217 research outputs found

    Raman scattering studies of spin, charge, and lattice dynamics in Ca_{2-x}Sr_{x}RuO_{4} (0 =< x < 0.2)

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    We use Raman scattering to study spin, charge, and lattice dynamics in various phases of Ca_{2-x}Sr_{x}RuO_{4}. With increasing substitution of Ca by Sr in the range 0 =< x < 0.2, we observe (1) evidence for an increase of the electron-phonon interaction strength, (2) an increased temperature-dependence of the two-magnon energy and linewidth in the antiferromagnetic insulating phase, and (3) evidence for charge gap development, and hysteresis associated with the structural phase change, both of which are indicative of a first-order metal-insulator transition (T_{MI}) and a coexistence of metallic and insulating components for T < T_{MI}

    Lattice dynamics and the electron-phonon interaction in Ca2_2RuO4_4

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    We present a Raman scattering study of Ca2_2RuO4_4, in which we investigate the temperature-dependence of the lattice dynamics and the electron-phonon interaction below the metal-insulator transition temperature ({\it T}MI_{\rm MI}). Raman spectra obtained in a backscattering geometry with light polarized in the ab-plane reveal 9 B1g_{1g} phonon modes (140, 215, 265, 269, 292, 388, 459, 534, and 683 cm1^{-1}) and 9 Ag_g phonon modes (126, 192, 204, 251, 304, 322, 356, 395, and 607 cm1^{-1}) for the orthorhombic crystal structure (Pbca-D2h15_{2h}^{15}). With increasing temperature toward {\it T}MI_{\rm MI}, the observed phonon modes shift to lower energies and exhibit reduced spectral weights, reflecting structural changes associated with the elongation of the RuO6_6 octahedra. Interestingly, the phonons exhibit significant increases in linewidths and asymmetries for {\it T} >> {\it T}N_{\rm N}. These results indicate that there is an increase in the effective number of electrons and the electron-phonon interaction strengths as the temperature is raised through {\it T}N_{\rm N}, suggesting the presence of orbital fluctuations in the temperature regime {\it T}N_{\rm N} << {\it T} << {\it T}MI_{\rm MI}.Comment: 6 pages, 4 figure

    Strong diamagnetic response and specific heat anomaly above T_c in underdoped La_(2-x)Sr_xCuO_4

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    By measuring AC susceptibility using a very low amplitude of the AC field (<1 mG) it is shown that underdoped samples of La_(2-x)Sr_xCuO_4 (LASCO), are diamagnetic in a temperature region above T_c up to a temperature T^*. This behavior is only observed with AC fields along the c-axis whereas for fields in the ab-plane no diamagnetism above Tc was detected. The diamagnetism is almost frequency independent in the frequency range 0.1-10 kHz. At T* a broad step anomaly in the specific heat is inferred through measurements of the elastic constant c33. We suggest that the observed diamagnetism and the anomaly in the elastic constant are associated with the existence of phase incoherent Cooper pairs between Tc and T*.Comment: 5 pages 7 figures, to appear in Phys. rev

    Extraction of thermal and electromagnetic properties in 45Ti

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    The level density and gamma-ray strength function of 45Ti have been determined by use of the Oslo method. The particle-gamma coincidences from the 46Ti(p,d gamma)45Ti pick-up reaction with 32 MeV protons are utilized to obtain gamma-ray spectra as function of excitation energy. The extracted level density and strength function are compared with models, which are found to describe these quantities satisfactorily. The data do not reveal any single-particle energy gaps of the underlying doubly magic 40Ca core, probably due to the strong quadruple deformation

    Level densities and thermodynamical properties of Pt and Au isotopes

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    The nuclear level densities of 194196^{194-196}Pt and 197,198^{197,198}Au below the neutron separation energy have been measured using transfer and scattering reactions. All the level density distributions follow the constant-temperature description. Each group of isotopes is characterized by the same temperature above the energy threshold corresponding to the breaking of the first Cooper pair. A constant entropy excess ΔS=1.9\Delta S=1.9 and 1.11.1 kBk_B is observed in 195^{195}Pt and 198^{198}Au with respect to 196^{196}Pt and 197^{197}Au, respectively, giving information on the available single-particle level space for the last unpaired valence neutron. The breaking of nucleon Cooper pairs is revealed by sequential peaks in the microcanonical caloric curve
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