1,091 research outputs found

    Exotics Searches at ATLAS

    Full text link
    While the Standard Model of particle physics is a very successful theory and has been tested to hold with great precision in numerous experiments, it still leaves a number of open questions. Among those are the matter-antimatter asymmetry in the universe, the hierarchy problem and dark matter. Many models for new physics beyond the Standard Model provide solutions to one or several of these shortcomings of the Standard Model. In this article, a selected subset of recent ATLAS results from searches for such models is high-lighted, with a special focus on searches for Dark Matter.Comment: 13 pages, 12 figures, to appear in the proceedings of the Interplay between Particle and Astroparticle Physics workshop, 18 - 22 August, 2014, held at Queen Mary University of London, UK; added references, contents unchange

    Physical properties and lattice dynamics of bixbyite-type V2O3

    Get PDF
    Dieser Beitrag ist mit Zustimmung des Rechteinhabers aufgrund einer (DFG geförderten) Allianz- bzw. Nationallizenz frei zugĂ€nglich.This publication is with permission of the rights owner freely accessible due to an Alliance licence and a national licence (funded by the DFG, German Research Foundation) respectively.Some time ago, we reported the synthesis of bixbyite-type V2O3, a new metastable polymorph of vanadium sesquioxide. Since, a number of investigations followed, dealing with different aspects like electronic and magnetic properties of the material, the deviation from ideal stoichiometry or the preparation of nanocrystals as oxygen storage material. However, most of the physical properties were only evaluated on a theoretical basis. Here, we report the lattice dynamics and physical properties of bixbyite-type V2O3 bulk material, which we acquired from physical property measurements and neutron diffraction experiments over a wide temperature range. Besides attributing different possible orientations of the magnetic moments for V1 and V2 to the identified antiferromagnetic (AFM) ground state with a NĂ©el temperature of 38.1(5) K, we use a first order GrĂŒneisen approximation to determine lattice-dependent parameters for the relatively stiff cubic lattice, and, amongst others identify the Debye temperature to be as low as 350 ± 65 K.DFG, 73789094, SPP 1415: Kristalline Nichtgleichgewichtsphasen - PrĂ€paration, Charakterisierung und in situ-Untersuchung der Bildungsmechanisme

    Mechanochemical Synthesis of Cu2MgSn3S8 and Ag2MgSn3S8

    Get PDF
    Two new thiospinels of the type AI2BIICIV3SVI8 were successfully synthesized via a mechanochemical route using binary sulfides and sulfur. Cu2MgSn3S8 and Ag2MgSn3S8 are the first AI2BIICIV3SVI8 compounds with magnesium as divalent cation. The crystal structures of Cu2MgSn3S8 and Ag2MgSn3S8 were refined in the cubic space group Fd3m using X‐ray powder diffraction. According to UV/Vis measurements, a direct optical bandgap of ca. 1.65 eV was determined for both Cu2MgSn3S8 and Ag2MgSn3S8. Temperature‐dependent magnetic susceptibility measurements of the Cu2MgSn3S8 sample indicate diamagnetism. A 119Sn Mössbauer spectrum confirms the tetravalent state of tin, underlining the electron‐precise description.TU Berlin, Open-Access-Mittel - 202

    Valence modulations in CeRuSn

    Get PDF
    CeRuSn exhibits an extraordinary room temperature structure at 300~K with coexistence of two types of Ce ions, namely trivalent Ce3+^{3+} and intermediate valent Ce(4−ή)+^{(4-\delta)+}, in a metallic environment. The ordered arrangement of these two Ce types on specific crystallographic sites results in a doubling of the unit cell along the cc-axis with respect to the basic monoclinic CeCoAl-type structure. Below room temperature, structural modulation transitions with very broad hysteresis have been reported from measurements of various bulk properties. X-ray diffraction revealed that at low temperatures the doubling of the CeCoAl type structure is replaced by a different modulated ground state, approximating a near tripling of the basic CeCoAl cell. The transition is accompanied by a significant contraction of the cc axis. We present new x-ray absorption near-edge spectroscopy data at the Ce L3_{3} absorption edge, measured on a freshly cleaved surface of a CeRuSn single crystal. In contrast to a previous report, the new data exhibit small but significant variations as function of temperature that are consistent with a transition of a fraction of Ce3+^{3+} ions to the intermediate valence state, analogous to the γ→α\gamma \rightarrow \alpha transition in elemental cerium, when cooling through the structural transitions of CeRuSn. Such results in a valence-modulated state

    Yb2_{2}Pt2_{2}Pb: Magnetic frustration in the Shastry-Sutherland lattice

    Full text link
    We have synthesized single crystals of Yb2_{2}Pt2_{2}Pb, which crystallize in the layered U2_{2}Pt2_{2}Sn-type structure, where planes of Yb ions lie on a triangular network. We report here the first results of magnetization, specific heat, and electrical resistivity experiments. The lattice constants and high temperature magnetic susceptibility indicate that the Yb ions are trivalent, while Schottky peaks in the specific heat show that the ground state is a well isolated doublet. Significant magnetic anisotropy is observed, with the ratio of susceptibilities perpendicular and parallel to the magnetic planes differing by as much as a factor of 30 at the lowest temperatures. Antiferromagnetic order occurs at a N\'eel temperature TNT_{\rm N}=2.07 K, a transition temperature which is more than an order of magnitude smaller than the mean field interactions reflected by the in-plane Weiss temperature. Further evidence for short ranged magnetic fluctuations is found in the magnetic susceptibility and electrical resistivity, which have broad peaks above TNT_{\rm N}, and in the slow development of the magnetic entropy at TNT_{\rm N}. Our experiments indicate that Yb2_{2}Pt2_{2}Pb is a quasi-two dimensional and localized moment system, where strong magnetic frustration may arise from the geometry of the underlying Shastry-Sutherland lattice.Comment: 8 pages, 8 figure

    Mixed Valence Europium Nitridosilicate Eu2SiN3

    Get PDF
    The mixed valence europium nitridosilicate Eu2SiN3 has been synthesized at 900°C in welded tantalum ampules starting from europium and silicon diimide Si(NH)2 in a lithium flux. The structure of the black material has been determined by single-crystal X-ray diffraction analysis (Cmca (no. 64), a=542.3(11) pm, b=1061.0(2) pm, c=1162.9(2) pm, Z=8, 767 independent reflections, 37 parameters, R1=0.017, wR2=0.032). Eu2SiN3 is a chain-type silicate comprising one-dimensional infinite nonbranched zweier chains of corner-sharing SiN4 tetrahedra running parallel [100] with a maximum stretching factor fs=1.0. The compound is isostructural with Ca2PN3 and Rb2TiO3, and it represents the first example of a nonbranched chain silicate in the class of nitridosilicates. There are two crystallographically distinct europium sites (at two different Wyckoff positions 8f) being occupied with Eu2+ and Eu3+, respectively. 151Eu Mössbauer spectroscopy of Eu2SiN3 differentiates unequivocally these two europium atoms and confirms their equiatomic multiplicity, showing static mixed valence with a constant ratio of the Eu2+ and Eu3+ signals over the whole temperature range. The Eu2+ site shows magnetic hyperfine field splitting at 4.2 K. Magnetic susceptibility measurements exhibit Curie-Weiss behavior above 24 K with an effective magnetic moment of 7.5 ÎŒB/f.u. and a small contribution of Eu3+, in accordance with Eu2+ and Eu3+ in equiatomic ratio. Ferromagnetic ordering at unusually high temperature is detected at TC=24 K. DFT calculations of Eu2SiN3 reveal a band gap of ∌0.2 eV, which is in agreement with the black color of the compound. Both DFT calculations and lattice energetic calculations (MAPLE) corroborate the assignment of two crystallographically independent Eu sites to Eu2+ and Eu3+

    Magnetoresistance, specific heat and magnetocaloric effect of equiatomic rare-earth transition-metal magnesium compounds

    Full text link
    We present a study of the magnetoresistance, the specific heat and the magnetocaloric effect of equiatomic RETRETMg intermetallics with RE=LaRE = {\rm La}, Eu, Gd, Yb and T=AgT = {\rm Ag}, Au and of GdAuIn. Depending on the composition these compounds are paramagnetic (RE=LaRE = {\rm La}, Yb) or they order either ferro- or antiferromagnetically with transition temperatures ranging from about 13 to 81 K. All of them are metallic, but the resistivity varies over 3 orders of magnitude. The magnetic order causes a strong decrease of the resistivity and around the ordering temperature we find pronounced magnetoresistance effects. The magnetic ordering also leads to well-defined anomalies in the specific heat. An analysis of the entropy change leads to the conclusions that generally the magnetic transition can be described by an ordering of localized S=7/2S=7/2 moments arising from the half-filled 4f74f^7 shells of Eu2+^{2+} or Gd3+^{3+}. However, for GdAgMg we find clear evidence for two phase transitions indicating that the magnetic ordering sets in partially below about 125 K and is completed via an almost first-order transition at 39 K. The magnetocaloric effect is weak for the antiferromagnets and rather pronounced for the ferromagnets for low magnetic fields around the zero-field Curie temperature.Comment: 12 pages, 7 figures include

    Searching for hexagonal analogues of the half-metallic half-Heusler XYZ compounds

    Full text link
    The XYZ half-Heusler crystal structure can conveniently be described as a tetrahedral zinc blende YZ structure which is stuffed by a slightly ionic X species. This description is well suited to understand the electronic structure of semiconducting 8-electron compounds such as LiAlSi (formulated Li+^+[AlSi]−^-) or semiconducting 18-electron compounds such as TiCoSb (formulated Ti4+^{4+}[CoSb]4−^{4-}). The basis for this is that [AlSi]−^- (with the same electron count as Si2_2) and [CoSb]4−^{4-} (the same electron count as GaSb), are both structurally and electronically, zinc-blende semiconductors. The electronic structure of half-metallic ferromagnets in this structure type can then be described as semiconductors with stuffing magnetic ions which have a local moment: For example, 22 electron MnNiSb can be written Mn3+^{3+}[NiSb]3−^{3-}. The tendency in the 18 electron compound for a semiconducting gap -- believed to arise from strong covalency -- is carried over in MnNiSb to a tendency for a gap in one spin direction. Here we similarly propose the systematic examination of 18-electron hexagonal compounds for semiconducting gaps; these would be the "stuffed wurtzite" analogues of the "stuffed zinc blende" half-Heusler compounds. These semiconductors could then serve as the basis for possibly new families of half-metallic compounds, attained through appropriate replacement of non-magnetic ions by magnetic ones. These semiconductors and semimetals with tunable charge carrier concentrations could also be interesting in the context of magnetoresistive and thermoelectric materials.Comment: 11 pages, 6 figures, of which 4 are colou
    • 

    corecore