154 research outputs found
Detection of electronic nematicity using scanning tunneling microscopy
Electronic nematic phases have been proposed to occur in various correlated
electron systems and were recently claimed to have been detected in scanning
tunneling microscopy (STM) conductance maps of the pseudogap states of the
cuprate high-temperature superconductor Bi2Sr2CaCu2O8+x (Bi-2212). We
investigate the influence of anisotropic STM tip structures on such
measurements and establish, with a model calculation, the presence of a
tunneling interference effect within an STM junction that induces
energy-dependent symmetry-breaking features in the conductance maps. We
experimentally confirm this phenomenon on different correlated electron
systems, including measurements in the pseudogap state of Bi-2212, showing that
the apparent nematic behavior of the imaged crystal lattice is likely not due
to nematic order but is related to how a realistic STM tip probes the band
structure of a material. We further establish that this interference effect can
be used as a sensitive probe of changes in the momentum structure of the
sample's quasiparticles as a function of energy.Comment: Accepted for publication (PRB - Rapid Communications). Main text (5
pages, 4 figures) + Supplemental Material (4 pages, 4 figures
Visualizing heavy fermions emerging in a quantum critical Kondo lattice
In solids containing elements with f orbitals, the interaction between
f-electron spins and those of itinerant electrons leads to the development of
low-energy fermionic excitations with a heavy effective mass. These excitations
are fundamental to the appearance of unconventional superconductivity and
non-Fermi-liquid behaviour observed in actinide- and lanthanide-based
compounds. Here we use spectroscopic mapping with the scanning tunnelling
microscope to detect the emergence of heavy excitations with lowering of
temperature in a prototypical family of cerium-based heavy-fermion compounds.
We demonstrate the sensitivity of the tunnelling process to the composite
nature of these heavy quasiparticles, which arises from quantum entanglement of
itinerant conduction and f electrons. Scattering and interference of the
composite quasiparticles is used to resolve their energy-momentum structure and
to extract their mass enhancement, which develops with decreasing temperature.
The lifetime of the emergent heavy quasiparticles reveals signatures of
enhanced scattering and their spectral lineshape shows evidence of
energy-temperature scaling. These findings demonstrate that proximity to a
quantum critical point results in critical damping of the emergent heavy
excitation of our Kondo lattice system.Comment: preprint version, 26 pages, 6 figures. Supplementary: 15 pages, 14
figure
Evidence of Aquaporin 4 Regulation by Thyroid Hormone During Mouse Brain Development and in Cultured Human Glioblastoma Multiforme Cells
Accumulating evidence indicates that thyroid function and the thyroid hormones L-thyroxine (T4) and L-triiodothyronine (T3) are important factors contributing to the improvement of various pathologies of the central nervous system, including stroke, and various types of cancer, including glioblastoma multiforme (GBM). Low levels of T3 are correlated with the poorest outcome of post-stroke brain function, as well as an increased migration and proliferation of GBM tumor cells. Thyroid hormones are known to stimulate maturation and brain development. Aquaporin 4 (AQP4) is a key factor mediating the cell swelling and edema that occurs during ischemic stroke, and plays a potential role in the migration and proliferation of GBM tumor cells. In this study, as a possible therapeutic target for GBM, we investigated the potential role of T3 in the expression of AQP4 during different stages of mouse brain development. Pregnant mice at gestational day 18, or young animals at postnatal days 27 and 57, received injection of T3 (1 μg/g) or NaOH (0.02 N vehicle). The brains of mice sacrificed on postnatal days 0, 30, and 60 were perfused with 4% paraformaldehyde and sections were prepared for immunohistochemistry of AQP4. AQP4 immunofluorescence was measured in the mouse brains and human GBM cell lines. We found that distribution of AQP4 was localized in astrocytes of the periventricular, subpial, and cerebral parenchyma. Newborn mice treated with T3 showed a significant decrease in AQP4 immunoreactivity followed by an increased expression at P30 and a subsequent stabilization of aquaporin levels in adulthood. All GBM cell lines examined exhibited significantly lower AQP4 expression than cultured astrocytes. T3 treatment significantly downregulated AQP4 in GBM-95 cells but did not influence the rate of GBM cell migration measured 24 h after treatment initiation. Collectively, our results showed that AQP4 expression is developmentally regulated by T3 in astrocytes of the cerebral cortex of newborn and young mice, and is discretely downregulated in GBM cells. These findings indicate that higher concentrations of T3 thyroid hormone would be more suitable for reducing AQP4 in GBM tumorigenic cells, thereby resulting in better outcomes regarding the reduction of brain tumor cell migration and proliferation
Detection of a two-phonon mode in a cuprate superconductor via polarimetric RIXS
Recent improvements in the energy resolution of resonant inelastic x-ray
scattering experiments (RIXS) at the Cu-L edge have enabled the study of
lattice, spin, and charge excitations. Here, we report on the detection of a
low intensity signal at 140meV, twice the energy of the bond-stretching (BS)
phonon mode, in the cuprate superconductor
(Bi-2212).
Ultra-high resolution polarimetric RIXS measurements allow us to resolve the
outgoing polarization of the signal and identify this feature as a two-phonon
excitation. Further, we study the connection between the two-phonon mode and
the BS one-phonon mode by constructing a joint density of states toy model that
reproduces the key features of the data
Doping-dependent charge order correlations in electron-doped cuprates
Understanding the interplay between charge order (CO) and other phenomena (for example, pseudogap, antiferromagnetism, and superconductivity) is one of the central questions in the cuprate high-temperature superconductors. The discovery that similar forms of CO exist in both hole- and electron-doped cuprates opened a path to determine what subset of the CO phenomenology is universal to all the cuprates. We use resonant x-ray scattering to measure the CO correlations in electron-doped cuprates (La2−xCexCuO4 and Nd2−xCexCuO4) and their relationship to antiferromagnetism, pseudogap, and superconductivity. Detailed measurements of Nd2−xCexCuO4 show that CO is present in the x = 0.059 to 0.166 range and that its doping-dependent wave vector is consistent with the separation between straight segments of the Fermi surface. The CO onset temperature is highest between x = 0.106 and 0.166 but decreases at lower doping levels, indicating that it is not tied to the appearance of antiferromagnetic correlations or the pseudogap. Near optimal doping, where the CO wave vector is also consistent with a previously observed phonon anomaly, measurements of the CO below and above the superconducting transition temperature, or in a magnetic field, show that the CO is insensitive to superconductivity. Overall, these findings indicate that, although verified in the electron-doped cuprates, material-dependent details determine whether the CO correlations acquire sufficient strength to compete for the ground state of the cuprates
Anomalous excitonic phase diagram in band-gap-tuned Ta2Ni(Se,S)5
During a band-gap-tuned semimetal-to-semiconductor transition, Coulomb
attraction between electrons and holes can cause spontaneously formed excitons
near the zero-band-gap point, or the Lifshitz transition point. This has become
an important route to realize bulk excitonic insulators -- an insulating ground
state distinct from single-particle band insulators. How this route manifests
from weak to strong coupling is not clear. In this work, using angle-resolved
photoemission spectroscopy (ARPES) and high-resolution synchrotron x-ray
diffraction (XRD), we investigate the broken symmetry state across the
semimetal-to-semiconductor transition in a leading bulk excitonic insulator
candidate system Ta2Ni(Se,S)5. A broken symmetry phase is found to be
continuously suppressed from the semimetal side to the semiconductor side,
contradicting the anticipated maximal excitonic instability around the Lifshitz
transition. Bolstered by first-principles and model calculations, we find
strong interband electron-phonon coupling to play a crucial role in the
enhanced symmetry breaking on the semimetal side of the phase diagram. Our
results not only provide insight into the longstanding debate of the nature of
intertwined orders in Ta2NiSe5, but also establish a basis for exploring
band-gap-tuned structural and electronic instabilities in strongly coupled
systems.Comment: 27 pages, 4 + 9 figure
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