7,556 research outputs found
Thermal Conductivity and Specific Heat of the Spin-Ice Compound DyTiO: Experimental Evidence for Monopole Heat Transport
Elementary excitations in the spin-ice compound DyTiO can be
described as magnetic monopoles propagating independently within the pyrochlore
lattice formed by magnetic Dy ions. We studied the magnetic-field dependence of
the thermal conductivity {\kappa}(B) for B || [001] and observe clear evidence
for magnetic heat transport originating from the monopole excitations. The
magnetic contribution {\kappa}_{mag} is strongly field-dependent and correlates
with the magnetization M(B). The diffusion coefficient obtained from the ratio
of {\kappa}_{mag} and the magnetic specific heat is strongly enhanced below 1 K
indicating a high mobility of the monopole excitations in the spin-ice state.Comment: 5 pages, 4 figure
Theoretical study of electronic damage in single particle imaging experiments at XFELs for pulse durations 0.1 - 10 fs
X-ray free-electron lasers (XFELs) may allow to employ the single particle
imaging (SPI) method to determine the structure of macromolecules that do not
form stable crystals. Ultrashort pulses of 10 fs and less allow to outrun
complete disintegration by Coulomb explosion and minimize radiation damage due
to nuclear motion, but electronic damage is still present. The major
contribution to the electronic damage comes from the plasma generated in the
sample that is strongly dependent on the amount of Auger ionization. Since the
Auger process has a characteristic time scale on the order of femtoseconds, one
may expect that its contribution will be significantly reduced for attosecond
pulses. Here, we study the effect of electronic damage on the SPI at pulse
durations from 0.1 fs to 10 fs and in a large range of XFEL fluences to
determine optimal conditions for imaging of biological samples. We analyzed the
contribution of different electronic excitation processes and found that at
fluences higher than - photons/m (depending on the
photon energy and pulse duration) the diffracted signal saturates and does not
increase further. A significant gain in the signal is obtained by reducing the
pulse duration from 10 fs to 1 fs. Pulses below 1 fs duration do not give a
significant gain in the scattering signal in comparison with 1 fs pulses. We
also study the limits imposed on SPI by Compton scattering.Comment: 35 pages, 9 figures, 1 table, 2 appendixes, 45 reference
Substitution effects on the temperature vs. magnetic-field phase diagrams of the quasi-1D effective Ising spin-1/2 chain system BaCoVO
BaCoVO is a one-dimensional antiferromagnetic spin-1/2 chain
system with pronounced Ising anisotropy of the magnetic exchange. Due to finite
interchain interactions long-range antiferromagnetic order develops below
K, which is accompanied by a structural distortion in
order to lift magnetic frustration effects. The corresponding temperature magnetic-field phase diagram is highly anisotropic with respect to the
magnetic-field direction and various details are still under vivid discussion.
Here, we report the influence of several substitutions on the magnetic
properties and the phase diagrams of BaCoVO. We investigate the
substitution series
BaSrCoVO
over the full range as well as the influence of a partial
substitution of the magnetic Co by small amounts of other magnetic
transition metals or by non-magnetic magnesium. In all cases, the phase
diagrams were obtained on single crystals from magnetization data and/or
high-resolution studies of the thermal expansion and magnetostriction.Comment: 10 pages, 10 figure
Magnetostrictive Neel ordering of the spin-5/2 ladder compound BaMn2O3: distortion-induced lifting of geometrical frustration
The crystal structure and the magnetism of BaMnO have been studied by
thermodynamic and by diffraction techniques using large single crystals and
powders. BaMnO is a realization of a spin ladder as the
magnetic interaction is dominant along 180 Mn-O-Mn bonds forming the
legs and the rungs of a ladder. The temperature dependence of the magnetic
susceptibility exhibits well-defined maxima for all directions proving the
low-dimensional magnetic character in BaMnO. The susceptibility and
powder neutron diffraction data, however, show that BaMnO exhibits a
transition to antiferromagnetic order at 184 K, in spite of a full frustration
of the nearest-neighbor inter-ladder coupling in the orthorhombic
high-temperature phase. This frustration is lifted by a remarkably strong
monoclinic distortion which accompanies the magnetic transition.Comment: 9 pages, 8 figures, 2 tables; in V1 fig. 2 was included twice and
fig. 4 was missing; this has been corrected in V
Evidence for Multiple Phase Transitions in La_1-xCa_xCoO_3
We report thermal-expansion and specific-heat data of the series
La_1-xCa_xCoO_3 for 0 <= x <= 0.3. For x = 0 the thermal-expansion coefficient
alpha(T) features a pronounced maximum around T = 50 K caused by a
temperature-dependent spin-state transition from a low-spin state (S=0) at low
temperatures towards a higher spin state of the Co^3+ ions. The partial
substitution of the La^3+ ions by divalent Ca^2+ ions causes drastic changes in
the macroscopic properties of LaCoO_3. Around x ~ 0.125 the large maximum in
alpha(T) has completely vanished. With further increasing x three different
anomalies develop
Low-temperature ordered phases of the spin- XXZ chain system CsCoCl
In this study the magnetic order of the spin-1/2 XXZ chain system
CsCoCl in a temperature range from 50 mK to 0.5 K and in applied
magnetic fields up to 3.5 T is investigated by high-resolution measurements of
the thermal expansion and the specific heat. Applying magnetic fields along a
or c suppresses completely at about 2.1 T. In addition, we find
an adjacent intermediate phase before the magnetization saturates close to 2.5
T. For magnetic fields applied along b, a surprisingly rich phase diagram
arises. Two additional transitions are observed at critical fields T and T, which we propose to
arise from a two-stage spin-flop transition.Comment: 10 pages, 10 figure
Resonant Auger decay of the core-excited CO molecule in intense X-ray laser fields
The dynamics of the resonant Auger (RA) process of the core-excited
CO(1s) molecule in an intense X-ray laser field is
studied theoretically. The theoretical approach includes the analogue of the
conical intersections of the complex potential energy surfaces of the ground
and `dressed' resonant states due to intense X-ray pulses, taking into account
the decay of the resonance and the direct photoionization of the ground state,
both populating the same final ionic states coherently, as well as the direct
photoionization of the resonance state itself. The light-induced non-adiabatic
effect of the analogue of the conical intersections of the resulting complex
potential energy surfaces gives rise to strong coupling between the electronic,
vibrational and rotational degrees of freedom of the diatomic CO molecule. The
interplay of the direct photoionization of the ground state and of the decay of
the resonance increases dramatically with the field intensity. The coherent
population of a final ionic state via both the direct photoionization and the
resonant Auger decay channels induces strong interference effects with distinct
patterns in the RA electron spectra. The individual impact of these physical
processes on the total electron yield and on the CO electron
spectrum are demonstrated.Comment: 13 figs, 1 tabe
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