Frank's constant in the hexatic phase
Using video-microscopy data of a two-dimensional colloidal system the
bond-order correlation function G6 is calculated and used to determine the
temperature-dependence of both the orientational correlation length xi6 in the
isotropic liquid phase and the Frank constant F_A in the hexatic phase. F_A
takes the value 72/pi at the hexatic to isotropic liquid phase transition and
diverges at the hexatic to crystal transition as predicted by the KTHNY-theory.
This is a quantitative test of the mechanism of breaking the orientational
symmetry by disclination unbinding
Elastic Behavior of a Two-dimensional Crystal near Melting
Using positional data from video-microscopy we determine the elastic moduli
of two-dimensional colloidal crystals as a function of temperature. The moduli
are extracted from the wave-vector-dependent normal mode spring constants in
the limit and are compared to the renormalized Young's modulus of the
KTHNY theory. An essential element of this theory is the universal prediction
that Young's modulus must approach at the melting temperature. This is
indeed observed in our experiment.Comment: 4 pages, 3 figure
The experimental realization of a two-dimensional colloidal model system
We present the technical details of an experimental method to realize a model
system for 2D phase transitions and the glass transition. The system consists
of several hundred thousand colloidal super-paramagnetic particles confined by
gravity at a flat water-air interface of a pending water droplet where they are
subjected to Brownian motion. The dipolar pair potential and therefore the
system temperature is not only known precisely but also directly and
instantaneously controllable via an external magnetic field B. In case of a one
component system of monodisperse particles the system can crystallize upon
application of B whereas in a two component system it undergoes a glass
transition. Up to 10000 particles are observed by video microscopy and image
processing provides their trajectories on all relative length and time scales.
The position of the interface is actively regulated thereby reducing surface
fluctuations to less than one micron and the setup inclination is controlled to
an accuracy of 1 microrad. The sample quality being necessary to enable the
experimental investigation of the 2D melting scenario, 2D crystallization, and
the 2D glass transition, is discussed.Comment: 13 pages, 11 figure
Magnetic properties of Quantum Corrals from first principles calculations
We present calculations for electronic and magnetic properties of surface
states confined by a circular quantum corral built of magnetic adatoms (Fe) on
a Cu(111) surface. We show the oscillations of charge and magnetization
densities within the corral and the possibility of the appearance of
spin--polarized states. In order to classify the peaks in the calculated
density of states with orbital quantum numbers we analyzed the problem in terms
of a simple quantum mechanical circular well model. This model is also used to
estimate the behaviour of the magnetization and energy with respect to the
radius of the circular corral. The calculations are performed fully
relativistically using the embedding technique within the
Korringa-Kohn-Rostoker method.Comment: 14 pages, 9 figures, submitted to J. Phys. Cond. Matt. special issue
on 'Theory and Simulation of Nanostructures
Harmonic lattice behavior of two-dimensional colloidal crystals
Using positional data from video-microscopy and applying the equipartition
theorem for harmonic Hamiltonians, we determine the wave-vector-dependent
normal mode spring constants of a two-dimensional colloidal model crystal and
compare the measured band-structure to predictions of the harmonic lattice
theory. We find good agreement for both the transversal and the longitudinal
mode. For , the measured spring constants are consistent with the
elastic moduli of the crystal.Comment: 4 pages, 3 figures, submitte
Spin-dependent electrical transport in ion-beam sputter deposited Fe-Cr multilayers
The temperature dependence of the electrical resistivity and
magnetoresistance of Xe-ion beam sputtered Fe-Cr multilayers has been
investigated. The electrical resistivity between 5 and 300 K in the fully
ferromagnetic state, obtained by applying a field beyond the saturation field
(H_sat) necessary for the antiferromagnetic(AF)-ferromagnetic(FM) field-induced
transition, shows evidence of spin-disorder resistivity as in crystalline Fe
and an s-d scattering contribution (as in 3d metals and alloys). The sublattice
magnetization m(T) in these multilayers has been calculated in terms of the
planar and interlayer exchange energies. The additional spin-dependent
scattering \Delta \rho (T) = \rho(T,H=0)_AF - \rho(T,H=H_sat)_FM in the AF
state over a wide range of temperature is found to be proportional to the
sublattice magnetization, both \Delta \rho(T) and m(T) reducing along with the
antiferromagnetic fraction. At intermediate fields, the spin-dependent part of
the electrical resistivity (\rho_s (T)) fits well to the power law \rho_s (T) =
b - cT^\alpha where c is a constant and b and \alpha are functions of H. At low
fields \alpha \approx 2 and the intercept b decreases with H much the same way
as the decrease of \Delta \rho (T) with T. A phase diagram (T vs. H_sat) is
obtained for the field- induced AF to FM transition. Comparisons are made
between the present investigation and similar studies using dc magnetron
sputtered and molecular beam epitaxy (MBE) grown Fe-Cr multilayers.Comment: 8 pages, 10 figures, to appear in Phys. Rev.
Injection of photoelectrons into dense argon gas
The injection of photoelectrons in a gaseous or liquid sample is a widespread
technique to produce a cold plasma in a weakly--ionized system in order to
study the transport properties of electrons in a dense gas or liquid. We report
here the experimental results of photoelectron injection into dense argon gas
at the temperatureT=142.6 K as a function of the externally applied electric
field and gas density. We show that the experimental data can be interpreted in
terms of the so called Young-Bradbury model only if multiple scattering effects
due to the dense environment are taken into account when computing the
scattering properties and the energetics of the electrons.Comment: 18 pages, 10 figures, figure nr. 10 has been redrawn, to be submitted
to Plasma Sources Science and Technolog
Interlayer Exchange Coupling Mediated by Valence Band Electrons
The interlayer exchange coupling mediated by valence band electrons in
all-semiconductor IV-VI magnetic/nonmagnetic superlattices is studied
theoretically. A 3D tight-binding model, accounting for the band and magnetic
structure of the constituent superlattice components is used to calculate the
spin-dependent part of the total electronic energy. The antiferromagnetic
coupling between ferromagnetic layers in EuS/PbS superlattices is obtained, in
agreement with the experimental evidences. The results obtained for the
coupling between antiferromagnetic layers in EuTe/PbTe superlattices are also
presented.Comment: 8 pages, 6 figures, to be submitted to Phys.Rev.
Testing the relevance of effective interaction potentials between highly charged colloids in suspension
Combining cell and Jellium model mean-field approaches, Monte Carlo together
with integral equation techniques, and finally more demanding many-colloid
mean-field computations, we investigate the thermodynamic behavior, pressure
and compressibility of highly charged colloidal dispersions, and at a more
microscopic level, the force distribution acting on the colloids. The
Kirkwood-Buff identity provides a useful probe to challenge the
self-consistency of an approximate effective screened Coulomb (Yukawa)
potential between colloids. Two effective parameter models are put to the test:
cell against renormalized Jellium models
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