13 research outputs found
Maximizing precision in saturation-limited absorption measurements
Quantum fluctuations in the intensity of an optical probe is noise which
limits measurement precision in absorption spectroscopy. Increased probe power
can offer greater precision, however, this strategy is often constrained by
sample saturation. Here, we analyse measurement precision for a generalised
absorption model in which we account for saturation and explore its effect on
both classical and quantum probe performance. We present a classical
probe-sample optimisation strategy to maximise precision and find that optimal
probe powers always fall within the saturation regime. We apply our
optimisation strategy to two examples, high-precision Doppler broadened
thermometry and an absorption spectroscopy measurement of Chlorophyll A. We
derive a limit on the maximum precision gained from using a non-classical probe
and find a strategy capable of saturating this bound. We evaluate
amplitude-squeezed light as a viable experimental probe state and find it
capable of providing precision that reaches to within > 85% of the ultimate
quantum limit with currently available technology.Comment: 12 pages and 5 figure
Demonstrating an absolute quantum advantage in direct absorption measurement
Engineering apparatus that harness quantum theory promises to offer practical advantages over current technology. A fundamentally more powerful prospect is that such quantum technologies could out-perform any future iteration of their classical counterparts, no matter how well the attributes of those classical strategies can be improved. Here, for optical direct absorption measurement, we experimentally demonstrate such an instance of an absolute advantage per photon probe that is exposed to the absorbative sample. We use correlated intensity measurements of spontaneous parametric downconversion using a commercially available air-cooled CCD, a new estimator for data analysis and a high heralding efficiency photon-pair source. We show this enables improvement in the precision of measurement, per photon probe, beyond what is achievable with an ideal coherent state (a perfect laser) detected with 100% efficient and noiseless detection. We see this absolute improvement for up to 50% absorption, with a maximum observed factor of improvement of 1.46. This equates to around 32% reduction in the total number of photons traversing an optical sample, compared to any future direct optical absorption measurement using classical light
Designing quantum experiments with a genetic algorithm
We introduce a genetic algorithm that designs quantum optics experiments for engineering quantum states with specific properties. Our algorithm is powerful and flexible, and can easily be modified to find methods of engineering states for a range of applications. Here we focus on quantum metrology. First, we consider the noise-free case, and use the algorithm to find quantum states with a large quantum Fisher information (QFI). We find methods, which only involve experimental elements that are available with current or near-future technology, for engineering quantum states with up to a 100 fold improvement over the best classical state, and a 20 fold improvement over the optimal Gaussian state. Such states are a superposition of the vacuum with a large number of photons (around 80), and can hence be seen as Schrödinger-cat-like states. We then apply the two most dominant noise sources in our setting—photon loss and imperfect heralding—and use the algorithm to find quantum states that still improve over the optimal Gaussian state with realistic levels of noise. This will open up experimental and technological work in using exotic non-Gaussian states for quantum-enhanced phase measurements. Finally, we use the Bayesian mean square error to look beyond the regime of validity of the QFI, finding quantum states with precision enhancements over the alternatives even when the experiment operates in the regime of limited data
Widely-tunable mid-infrared ring cavity pump-enhanced OPO and application in photo-thermal interferometric trace ethane detection
Funding: Innovate UK (133076); Engineering and Physical Sciences Research Council (EP//L01596X/1, EP/M01326X/1, EP/M024385/1); European Research Council (ERC-2018-STG 803665).The development of a broadly and accurately tunable single-frequency mid-infrared laser source and its application to a sensitive laser absorption detection method are described. Photo-thermal interferometric spectroscopy is employed as a phase-sensitive method to detect the minute refractive index change caused by the heating of a gas under laser radiation. A separate probe beam allows for the spectrally-interesting mid-infrared region to be examined whilst utilizing low cost, high detectivity photodetectors in the visible/near-infrared region. We also describe the implementation of a Sagnac interferometer to minimize the effects of environmental perturbation and provide inherent passive stability. A continuous-wave ring-cavity pump-enhanced OPO has been developed to provide excitation light from 3–4 µm at 140 mW with the ability to mode-hop tune continuously over 90 cm−1 in 0.07 cm−1 steps. Complementary use of both detection apparatus and excitation source has allowed for presence of ethane to be detected down to 200 parts per billion.developed to provide excitation light from 3–4 µm at 140 mW with the ability to mode-hop tune continuously over 90 cm−1 in 0.07 cm−1 steps. Complementary use of both detection apparatus and excitation source has allowed for presence of ethane to be detected down to 200 parts per billion.Publisher PDFPeer reviewe
Generation of random numbers by measuring phase fluctuations from a laser diode with a silicon-on-insulator chip
Multimode interferometry for entangling atoms in quantum networks
© 2019 IOP Publishing Ltd. We bring together a cavity-enhanced light-matter interface with a multimode interferometer (MMI) integrated onto a photonic chip and demonstrate the potential of such hybrid systems to tailor distributed entanglement in a quantum network. The MMI is operated with pairs of narrowband photons produced a priori deterministically from a single 87Rb atom strongly coupled to a high-finesse optical cavity. Non-classical coincidences between photon detection events show no loss of coherence when interfering pairs of these photons through the MMI in comparison to the two-photon visibility directly measured using Hong-Ou-Mandel interference on a beam splitter. This demonstrates the ability of integrated multimode circuits to mediate the entanglement of remote stationary nodes in a quantum network interlinked by photonic qubits