Coherent Storage of Temporally Multimode Light Using a Spin-Wave Atomic Frequency Comb Memory

We report on coherent and multi-temporal mode storage of light using the full atomic frequency comb memory scheme. The scheme involves the transfer of optical atomic excitations in Pr3+:Y2SiO5 to spin-waves in the hyperfine levels using strong single-frequency transfer pulses. Using this scheme, a total of 5 temporal modes are stored and recalled on-demand from the memory. The coherence of the storage and retrieval is characterized using a time-bin interference measurement resulting in visibilities higher than 80%, independent of the storage time. This coherent and multimode spin-wave memory is promising as a quantum memory for light.Comment: 17 pages, 5 figure

A solid state spin-wave quantum memory for time-bin qubits

We demonstrate the first solid-state spin-wave optical quantum memory with on-demand read-out. Using the full atomic frequency comb scheme in a \PrYSO crystal, we store weak coherent pulses at the single-photon level with a signal to noise ratio $> 10$. Narrow-band spectral filtering based on spectral hole burning in a second \PrYSO crystal is used to filter out the excess noise created by control pulses to reach an unconditional noise level of $(2.0 \pm 0.3) \times10^{-3}$ photons per pulse. We also report spin-wave storage of photonic time-bin qubits with conditional fidelities higher than a measure and prepare strategy, demonstrating that the spin-wave memory operates in the quantum regime. This makes our device the first demonstration of a quantum memory for time-bin qubits, with on demand read-out of the stored quantum information. These results represent an important step for the use of solid-state quantum memories in scalable quantum networks.Comment: 10 pages, 10 figure

Storage of up-converted telecom photons in a doped crystal

We report on an experiment that demonstrates the frequency up-conversion of telecommunication wavelength single-photon-level pulses to be resonant with a $\mathrm{Pr}^{3+}$:$\mathrm{Y}_2\mathrm{Si}\mathrm{O}_5$ crystal. We convert the telecom photons at $1570\,\mathrm{nm}$ to $606\,\mathrm{nm}$ using a periodically-poled potassium titanyl phosphate nonlinear waveguide. The maximum device efficiency (which includes all optical loss) is inferred to be $\eta_{\mathrm{dev}}^{\mathrm{max}} = 22 \pm 1\,$ (internal efficiency $\eta_{\mathrm{int}} = 75\pm8\,$) with a signal to noise ratio exceeding 1 for single-photon-level pulses with durations of up to 560$\,$ns. The converted light is then stored in the crystal using the atomic frequency comb scheme with storage and retrieval efficiencies exceeding $\eta_{\mathrm{AFC}} = 20\,$ for predetermined storage times of up to $5\,\mu\mathrm{s}$. The retrieved light is time delayed from the noisy conversion process allowing us to measure a signal to noise ratio exceeding 100 with telecom single-photon-level inputs. These results represent the first demonstration of single-photon-level optical storage interfaced with frequency up-conversion

Frequency-Bin Entanglement of Ultra-Narrow Band Non-Degenerate Photon Pairs

We demonstrate frequency-bin entanglement between ultra-narrowband photons generated by cavity enhanced spontaneous parametric down conversion. Our source generates photon pairs in widely non-degenerate discrete frequency modes, with one photon resonant with a quantum memory material based on praseodymium doped crystals and the other photon at telecom wavelengths. Correlations between the frequency modes are analyzed using phase modulators and narrowband filters before detection. We show high-visibility two photon interference between the frequency modes, allowing us to infer a coherent superposition of the modes. We develop a model describing the state that we create and use it to estimate optimal measurements to achieve a violation of the Clauser-Horne (CH) Bell inequality under realistic assumptions. With these settings we perform a Bell test and show a significant violation of the CH inequality, thus proving the entanglement of the photons. Finally we demonstrate the compatibility with a quantum memory material by using a spectral hole in the praseodymium (Pr) doped crystal as spectral filter for measuring high-visibility two-photon interference. This demonstrates the feasibility of combining frequency-bin entangled photon pairs with Pr-based solid state quantum memories.Comment: 15 pages, 6 figure

A spectral hole memory for light at the single photon level

We demonstrate a solid state spin-wave optical memory based on stopped light in a spectral hole. A long lived narrow spectral hole is created by optical pumping in the inhomogeneous absorption profile of a Pr$^{3+}$:Y$_2$SiO$_5$ crystal. Optical pulses sent through the spectral hole experience a strong reduction of their group velocity and are spatially compressed in the crystal. A short Raman pulse transfers the optical excitation to the spin state before the light pulse exits the crystal, effectively stopping the light. After a controllable delay, a second Raman pulse is sent, which leads to the emission of the stored photons. We reach storage and retrieval efficiencies for bright pulses of up to $39\,\%$ in a $5 \,\mathrm{mm}$-long crystal. We also show that our device works at the single photon level by storing and retrieving $3\,\mathrm{\mu s}$-long weak coherent pulses with efficiencies up to $31\,\%$, demonstrating the most efficient spin-wave solid state optical memory at the single-photon level so far. We reach an unconditional noise level of $(9\pm1)\times 10^{-3}$ photons per pulse in a detection window of $4\,\mathrm{\mu s}$ leading to a signal-to-noise ratio of $33 \pm 4$ for an average input photon number of 1, making our device promising for long-lived storage of non-classical light.Comment: 5 pages, 4 figure

High resolution spectroscopy to investigate impurities in YAB single crystals

The work explores the feasibility of high resolution (as fine as 0.02 cm-1) Fourier transform spectroscopy applied at 9 K in the 500-25000 cm-1 range to detect traces of unwanted impurities, mainly rare earths (RE3+) in crystals: the system chosen is YAl3(BO3)4 (YAB). Weak traces of RE3+ (Nd, Dy, Er, Tm, Yb), but also of Cr3+ and OH-, were successfully monitored by comparing the spectra of YAB samples under examination with those intentionally doped with a given ion. The analysis performed on a variety of samples shows how Cr3+, Nd3+, and Yb3+ are the most frequent unwanted dopants and can provide suggestions to the crystal growers about the performances of different crystal growth lines. According to a preliminary evaluation, the Er3+ traces detection limit is as low as 1-2x10-4 mol% in 1 cm thick samples. The advantages of the method, which is sample non-destructive, are discussed in comparison with those currently applied

Entanglement between a telecom photon and an on-demand multimode solid-state quantum memory

Entanglement between photons at telecommunication wavelengths and long-lived quantum memories is one of the fundamental requirements of long-distance quantum communication. Quantum memories featuring on-demand read-out and multimode operation are additional precious assets that will benefit the communication rate. In this work we report the first demonstration of entanglement between a telecom photon and a collective spin excitation in a multimode solid-state quantum memory. Photon pairs are generated through widely non-degenerate parametric down-conversion, featuring energy-time entanglement between the telecom-wavelength idler and a visible signal photon. The latter is stored in a Pr$^{3+}$:Y$_2$SiO$_5$ crystal as a spin wave using the full Atomic Frequency Comb scheme. We then recall the stored signal photon and analyze the entanglement using the Franson scheme. We measure conditional fidelities of $92(2)\%$ for excited-state storage, enough to violate a CHSH inequality, and $77(2)\%$ for spin-wave storage. Taking advantage of the on-demand read-out from the spin state, we extend the entanglement storage in the quantum memory for up to 47.7~$\mu$s, which could allow for the distribution of entanglement between quantum nodes separated by distances of up to 10 km

Quantum storage of heralded single photons in a praseodymium-doped crystal

We report on experiments demonstrating the reversible mapping of heralded single photons to long-lived collective optical atomic excitations stored in a Pr3+:Y2SiO5 crystal. A cavity-enhanced spontaneous down-conversion source is employed to produce widely nondegenerate narrow-band (≈2 MHz) photon pairs. The idler photons, whose frequency is compatible with telecommunication optical fibers, are used to herald the creation of the signal photons, compatible with the Pr3þ transition. The signal photons are stored and retrieved using the atomic frequency comb protocol. We demonstrate storage times up to 4.5 μs while preserving nonclassical correlations between the heralding and the retrieved photon. This is more than 20 times longer than in previous realizations in solid state devices, and implemented in a system ideally suited for the extension to spin-wave storage

Photonic quantum state transfer between a cold atomic gas and a crystal

Interfacing fundamentally different quantum systems is key to build future hybrid quantum networks. Such heterogeneous networks offer superior capabilities compared to their homogeneous counterparts as they merge individual advantages of disparate quantum nodes in a single network architecture. However, only very few investigations on optical hybrid-interconnections have been carried out due to the high fundamental and technological challenges, which involve e.g. wavelength and bandwidth matching of the interfacing photons. Here we report the first optical quantum interconnection between two disparate matter quantum systems with photon storage capabilities. We show that a quantum state can be faithfully transferred between a cold atomic ensemble and a rare-earth doped crystal via a single photon at telecommunication wavelength, using cascaded quantum frequency conversion. We first demonstrate that quantum correlations between a photon and a single collective spin excitation in the cold atomic ensemble can be transferred onto the solid-state system. We also show that single-photon time-bin qubits generated in the cold atomic ensemble can be converted, stored and retrieved from the crystal with a conditional qubit fidelity of more than $85\%$. Our results open prospects to optically connect quantum nodes with different capabilities and represent an important step towards the realization of large-scale hybrid quantum networks