404 research outputs found
Observation of Field-Induced Transverse N\'{e}el Ordering in the Spin Gap System TlCuCl
Neutron elastic scattering experiments have been performed on the spin gap
system TlCuCl in magnetic fields parallel to the -axis. The magnetic
Bragg peaks which indicate the field-induced N\'{e}el ordering were observed
for magnetic field higher than the gap field T at with odd in the plane. The spin structure in the ordered
phase was determined. The temperature and field dependence of the Bragg peak
intensities and the phase boundary obtained were discussed in connection with a
recent theory which describes the field-induced N\'{e}el ordering as a
Bose-Einstein condensation of magnons.Comment: 4 pages, 5 eps figures, jpsj styl
Simultaneous loss of interlayer coherence and long-range magnetism in quasi-two-dimensional PdCrO\u3csub\u3e2\u3c/sub\u3e
Incoherent transport is an important feature of many anisotropic quantum materials but often its origin is not well understood. Here, the authors show that in a layered quantum magnet, incoherence is driven by the interaction of electrons with spin fluctuations after the
Random Bond Effect in the Quantum Spin System (TlK)CuCl
The effect of exchange bond randomness on the ground state and the
field-induced magnetic ordering was investigated through magnetization
measurements in the spin-1/2 mixed quantum spin system
(TlK)CuCl for . Both parent compounds TlCuCl and
KCuCl are coupled spin dimer systems, which have the singlet ground state
with excitation gaps K and 31 K, respectively. Due to
bond randomness, the singlet ground state turns into the magnetic state with
finite susceptibility, nevertheless, the excitation gap remains. Field-induced
magnetic ordering, which can be described by the Bose condensation of excited
triplets, magnons, was observed as in the parent systems. The phase transition
temperature is suppressed by the bond randomness. This behavior may be
attributed to the localization effect.Comment: 19 pages, 7 figures, 12 eps files, revtex, will appear in PR
Drastic Change of Magnetic Phase Diagram in Doped Quantum Antiferromagnet TlCuMgCl
TlCuCl is a coupled spin dimer system, which has a singlet ground state
with an excitation gap of = 5.5 T.
TlCuMgCl doped with nonmagnetic Mg ions undergoes
impurity-induced magnetic ordering. Because triplet excitation with a finite
gap still remains, this doped system can also undergo magnetic-field-induced
magnetic ordering. By specific heat measurements and neutron scattering
experiments under a magnetic field, we investigated the phase diagram in
TlCuMgCl with , and found that impurity- and
field-induced ordered phases are the same. The gapped spin liquid state
observed in pure TlCuCl is completely wiped out by the small amount of
doping.Comment: 9 pages, 5 figures, jpsj2 class file, to be published in J. Phy. Soc.
Jpn. Vol.75 No.3 (2006); layout changed, unrelated figure remove
Spin-resonance modes of the spin-gap magnet TlCuCl_3
Three kinds of magnetic resonance signals were detected in crystals of the
spin-gap magnet TlCuCl_3.
First, we have observed the microwave absorption due to the excitation of the
transitions between the singlet ground state and the excited triplet states.
This mode has the linear frequency-field dependence corresponding to the
previously known value of the zero-field spin-gap of 156 GHz and to the closing
of spin-gap at the magnetic field H_c of about 50 kOe.
Second, the thermally activated resonance absorption due to the transitions
between the spin sublevels of the triplet excitations was found. These
sublevels are split by the crystal field and external magnetic field.
Finally, we have observed antiferromagnetic resonance absorption in the
field-induced antiferromagnetic phase above the critical field H_c. This
resonance frequency is strongly anisotropic with respect to the direction of
the magnetic field.Comment: v.2: typo correction (one of the field directions was misprinted in
the v.1
Pressure-Induced Magnetic Quantum Phase Transitions from Gapped Ground State in TlCuCl3
Magnetization maesurements under hydrostatic pressure were performed on an
S=1/2 coupled spin system TlCuCl3 with a gapped ground state under magnetic
field H parallel to the [2,0,1] direction. With increasing applied pressure P,
the gap decreases and closes completely at Pc=0.42 kbar. For P>Pc, TlCuCl3
undergoes antiferromagnetic ordering. A spin-flop transition was observed at
Hsf=0.7T. The spin-flop field is approximately independent of pressure,
although the sublattice magnetization increases with pressure. The gap and Neel
temperature are presented as function is attributed to to the relative
enhancement of the interdimer exchange interactions compared with the
intradimer exchange interaction.Comment: 4pages,3figures To be published in J. Phys. Soc. Jpn. Vol.73 No.1
Few-electron molecular states and their transitions in a single InAs quantum dot molecule
We study electronic configurations in a single pair of vertically coupled
self-assembled InAs quantum dots, holding just a few electrons. By comparing
the experimental data of non-linear single-electron transport spectra in a
magnetic field with many-body calculations, we identify the spin and orbital
configurations to confirm the formation of molecular states by filling both the
quantum mechanically coupled symmetric and anti-symmetric states. Filling of
the anti-symmetric states is less favored with increasing magnetic field, and
this leads to various magnetic field induced transitions in the molecular
states.Comment: 14 pages, 3 figures, Accepted for publication in Phys. Rev. Let
Impurity-Induced Antiferromagnetic Ordering in the Spin Gap System TlCuCl_3
The magnetization measurements have been performed on the doped spin gap
system TlCu_{1-x}Mg_xCl_3 with x <= 0.025. The parent compound TlCuCl_3 is a
three-dimensional coupled spin dimer system with the excitation gap Delta/k_B =
7.7 K. The impurity-induced antiferromagnetic ordering was clearly observed.
The easy axis lies in the (0,1,0) plane. It was found that the transition
temperature increases with increasing Mg^{2+} concentration x, while the
spin-flop transition field is almost independent of x. The magnetization curve
suggests that the impurity-induced antiferromagnetic ordering coexists with the
spin gap for x <= 0.017.Comment: 5 pages, 6 figures, revtex styl
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