6,884 research outputs found
Time-resolved photoemission of correlated electrons driven out of equilibrium
We describe the temporal evolution of the time-resolved photoemission
response of the spinless Falicov-Kimball model driven out of equilibrium by
strong applied fields. The model is one of the few possessing a metal-insulator
transition and admitting an exact solution in the time domain. The
nonequilibrium dynamics, evaluated using an extension of dynamical mean-field
theory, show how the driven system differs from two common viewpoints - a
quasiequilibrium system at an elevated effective temperature (the "hot"
electron model) or a rapid interaction quench ("melting" of the Mott gap) - due
to the rearrangement of electronic states and redistribution of spectral
weight. The results demonstrate the inherent trade-off between energy and time
resolution accompanying the finite width probe pulses, characteristic of those
employed in pump-probe time-domain experiments, which can be used to focus
attention on different aspects of the dynamics near the transition.Comment: Original: 5 pages, 3 figures; Replaced: updated text and figures, 5
pages, 4 figure
Doping evolution of spin and charge excitations in the Hubbard model
To shed light on how electronic correlations vary across the phase diagram of
the cuprate superconductors, we examine the doping evolution of spin and charge
excitations in the single-band Hubbard model using determinant quantum Monte
Carlo (DQMC). In the single-particle response, we observe that the effects of
correlations weaken rapidly with doping, such that one may expect the random
phase approximation (RPA) to provide an adequate description of the
two-particle response. In contrast, when compared to RPA, we find that
significant residual correlations in the two-particle excitations persist up to
hole and electron doping (the range of dopings achieved in the
cuprates). These fundamental differences between the doping evolution of
single- and multi-particle renormalizations show that conclusions drawn from
single-particle processes cannot necessarily be applied to multi-particle
excitations. Eventually, the system smoothly transitions via a
momentum-dependent crossover into a weakly correlated metallic state where the
spin and charge excitation spectra exhibit similar behavior and where RPA
provides an adequate description.Comment: 5 pages, 4 figures, plus supplementary materia
Electronic structure theory of the hidden order material URuSi
We report a comprehensive electronic structure investigation of the
paramagnetic (PM), the large moment antiferromagnetic (LMAF), and the hidden
order (HO) phases of URuSi. We have performed relativistic
full-potential calculations on the basis of the density functional theory
(DFT), employing different exchange-correlation functionals to treat electron
correlations within the open -shell of uranium. Specifically, we
investigate---through a comparison between calculated and low-temperature
experimental properties---whether the electrons are localized or
delocalized in URuSi. We also performed dynamical mean field theory
calculations (LDA+DMFT) to investigate the temperature evolution of the
quasi-particle states at 100~K and above, unveiling a progressive opening of a
quasi-particle gap at the chemical potential when temperature is reduced. A
detailed comparison of calculated properties with known experimental data
demonstrates that the LSDA and GGA approaches, in which the uranium
electrons are treated as itinerant, provide an excellent explanation of the
available low-temperature experimental data of the PM and LMAF phases. We show
furthermore that due to a materials-specific Fermi surface instability a large,
but partial, Fermi surface gapping of up to 750 K occurs upon antiferromagnetic
symmetry breaking. The occurrence of the HO phase is explained through
dynamical symmetry breaking induced by a mode of long-lived antiferromagnetic
spin-fluctuations. This dynamical symmetry breaking model explains why the
Fermi surface gapping in the HO phase is similar but smaller than that in the
LMAF phase and it also explains why the HO and LMAF phases have the same Fermi
surfaces yet different order parameters. Suitable derived order parameters for
the HO are proposed to be the Fermi surface gap or the dynamic spin-spin
correlation function.Comment: 23 pages, 20 figure
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