Instantaneous coherent destruction of tunneling and fast quantum state preparation for strongly pulsed spin qubits in diamond

Qubits driven by resonant strong pulses are studied and a parameter regime is explored in which the dynamics can be solved in closed form. Instantaneous coherent destruction of tunneling can be seen for longer pulses, whereas shorter pulses allow a fast preparation of the qubit state. Results are compared with recent experiments of pulsed nitrogen-vacancy center spin qubits in diamond.Comment: 9 pages, 4 figures. Published in the special issue of Chemical Physics in honor of Peter Hangg

Foerster resonance energy transfer rate and local density of optical states are uncorrelated in any dielectric nanophotonic medium

Motivated by the ongoing debate about nanophotonic control of Foerster resonance energy transfer (FRET), notably by the local density of optical states (LDOS), we study an analytic model system wherein a pair of ideal dipole emitters - donor and acceptor - exhibit energy transfer in the vicinity of an ideal mirror. The FRET rate is controlled by the mirror up to distances comparable to the donor-acceptor distance, that is, the few-nanometer range. For vanishing distance, we find a complete inhibition or a four-fold enhancement, depending on dipole orientation. For mirror distances on the wavelength scale, where the well-known `Drexhage' modification of the spontaneous-emission rate occurs, the FRET rate is constant. Hence there is no correlation between the Foerster (or total) energy transfer rate and the LDOS. At any distance to the mirror, the total energy transfer between a closely-spaced donor and acceptor is dominated by Foerster transfer, i.e., by the static dipole-dipole interaction that yields the characteristic inverse-sixth-power donor-acceptor distance dependence in homogeneous media. Generalizing to arbitrary inhomogeneous media with weak dispersion and weak absorption in the frequency overlap range of donor and acceptor, we derive two main theoretical results. Firstly, the spatially dependent Foerster energy transfer rate does not depend on frequency, hence not on the LDOS. Secondly the FRET rate is expressed as a frequency integral of the imaginary part of the Green function. This leads to an approximate FRET rate in terms of the LDOS integrated over a huge bandwidth from zero frequency to about 10 times the donor emission frequency, corresponding to the vacuum-ultraviolet. Even then, the broadband LDOS hardly contributes to the energy transfer rates. We discuss practical consequences including quantum information processing.Comment: 17 pages, 9 figure

Entanglement creation in circuit QED via Landau-Zener sweeps

A qubit may undergo Landau-Zener transitions due to its coupling to one or several quantum harmonic oscillators. We show that for a qubit coupled to one oscillator, Landau-Zener transitions can be used for single-photon generation and for the controllable creation of qubit-oscillator entanglement, with state-of-the-art circuit QED as a promising realization. Moreover, for a qubit coupled to two cavities, we show that Landau-Zener sweeps of the qubit are well suited for the robust creation of entangled cavity states, in particular symmetric Bell states, with the qubit acting as the entanglement mediator. At the heart of our proposals lies the calculation of the exact Landau-Zener transition probability for the qubit, by summing all orders of the corresponding series in time-dependent perturbation theory. This transition probability emerges to be independent of the oscillator frequencies, both inside and outside the regime where a rotating-wave approximation is valid.Comment: 12 pages, 7 figure

How nonlocal damping reduces plasmon-enhanced fluorescence in ultranarrow gaps

The nonclassical modification of plasmon-assisted fluorescence enhancement is theoretically explored by placing two-level dipole emitters at the narrow gaps encountered in canonical plasmonic architectures, namely dimers and trimers of different metallic nanoparticles. Through detailed simulations, in comparison with appropriate analytical modelling, it is shown that within classical electrodynamics, and for the reduced separations explored here, fluorescence enhancement factors of the order of $10^{5}$ can be achieved, with a divergent behaviour as the particle touching regime is approached. This remarkable prediction is mainly governed by the dramatic increase in excitation rate triggered by the corresponding field enhancement inside the gaps. Nevertheless, once nonclassical corrections are included, the amplification factors decrease by up to two orders of magnitude and a saturation regime for narrower gaps is reached. These nonclassical limitations are demonstrated by simulations based on the generalised nonlocal optical response theory, which accounts in an efficient way not only for nonlocal screening, but also for the enhanced Landau damping near the metal surface. A simple strategy to introduce nonlocal corrections to the analytic solutions is also proposed. It is therefore shown that the nonlocal optical response of the metal imposes more realistic, finite upper bounds to the enhancement feasible with ultrasmall plasmonic cavities, thus providing a theoretical description closer to state of the art experiments

Robustness of the Rabi splitting under nonlocal corrections in plexcitonics

We explore theoretically how nonlocal corrections in the description of the metal affect the strong coupling between excitons and plasmons in typical examples where nonlocal effects are anticipated to be strong, namely small metallic nanoparticles, thin metallic nanoshells or dimers with narrow separations, either coated with or encapsulating an excitonic layer. Through detailed simulations based on the generalised nonlocal optical response theory, which simultaneously accounts both for modal shifts due to screening and for surface-enhanced Landau damping, we show that, contrary to expectations, the influence of nonlocality is rather limited, as in most occasions the width of the Rabi splitting remains largely unaffected and the two hybrid modes are well distinguishable. We discuss how this behaviour can be understood in view of the popular coupled-harmonic-oscillator model, while we also provide analytic solutions based on Mie theory to describe the hybrid modes in the case of matryoshka-like single nanoparticles. Our analysis provides an answer to a so far open question, that of the influence of nonlocality on strong coupling, and is expected to facilitate the design and study of plexcitonic architectures with ultrafine geometrical details

Incomplete pure dephasing of N-qubit entangled W states

We consider qubits in a linear arrangement coupled to a bosonic field which acts as a quantum heat bath and causes decoherence. By taking the spatial separation of the qubits explicitly into account, the reduced qubit dynamics acquires an additional non-Markovian element. We investigate the time evolution of an entangled many-qubit W state, which for vanishing qubit separation remains robust under pure dephasing. For finite separation, by contrast, the dynamics is no longer decoherence-free. On the other hand, spatial noise correlations may prevent a complete dephasing. While a standard Bloch-Redfield master equation fails to describe this behavior even qualitatively, we propose instead a widely applicable causal master equation. Here we employ it to identify and characterize decoherence-poor subspaces. Consequences for quantum error correction are discussed.Comment: 14 pages, 6 figures, revised version, to appear in Phys. Rev.

Two-fluid hydrodynamic model for semiconductors

The hydrodynamic Drude model (HDM) has been successful in describing the optical properties of metallic nanostructures, but for semiconductors where several different kinds of charge carriers are present, an extended theory is required. We present a two-fluid hydrodynamic model for semiconductors containing electrons and holes (from thermal or external excitation) or light and heavy holes (in $p$-doped materials). The two-fluid model predicts the existence of two longitudinal modes, an acoustic and an optical, whereas only an optical mode is present in the HDM. By extending nonlocal Mie theory to two plasmas, we are able to simulate the optical properties of two-fluid nanospheres and predict that the acoustic mode gives rise to peaks in the extinction spectra that are absent in the HDM.Comment: Accepted in PRB. 17 pages, 9 figures, 1 tabl

Qubit coherence decay down to threshold: influence of substrate dimensions

Keeping single-qubit quantum coherence above some threshold value not far below unity is a prerequisite for fault-tolerant quantum error correction (QEC). We study the initial dephasing of solid-state qubits in the independent-boson model, which describes well recent experiments on quantum dot (QD) excitons both in bulk and in substrates of reduced geometry such as nanotubes. Using explicit expressions for the exact coherence dynamics, a minimal QEC rate is identified in terms of the error threshold, temperature, and qubit-environment coupling strength. This allows us to systematically study the benefit of a current trend towards substrates with reduced dimensions.Comment: 4 pages, 4 figure