Infrared spectroscopy of hole doped ABA-stacked trilayer graphene

Using infrared spectroscopy, we investigate bottom gated ABA-stacked trilayer graphene subject to an additional environment-induced p-type doping. We find that the Slonczewski-Weiss-McClure tight-binding model and the Kubo formula reproduce the gate voltage-modulated reflectivity spectra very accurately. This allows us to determine the charge densities and the potentials of the {\pi}-band electrons on all graphene layers separately and to extract the interlayer permittivity due to higher energy bands.Comment: 6 pages, 6 figures Corrected sign of fig 3 and visibilty of fig

Full Quantum Analysis of Two-Photon Absorption Using Two-Photon Wavefunction: Comparison with One-Photon Absorption

For dissipation-free photon-photon interaction at the single photon level, we analyze one-photon transition and two-photon transition induced by photon pairs in three-level atoms using two-photon wavefunctions. We show that the two-photon absorption can be substantially enhanced by adjusting the time correlation of photon pairs. We study two typical cases: Gaussian wavefunction and rectangular wavefunction. In the latter, we find that under special conditions one-photon transition is completely suppressed while the high probability of two-photon transition is maintained.Comment: 6 pages, 4 figure

General properties of response functions of nonequilibrium steady states

We derive general properties, which hold for both quantum and classical systems, of response functions of nonequilibrium steady states. We clarify differences from those of equilibrium states. In particular, sum rules and asymptotic behaviors are derived, and their implications are discussed. Since almost no assumptions are made, our results are applicable to diverse physical systems. We also demonstrate our results by a molecular dynamics simulation of a many-body interacting system.Comment: After publication of this paper, several typos were found, which have been fixed in the erratum (J. Phys. Soc. Jpn., 80 (2011) 128001). All the corrections have been made in this updated arXive version. 13 pages with 3 figure

Transient Oscillation of Currents in Quantum Hall Effect of Bloch Electrons

We consider the quantum Hall effect of two-dimensional electrons with a periodic potential and study the time dependence of the Hall and longitudinal currents when the electric field is applied abruptly. We find that the currents oscillate in time with very large frequencies because of quantum fluctuation and the oscillations eventually vanish, for their amplitudes decay as 1/t.Comment: 16 pages and 8 figure

Gate-induced magneto-oscillation phase anomalies in graphene bilayers

The magneto-oscillations in graphene bilayers are studied in the vicinity of the K and K' points of the Brillouin zone within the four-band continuum model ased on the simplest tight-binding approximation involving only the nearest neighbor interactions. The model is employed to construct Landau plots for a variety of carrier concentrations and bias strengths between the graphene planes. The quantum-mechanical and quasiclassical approaches are compared. We found that the quantum magneto-oscillations are only asymptotically periodic and reach the frequencies predicted quasiclassically for high indices of Landau levels. In unbiased bilayers the phase of oscillations is equal to the phase of massive fermions. Anomalous behavior of oscillation phases was found in biased bilayers with broken inversion symmetry. The oscillation frequencies again tend to quasiclassically predicted ones, which are the same for $K$ and $K'$, but the quantum approach yields the gate-tunable corrections to oscillation phases, which differ in sign for K and K'. These valley-dependent phase corrections give rise, instead of a single quasiclassical series of oscillations, to two series with the same frequency but shifted in phase.Comment: 8 pages, 8 figure

The electronic properties of bilayer graphene

We review the electronic properties of bilayer graphene, beginning with a description of the tight-binding model of bilayer graphene and the derivation of the effective Hamiltonian describing massive chiral quasiparticles in two parabolic bands at low energy. We take into account five tight-binding parameters of the Slonczewski-Weiss-McClure model of bulk graphite plus intra- and interlayer asymmetry between atomic sites which induce band gaps in the low-energy spectrum. The Hartree model of screening and band-gap opening due to interlayer asymmetry in the presence of external gates is presented. The tight-binding model is used to describe optical and transport properties including the integer quantum Hall effect, and we also discuss orbital magnetism, phonons and the influence of strain on electronic properties. We conclude with an overview of electronic interaction effects.Comment: review, 31 pages, 15 figure

Phase Transition in a One-Dimensional Extended Peierls-Hubbard Model with a Pulse of Oscillating Electric Field: I. Threshold Behavior in Ionic-to-Neutral Transition

Photoinduced dynamics of charge density and lattice displacements is calculated by solving the time-dependent Schr\"odinger equation for a one-dimensional extended Peierls-Hubbard model with alternating potentials for the mixed-stack organic charge-transfer complex, TTF-CA. A pulse of oscillating electric field is incorporated into the Peierls phase of the transfer integral. The frequency, the amplitude, and the duration of the pulse are varied to study the nonlinear and cooperative character of the photoinduced transition. When the dimerized ionic phase is photoexcited, the threshold behavior is clearly observed by plotting the final ionicity as a function of the increment of the total energy. Above the threshold photoexcitation, the electronic state reaches the neutral one with equidistant molecules after the electric field is turned off. The transition is initiated by nucleation of a metastable neutral domain, for which an electric field with frequency below the linear absorption peak is more effective than that at the peak. When the pulse is strong and short, the charge transfer takes place on the same time scale with the disappearance of dimerization. As the pulse becomes weak and long, the dimerization-induced polarization is disordered to restore the inversion symmetry on average before the charge transfer takes place to bring the system neutral. Thus, a paraelectric ionic phase is transiently realized by a weak electric field. It is shown that infrared light also induces the ionic-to-neutral transition, which is characterized by the threshold behavior.Comment: 24 pages, 11 figure