Large non-adiabatic hole polarons and matrix element effects in the angle-resolved photoemission spectroscopy of dielectric cuprates

It has been made an extention of the conventional theory based on the assumption of the well isolated Zhang-Rice singlet to be a first electron-removal state in dielectric copper oxide. One assumes the photohole has been localised on either small (pseudo)Jahn-Teller polaron or large non-adiabatic polaron enclosed one or four to five $CuO_4$ centers, respectively, with active one-center valent $(^{1}A_{1g}-{}^{1,3}E_{u})$ manifold. In the framework of the cluster model we have performed a model microscopic calculation of the ${\bf k}$-dependence of the matrix element effects and photon polarization effects for the angle-resolved photoemission in dielectric cuprate like $Sr_{2}CuO_{2}Cl_{2}$. We show that effects like the ''remnant Fermi surface'' detected in ARPES experiment for $Ca_{2}CuO_{2}Cl_{2}$ may be, in fact, a reflection of the matrix element effects, not a reflection of the original band-structure Fermi surface, or the strong antiferromagnetic correlations. The measured dispersion-like features in the low-energy part of the ARPES spectra may be a manifestation of the complex momentum-dependent spectral line-shape of the large PJT polaron response, not the dispersion of the well-isolated Zhang-Rice singlet in antiferromagnetic matrix.Comment: 16 pages, TeX, 9 eps figures adde

Superconductivity in model cuprate as an S=1 pseudomagnon condensation

We make use of the S=1 pseudospin formalism to describe the charge degree of freedom in a model high-$T_c$ cuprate with the on-site Hilbert space reduced to the three effective valence centers, nominally Cu$^{1+,\,2+,\,3+}$. Starting with a parent cuprate as an analogue of the quantum paramagnet ground state and using the Schwinger boson technique we found the pseudospin spectrum and conditions for the pseudomagnon condensation with phase transition to a superconducting state.Comment: Version to be published in JLT

Role of the Dzyaloshinskii-Moriya interaction in multiferroic perovskites

With the perovskite multiferroic RMnO3 (R = Gd, Tb, Dy) as guidance, we argue that the Dzyaloshinskii-Moriya interaction (DMI) provides the microscopic mechanism for the coexistence and strong coupling between ferroelectricity and incommensurate magnetism. We use Monte-Carlo simulations and zero temperature exact calculations to study a model incorporating the double-exchange, superexchange, Jahn-Teller and DMI terms. The phase diagram contains a multiferroic phase between A and E antiferromagnetic phases, in excellent agreement with experiments.Comment: 6 pages, 5 figure

Electron-conformational transformations in nanoscopic RyR channels govern both the heart's contraction and beating

We show that a simple biophysically based electron-conformational model of RyR channel is able to explain and describe on equal footing the oscillatory regime of the heart's cell release unit both in sinoatrial node (pacemaker) cells under normal physiological conditions and in ventricular myocytes under Ca$^{2+}$ SR overload.Comment: 6 pages, 3 figure

Complex Chiral Modulations in FeGe close to Magnetic Ordering

We report on detailed polarized small-angle neutron scattering on cubic FeGe in magnetic fields applied either along (transverse) the scattering vector or parallel (longitudinal)to the neutron beam. The ($H,T$) phase diagrams for all principal axes contain a segmented $A$-phase region just below the onset of magnetic order. Hexagonal Bragg-spot patterns were observed across the entire $A$-phase region for the longitudinal geometry. Scattering intensity was observed in parts of the A phase for both scattering configurations. Only in a distinct pocket ($A_1$) vanishing scattering intensity was found in the transverse geometry.Comment: This paper has been withdrawn by the author due to misunderstanding with some of the co-author

Disproportionation and electronic phase separation in parent manganite LaMnO_3

Nominally pure undoped parent manganite LaMnO_3 exhibits a puzzling behavior inconsistent with a simple picture of an A-type antiferromagnetic insulator (A-AFI) with a cooperative Jahn-Teller ordering. We do assign its anomalous properties to charge transfer instabilities and competition between insulating A-AFI phase and metallic-like dynamically disproportionated phase formally separated by a first-order phase transition at T_{disp}=T_{JT}\approx 750 K. The unconventional high-temperature phase is addressed to be a specific electron-hole Bose liquid (EHBL) rather than a simple "chemically" disproportionated R(Mn^{2+}Mn^{4+})O_3 phase. New phase does nucleate as a result of the charge transfer (CT) instability and evolves from the self-trapped CT excitons, or specific EH-dimers, which seem to be a precursor of both insulating and metallic-like ferromagnetic phases observed in manganites. We arrive at highly frustrated system of triplet (e_g^2)^3A_{2g} bosons moving in a lattice formed by hole Mn^{4+} centers. Starting with different experimental data we have reproduced a typical temperature dependence of the volume fraction of high-temperature mixed-valent EHBL phase. We argue that a slight nonisovalent substitution, photo-irradiation, external pressure or magnetic field gives rise to an electronic phase separation with a nucleation or an overgrowth of EH-droplets. Such a scenario provides a comprehensive explanation of numerous puzzling properties observed in parent and nonisovalently doped manganite LaMnO_3 including an intriguing manifestation of superconducting fluctuations.Comment: 20 pages, 8 figure

Dzyaloshinsky-Moriya antisymmetric exchange coupling in cuprates: Oxygen effects

We revisit a problem of Dzyaloshinsky-Moriya antisymmetric exchange coupling for a single bond in cuprates specifying the local spin-orbital contributions to Dzyaloshinsky vector focusing on the oxygen term. The Dzyaloshinsky vector and respective weak ferromagnetic moment is shown to be a superposition of comparable and, sometimes, competing local Cu and O contributions. The intermediate oxygen $^{17}$O Knight shift is shown to be an effective tool to inspect the effects of Dzyaloshinsky-Moriya coupling in an external magnetic field. We predict the effect of $strong$ oxygen weak antiferromagnetism in edge-shared CuO$_2$ chains due to uncompensated oxygen Dzyaloshinsky vectors. Finally, we revisit the effects of symmetric spin anisotropy, in particular, those directly induced by Dzyaloshinsky-Moriya coupling.Comment: 12 pages, 2 figures, submitted to JET

The Dzyaloshinskii-Moriya interaction is under control: an orchestrated flip of the chiral link between structure and magnetism for Fe1−x_{1-x}Cox_xSi

Monosilicides of 3d-metals frequently show a chiral magnetic ordering with the absolute configuration defined by the chirality of the crystal structure and the sign of the Dzyaloshinskii-Moriya interaction (DMI). Structural and magnetic chiralities are probed here for Fe$_{1-x}$Co$_x$Si series and their mutual relationship is found to be dependent on the chemical composition. The chirality of crystal structure was previously shown to be governed by crystal growth, and the value of the DMI is nearly the same for all monosilicides of Fe, Co and Mn. Our findings indicate that the sign of the DMI in Fe$_{1-x}$Co$_x$Si is controlled by the Co composition $x$, thus, opening a route towards controlled design of chiral spintronics devices.Comment: 4 pages, 4 figures, 1 tabl

Chiral criticality in doped Mn1−y_{1-y}Fey_ySi compounds

The critical spin fluctuations in doped compounds Mn$_{1-y}$Fe$_y$Si have been studied by means of ac-susceptibility measurements, polarized neutron small angle scattering and spin echo spectroscopy. It is shown that these compounds undergo the transition from the paramagnetic to helimagnetic phase through continuous, yet well distinguishable crossovers: (i) from paramagnetic to partially chiral, (ii) from partially chiral to highly chiral fluctuating state. The crossover points are identified on the basis of combined analysis of the temperature dependence of ac-susceptibility and polarized SANS data. The whole transition is marked by two inflection point of the temperature dependence of ac-susceptibility: the upper one corresponds to the crossover to partially chiral state at $T^*$, where the inverse correlation length $\kappa \approx 2 k$, the lower one corresponds to the transition to the spin helix structure. The intermediate crossover to the highly chiral phase is observed at the inflection point $T_k$ of the first derivative of ac-susceptibility, where $\kappa \approx k$. The temperature crossovers to the highly chiral fluctuating state is associated with the enhancing influence of the Dzyaloshinskii-Moria interaction close to $T_c$.Comment: 5 pages, 5 figures, 1 table, 13 cite