48 research outputs found
Band Calculations for Ce Compounds with AuCu-type Crystal Structure on the basis of Dynamical Mean Field Theory I. CePd and CeRh
Band calculations for Ce compounds with the AuCu-type crystal structure
were carried out on the basis of dynamical mean field theory (DMFT). The
auxiliary impurity problem was solved by a method named NCAvc
(noncrossing approximation including the state as a vertex correction).
The calculations take into account the crystal-field splitting, the spin-orbit
interaction, and the correct exchange process of the virtual excitation. These are necessary features in the
quantitative band theory for Ce compounds and in the calculation of their
excitation spectra. The results of applying the calculation to CePd and
CeRh are presented as the first in a series of papers. The experimental
results of the photoemission spectrum (PES), the inverse PES, the
angle-resolved PES, and the magnetic excitation spectra were reasonably
reproduced by the first-principles DMFT band calculation. At low temperatures,
the Fermi surface (FS) structure of CePd is similar to that of the band
obtained by the local density approximation. It gradually changes into a form
that is similar to the FS of LaPd as the temperature increases, since the
band shifts to the high-energy side and the lifetime broadening becomes
large.}Comment: 12 pasges, 13 figure
Band Calculation for Ce-compounds on the basis of Dynamical Mean Field Theory
The band calculation scheme for electron compounds is developed on the
basis of the dynamical mean field theory (DMFT) and the LMTO method. The
auxiliary impurity problem is solved by a method named as NCAv', which
includes the correct exchange process of the virtual
excitation as the vertex correction to the non-crossing approximation (NCA) for
the fluctuation. This method leads to the correct magnitude
of the Kondo temperature, , and makes it possible to carry out
quantitative DMFT calculation including the crystalline field (CF) and the
spin-orbit (SO) splitting of the self-energy. The magnetic excitation spectra
are also calculated to estimate . It is applied to Ce metal and CeSb
at T=300 K as the first step. In Ce metal, the hybridization intensity (HI)
just below the Fermi energy is reduced in the DMFT band. The photo-emission
spectra (PES) have a conspicuous SO side peak, similar to that of experiments.
is estimated to be about 70 K in -Ce, while to be about
1700 K in -Ce. In CeSb, the double-peak-like structure of PES is
reproduced. In addition, which is not so low is obtained because HI
is enhanced just at the Fermi energy in the DMFT band.Comment: 30pages, 18 figure
Magnetic fluctuations in frustrated Laves hydrides R(Mn_{1-x}Al_{x})_{2}H_{y}
By neutron scattering, we have studied the spin correlations and spin
fluctuations in frustrated Laves hydrides, where magnetic disorder sets in the
topologically frustrated Mn lattice. Below the transition towards short range
magnetic order, static spin clusters coexist with fluctuating and alsmost
uncorrelated spins. The magnetic response shows a complexe lineshape, connected
with the presence of the magnetic inhomogeneities. Its analysis shows the
existence of two different processes, relaxation and local excitations, for the
spin fluctuations below the transition. The paramagnetic fluctuations are
discussed in comparison with classical spin glasses, cluster glasses, and non
Fermi liquid itinerant magnets
Electronic structure of the strongly hybridized ferromagnet CeFe2
We report on results from high-energy spectroscopic measurements on CeFe2, a
system of particular interest due to its anomalous ferromagnetism with an
unusually low Curie temperature and small magnetization compared to the other
rare earth-iron Laves phase compounds. Our experimental results indicate very
strong hybridization of the Ce 4f states with the delocalized band states,
mainly the Fe 3d states. In the interpretation and analysis of our measured
spectra, we have made use of two different theoretical approaches: The first
one is based on the Anderson impurity model, with surface contributions
explicitly taken into account. The second method consists of band-structure
calculations for bulk CeFe2. The analysis based on the Anderson impurity model
gives calculated spectra in good agreement with the whole range of measured
spectra, and reveals that the Ce 4f -- Fe 3d hybridization is considerably
reduced at the surface, resulting in even stronger hybridization in the bulk
than previously thought. The band-structure calculations are ab initio
full-potential linear muffin-tin orbital calculations within the
local-spin-density approximation of the density functional. The Ce 4f electrons
were treated as itinerant band electrons. Interestingly, the Ce 4f partial
density of states obtained from the band-structure calculations also agree well
with the experimental spectra concerning both the 4f peak position and the 4f
bandwidth, if the surface effects are properly taken into account. In addition,
results, notably the partial spin magnetic moments, from the band-structure
calculations are discussed in some detail and compared to experimental findings
and earlier calculations.Comment: 10 pages, 8 figures, to appear in Phys. Rev. B in December 200
Unconventional ferromagnetic and spin-glass states of the reentrant spin glass Fe0.7Al0.3
Spin excitations of single crystal Fe0.7Al0.3 were investigated over a wide
range in energy and reciprocal space with inelastic neutron scattering. In the
ferromagnetic phase, propagating spin wave modes become paramagnon-like
diffusive modes beyond a critical wave vector q0, indicating substantial
disorder in the long-range ordered state. In the spin glass phase, spin
dynamics is strongly q-dependent, suggesting remnant short-range spin
correlations. Quantitative model for S(energy,q) in the ``ferromagnetic'' phase
is determined.Comment: 4 pages, 5 figure
Suppression of the structural phase transition in by large magnetic fields
The transition in CeLaTh is measured
as a function of applied magnetic field using both resistivity and
magnetization. The transition temperature decreases with
increasing magnetic field, reaching zero temperature at around 56 T. The
magnetic-field dependence of the transition temperature may be fitted using a
model that invokes the field and temperature dependence of the entropy of the
-electron moments of the phase, suggesting that the volume
collapse in Ce and its alloys is primarily driven by entropic considerations
Microwave studies of the fractional Josephson effect in HgTe-based Josephson junctions
The rise of topological phases of matter is strongly connected to their
potential to host Majorana bound states, a powerful ingredient in the search
for a robust, topologically protected, quantum information processing. In order
to produce such states, a method of choice is to induce superconductivity in
topological insulators. The engineering of the interplay between
superconductivity and the electronic properties of a topological insulator is a
challenging task and it is consequently very important to understand the
physics of simple superconducting devices such as Josephson junctions, in which
new topological properties are expected to emerge. In this article, we review
recent experiments investigating topological superconductivity in topological
insulators, using microwave excitation and detection techniques. More
precisely, we have fabricated and studied topological Josephson junctions made
of HgTe weak links in contact with two Al or Nb contacts. In such devices, we
have observed two signatures of the fractional Josephson effect, which is
expected to emerge from topologically-protected gapless Andreev bound states.
We first recall the theoretical background on topological Josephson junctions,
then move to the experimental observations. Then, we assess the topological
origin of the observed features and conclude with an outlook towards more
advanced microwave spectroscopy experiments, currently under development.Comment: Lectures given at the San Sebastian Topological Matter School 2017,
published in "Topological Matter. Springer Series in Solid-State Sciences,
vol 190. Springer
A Gestational High Protein Diet Affects the Abundance of Muscle Transcripts Related to Cell Cycle Regulation throughout Development in Porcine Progeny
BACKGROUND: In various animal models pregnancy diets have been shown to affect offspring phenotype. Indeed, the underlying programming of development is associated with modulations in birth weight, body composition, and continual diet-dependent modifications of offspring metabolism until adulthood, producing the hypothesis that the offspring's transcriptome is permanently altered depending on maternal diet. METHODOLOGY/PRINCIPAL FINDINGS: To assess alterations of the offspring's transcriptome due to gestational protein supply, German Landrace sows were fed isoenergetic diets containing protein levels of either 30% (high protein--HP) or 12% (adequate protein--AP) throughout their pregnancy. Offspring muscle tissue (M. longissimus dorsi) was collected at 94 days post conception (dpc), and 1, 28, and 188 days post natum (dpn) for use with Affymetrix GeneChip Porcine Genome Arrays and subsequent statistical and Ingenuity pathway analyses. Numerous transcripts were found to have altered abundance at 94 dpc and 1 dpn; at 28 dpn no transcripts were altered, and at 188 dpn only a few transcripts showed a different abundance between diet groups. However, when assessing transcriptional changes across developmental time points, marked differences were obvious among the dietary groups. Depending on the gestational dietary exposure, short- and long-term effects were observed for mRNA expression of genes related to cell cycle regulation, energy metabolism, growth factor signaling pathways, and nucleic acid metabolism. In particular, the abundance of transcripts related to cell cycle remained divergent among the groups during development. CONCLUSION: Expression analysis indicates that maternal protein supply induced programming of the offspring's genome; early postnatal compensation of the slight growth retardation obvious at birth in HP piglets resulted, as did a permanently different developmental alteration and responsiveness to the common environment of the transcriptome. The transcriptome modulations are interpreted as the molecular equivalent of developmental plasticity of the offspring that necessitates adaptation and maintenance of the organismal phenotype
The spectral and magnetic properties of - and -Ce from the Dynamical Mean-Field Theory and Local Density Approximation
We have calculated ground state properties and excitation spectra for Ce
metal with the {\it ab initio} computational scheme combining local density
approximation and dynamical mean-field theory (LDA+DMFT). We considered all
electronic states, i.e. correlated f-states and non-correlated s-, p- and
d-states. The strong local correlations (Coulomb interaction) among the
f-states lead to typical many-body resonances in the partial f-density, such as
lower and upper Hubbard band. Additionally the well known Kondo resonance is
observed. The s-, p- and d-densities show small to mediate renormalization
effects due to hybridization. We observe different Kondo temperatures for
- and -Ce ( and
), due to strong volume dependence of the effective
hybridization strength for the localized f-electrons. Finally we compare our
results with a variety of experimental data, i.e. from photoemission
spectroscopy (PES), inverse photoemission spectroscopy (BIS), resonant inverse
photoemission spectroscopy (RIPES) and magnetic susceptibility measurements.Comment: 7 pages, 4 figure