308 research outputs found
More Evidence for a Distribution of Tunnel Splittings in Mn-acetate
In magnetic fields applied parallel to the anisotropy axis, the magnetization
of Mn has been measured in response to a field that is swept back and
forth across the resonances corresponding to steps . The fraction
of molecules remaining in the metastable well after each sweep through the
resonance is inconsistent with expectations for an ensemble of identical
molecules. The data are consistent instead with the presence of a broad
distribution of tunnel splittings. A very good fit is obtained for a Gaussian
distribution of the second-order anisotropy tunneling parameter . We show that dipolar shuffling is a negligible effect which cannot
explain our data.Comment: minor corrections (PACS nos, signs in Fig. 2
Black Carbon Contribution to the Aerosol Phase and its Scavenged Fraction in Mixed Phase Clouds at the High Alpine Site Jungfraujoch (3580m asl)
The mass fraction of black carbon (BC) in the atmospheric aerosol and its mixing state are important for the direct aerosol climate effect. These properties also determine if BC is incorporated into cloud hydrometeors (i.e. droplets and ice crystals) and are important because the microphysical and optical properties of the cloud are altered (indirect aerosol effect). Measurements were performed during several Cloud and Aerosol Characterization Experiments, in winter 2004 (CLACE3), summer 2004 (CLACE3.5), winter 2005 (CLACE4) and summer 2005 (CLACE4.5)
at the high Alpine research station Jungfraujoch (3580 m asl)
Experimental Upper Bound on Superradiance Emission from Mn12 Acetate
We used a Josephson junction as a radiation detector to look for evidence of
the emission of electromagnetic radiation during magnetization avalanches in a
crystal assembly of Mn_12-Acetate. The crystal assembly exhibits avalanches at
several magnetic fields in the temperature range from 1.8 to 2.6 K with
durations of the order of 1 ms. Although a recent study shows evidence of
electromagnetic radiation bursts during these avalanches [J. Tejada, et al.,
Appl. Phys. Lett. {\bf 84}, 2373 (2004)], we were unable to detect any
significant radiation at well-defined frequencies. A control experiment with
external radiation pulses allows us to determine that the energy released as
radiation during an avalanche is less than 1 part in 10^4 of the total energy
released. In addition, our avalanche data indicates that the magnetization
reversal process does not occur uniformly throughout the sample.Comment: 4 RevTeX pages, 3 eps figure
Exploring emotional prototypes in a high dimensional TTS latent space
Recent TTS systems are able to generate prosodically varied and realistic speech. However, it is unclear how this prosodic variation contributes to the perception of speakers’ emotional states. Here we use the recent psychological paradigm ‘Gibbs Sampling with People’ to search the prosodic latent space in a trained Global Style Token Tacotron model to explore prototypes of emotional prosody. Participants are recruited online and collectively manipulate the latent space of the generative speech model in a sequentially adaptive way so that the stimulus presented to one group of participants is determined by the response of the previous groups. We demonstrate that (1) particular regions of the model’s latent space are reliably associated with particular emotions, (2) the resulting emotional prototypes are well-recognized by a separate group of human raters, and (3) these emotional prototypes can be effectively transferred to new sentences. Collectively, these experiments demonstrate a novel approach to the understanding of emotional speech by providing a tool to explore the relation between the latent space of generative models and human semantics
Abrupt Transition between Thermally-Activated Relaxation and Quantum Tunneling in a Molecular Magnet
We report Hall sensor measurements of the magnetic relaxation of Mn
acetate as a function of magnetic field applied along the easy axis of
magnetization. Data taken at a series of closely-spaced temperatures between
0.24 K and 1.4 K provide strong new evidence for an abrupt ``first-order''
transition between thermally-assisted relaxation and magnetic decay via quantum
tunneling.Comment: 4 pages, including 7 figure
A Distribution of Tunnel Splittings in Mn-Acetate
In magnetic fields applied parallel to the anisotropy axis, the relaxation of
the magnetization of Mn measured for different sweep rates is shown to
collapse onto a single scaled curve. The form of the scaling implies that the
dominant symmetry-breaking process that gives rise to tunneling is a locally
varying second-order anisotropy, forbidden by tetragonal symmetry in the
perfect crystal, which gives rise to a broad distribution of tunnel splittings
in a real crystal of Mn-acetate. Different forms applied to even and
odd-numbered steps provide a distinction between even step resonances
(associated with crystal anisotropy) and odd resonances (which require a
transverse component of magnetic field).Comment: 4 pages, 5 figures. New title; text more clearly writte
Photon-Induced Magnetization Reversal in Single-Molecule Magnets
We use millimeter wave radiation to manipulate the populations of the energy
levels of a single crystal molecular magnet Fe8. When a continuous wave
radiation is in resonance with the transitions from the ground state to the
first excited state, the equilibrium magnetization exhibits a dip. The position
of this dip varies linearly with the radiation frequency. Our results provide a
lower bound of 0.17 ns for transverse relaxation time and suggest the
possibility that single-molecule magnets might be utilized for quantum
computation.Comment: 16 pages, 3 figure
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Temporal evolution of stable water isotopologues in cloud droplets in a hill cap cloud in central Europe (HCCT-2010)
In this work, we present the first study resolving the temporal evolution of δ2H and δ18O values in cloud droplets during 13 different cloud events. The cloud events were probed on a 937 m high mountain chain in Germany in the framework of the Hill Cap Cloud Thuringia 2010 campaign (HCCT-2010) in September and October 2010. The δ values of cloud droplets ranged from −77‰ to −15‰ (δ2H) and from −12.1‰ to −3.9‰ (δ18O) over the whole campaign. The cloud water line of the measured δ values was δ2H=7.8×δ18O+13×10−3, which is of similar slope, but with higher deuterium excess than other Central European Meteoric Water Lines. Decreasing δ values in the course of the campaign agree with seasonal trends observed in rain in central Europe. The deuterium excess was higher in clouds developing after recent precipitation revealing episodes of regional moisture recycling. The variations in δ values during one cloud event could either result from changes in meteorological conditions during condensation or from variations in the δ values of the water vapor feeding the cloud. To test which of both aspects dominated during the investigated cloud events, we modeled the variation in δ values in cloud water using a closed box model. We could show that the variation in δ values of two cloud events was mainly due to changes in local temperature conditions. For the other eleven cloud events, the variation was most likely caused by changes in the isotopic composition of the advected and entrained vapor. Frontal passages during two of the latter cloud events led to the strongest temporal changes in both δ2H (≈ 6‰ per hour) and δ18O (≈ 0.6‰ per hour). Moreover, a detailed trajectory analysis for the two longest cloud events revealed that variations in the entrained vapor were most likely related to rain out or changes in relative humidity and temperature at the moisture source region or both. This study illustrates the sensitivity of stable isotope composition of cloud water to changes in large scale air mass properties and regional recycling of moisture
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