255 research outputs found

    The band structure and Fermi surface of La0.6_{0.6}Sr0.4_{0.4}MnO3_{3} thin films studied by in-situ angle-resolved photoemission spectroscopy

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    We have performed an in situ angle-resolved photoemission spectroscopy (ARPES) on single-crystal surfaces of La0.6_{0.6}Sr0.4_{0.4}MnO3_{3} (LSMO) thin films grown on SrTiO3_{3} (001) substrates by laser molecular beam epitaxy, and investigated the electronic structure near the Fermi level (EFE_{F}). The experimental results were compared with the band-structure calculation based on LDA + UU. The band structure of LSMO thin films consists of several highly dispersive O 2pp derived bands in the binding energy range of 2.0 - 6.0 eV and Mn 3dd derived bands near EFE_{F}. ARPES spectra around the GammaGamma point show a dispersive band near EFE_{F} indicative of an electron pocket centered at the GammaGamma point, although it was not so clearly resolved as an electronlike pocket due to the suppression of spectral weight in the vicinity of EFE_{F}. Compared with the band-structure calculation, the observed conduction band is assigned to the Mn 3degde_{g} majority-spin band responsible for the half-metallic nature of LSMO. We have found that the estimated size of the Fermi surface is consistent with the prediction of the band-structure calculation, while the band width becomes significantly narrower than the calculation. Also, the intensity near EFE_{F} is strongly reduced. The origin of these discrepancies between the experiment and the calculation is discussed.Comment: 7 pages, 5 figure

    Gradual Disappearance of the Fermi Surface near the Metal-Insulator Transition in La1x_{1-x}Srx_{x}MnO3_{3}

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    We report the first observation of changes in the electronic structure of La1x_{1-x}Srx_{x}MnO3_{3} (LSMO) across the filling-control metal-insulator (MI) transition by means of in situ angle-resolved photoemission spectroscopy (ARPES) of epitaxial thin films. The Fermi surface gradually disappears near the MI transition by transferring the spectral weight from the coherent band near the Fermi level (EFE_{F}) to the lower Hubbard band, whereas a pseudogap behavior also exists in the ARPES spectra in the close vicinity of EFE_{F} for the metallic LSMO. These results indicate that the spectral weight transfer derived from strong electron-electron interaction dominates the gap formation in LSMO associated with the filling-control MI transition.Comment: 11 pages, 4 figure

    New Perspectives in Sinographic Language Processing Through the Use of Character Structure

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    Chinese characters have a complex and hierarchical graphical structure carrying both semantic and phonetic information. We use this structure to enhance the text model and obtain better results in standard NLP operations. First of all, to tackle the problem of graphical variation we define allographic classes of characters. Next, the relation of inclusion of a subcharacter in a characters, provides us with a directed graph of allographic classes. We provide this graph with two weights: semanticity (semantic relation between subcharacter and character) and phoneticity (phonetic relation) and calculate "most semantic subcharacter paths" for each character. Finally, adding the information contained in these paths to unigrams we claim to increase the efficiency of text mining methods. We evaluate our method on a text classification task on two corpora (Chinese and Japanese) of a total of 18 million characters and get an improvement of 3% on an already high baseline of 89.6% precision, obtained by a linear SVM classifier. Other possible applications and perspectives of the system are discussed.Comment: 17 pages, 5 figures, presented at CICLing 201

    Ab-initio electronic and magnetic structure in La_0.66Sr_0.33MnO_3: strain and correlation effects

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    The effects of tetragonal strain on electronic and magnetic properties of strontium-doped lanthanum manganite, La_{2/3}Sr_{1/3}MnO_3 (LSMO), are investigated by means of density-functional methods. As far as the structural properties are concerned, the comparison between theory and experiments for LSMO strained on the most commonly used substrates, shows an overall good agreement: the slight overestimate (at most of 1-1.5 %) for the equilibrium out-of-plane lattice constants points to possible defects in real samples. The inclusion of a Hubbard-like contribution on the Mn d states, according to the so-called "LSDA+U" approach, is rather ineffective from the structural point of view, but much more important from the electronic and magnetic point of view. In particular, full half-metallicity, which is missed within a bare density-functional approach, is recovered within LSDA+U, in agreement with experiments. Moreover, the half-metallic behavior, particularly relevant for spin-injection purposes, is independent on the chosen substrate and is achieved for all the considered in-plane lattice constants. More generally, strain effects are not seen to crucially affect the electronic structure: within the considered tetragonalization range, the minority gap is only slightly (i.e. by about 0.1-0.2 eV) affected by a tensile or compressive strain. Nevertheless, we show that the growth on a smaller in-plane lattice constant can stabilize the out-of-plane vs in-plane e_g orbital and significatively change their relative occupancy. Since e_g orbitals are key quantities for the double-exchange mechanism, strain effects are confirmed to be crucial for the resulting magnetic coupling.Comment: 16 pages, 7 figures, to be published on J. Phys.: Condensed Matte

    Systematic tight-binding analysis of ARPES spectra of transition-metal oxides

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    We have performed systematic tight-binding (TB) analyses of the angle-resolved photoemission spectroscopy (ARPES) spectra of transition-metal (TM) oxides AMMO3_3 (M=M= Ti, V, Mn, and Fe) with the perovskite-type structure and compared the obtained parameters with those obtained from configuration-interaction (CI) cluster-model analyses of photoemission spectra. The values of ϵdϵp\epsilon_d-\epsilon_p from ARPES are found to be similar to the charge-transfer energy Δ\Delta from O 2p2p orbitals to empty TM 3d orbitals and much larger than ΔU/2\Delta-U/2 (UU: on-site Coulomb energy) expected for Mott-Hubbard-type compounds including SrVO3_3. ϵdϵp\epsilon_d-\epsilon_p values from {\it ab initio} band-structure calculations show similar behaviors to those from ARPES. The values of the pdp-d transfer integrals to describe the global electronic structure are found to be similar in all the estimates, whereas additional narrowing beyond the TB description occurs in the ARPES spectra of the dd band.Comment: 5 pages, 3 figure

    Photo induced antiferromagnetic ferromagnetic and spin state transition in a double perovskite cobalt oxide thin film

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    Investigation of ultrafast dynamic behaviors can provide novel insights about the coupling mechanisms among multiple degrees of freedom in condensed matters, such as lattice, magnetism and electronic structure. Here we investigate both the ferromagnetic FM and antiferromagnetic AFM dynamics of a strongly correlated oxide system, GdBaCo2O5.5 thin film by time resolved x ray magnetic circular dichroism in reflectivity XMCDR and resonant magnetic x ray diffraction RMXD . A photo induced AFM FM transition characterized by an increase of the transient XMCDR sensitive to FM order beyond the unpumped value and a decay of RMXD sensitive to AFM order was observed. The photon energy dependence of the transient XMCDR and reflectivity could be interpreted as a concomitant photo induced spin state transition SST . The AFM FM transition and SST couple with each other in the time domain, resulting in unusual dynamic behaviors of the magnetis

    Measurement of Dijet Angular Distributions at CDF

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    We have used 106 pb^-1 of data collected in proton-antiproton collisions at sqrt(s)=1.8 TeV by the Collider Detector at Fermilab to measure jet angular distributions in events with two jets in the final state. The angular distributions agree with next to leading order (NLO) predictions of Quantum Chromodynamics (QCD) in all dijet invariant mass regions. The data exclude at 95% confidence level (CL) a model of quark substructure in which only up and down quarks are composite and the contact interaction scale is Lambda_ud(+) < 1.6 TeV or Lambda_ud(-) < 1.4 TeV. For a model in which all quarks are composite the excluded regions are Lambda(+) < 1.8 TeV and Lambda(-) < 1. 6 TeV.Comment: 16 pages, 2 figures, 2 tables, LaTex, using epsf.sty. Submitted to Physical Review Letters on September 17, 1996. Postscript file of full paper available at http://www-cdf.fnal.gov/physics/pub96/cdf3773_dijet_angle_prl.p

    Search for charged Higgs decays of the top quark using hadronic tau decays

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    We present the result of a search for charged Higgs decays of the top quark, produced in ppˉp\bar{p} collisions at s=\surd s = 1.8 TeV. When the charged Higgs is heavy and decays to a tau lepton, which subsequently decays hadronically, the resulting events have a unique signature: large missing transverse energy and the low-charged-multiplicity tau. Data collected in the period 1992-1993 at the Collider Detector at Fermilab, corresponding to 18.7±\pm0.7~pb1^{-1}, exclude new regions of combined top quark and charged Higgs mass, in extensions to the standard model with two Higgs doublets.Comment: uuencoded, gzipped tar file of LaTeX and 6 Postscript figures; 11 pp; submitted to Phys. Rev.
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