121 research outputs found
High sensitive quasi freestanding epitaxial graphene gassensor on 6H-SiC
We have measured the electrical response to NO, N, NH and CO for
epitaxial graphene and quasi freestanding epitaxial graphene on 6H-SiC
substrates. Quasi freestanding epitaxial graphene shows a 6 fold increase in
NO2 sensitivity compared to epitaxial graphene. Both samples show a sensitivity
better than the experimentally limited 1 ppb. The strong increase in
sensitivity of quasi freestanding epitaxial graphene can be explained by a
Fermi-energy close to the Dirac Point leading to a strongly surface doping
dependent sample resistance. Both sensors show a negligible sensitivity to
N, NH and CO
Comparison of the magneto-Peltier and magneto-Seebeck effects in magnetic tunnel junctions
Understanding heat generation and transport processes in a magnetic tunnel
junction (MTJ) is a significant step towards improving its application in
current memory devices. Recent work has experimentally demonstrated the
magneto-Seebeck effect in MTJs, where the Seebeck coefficient of the junction
varies as the magnetic configuration changes from a parallel (P) to an
anti-parallel (AP) configuration. Here we report the study on its
as-yet-unexplored reciprocal effect, the magneto-Peltier effect, where the heat
flow carried by the tunneling electrons is altered by changing the magnetic
configuration of the MTJ. The magneto-Peltier signal that reflects the change
in the temperature difference across the junction between the P and AP
configurations scales linearly with the applied current in the small bias but
is greatly enhanced in the large bias regime, due to higher-order Joule heating
mechanisms. By carefully extracting the linear response which reflects the
magneto-Peltier effect, and comparing it with the magneto-Seebeck measurements
performed on the same device, we observe results consistent with Onsager
reciprocity. We estimate a magneto-Peltier coefficient of 13.4 mV in the linear
regime using a three-dimensional thermoelectric model. Our result opens up the
possibility of programmable thermoelectric devices based on the Peltier effect
in MTJs
Atomic Force Microscopy Study of an Ideally Hard Contact: The Diamond(111)/Tungsten Carbide Interface
A comprehensive nanotribological study of a hydrogen-terminated diamond(111)/tungsten carbide interface has been performed using ultrahigh vacuum atomic force microscopy. Both contact conductance, which is proportional to contact area, and friction have been measured as a function of applied load. We demonstrate for the first time that the load dependence of the contact area in UHV for this extremely hard single asperity contact is described by the Derjaguin-MĂĽller-Toporov continuum mechanics model. Furthermore, the frictional force is found to be directly proportional to the contact area
Existence and role of low energy charge-paramagnon modes in the strange metal phase of BiSrCaCuO
The strange metal phase is characteristic for the -linear dc resistivity behaviour over a large -range. The effect of the strength of the charge-paramagnon interactions on the charge fluctuations in optimally doped and underdoped regions of BiSrCaCuO (Bi-2212) may shine light on the anomalous behaviour of the optical conductivity response in the energy range 50 - 500 meV. We present a preliminary analysis of a single initial run of electron energy loss spectroscopy (EELS) measurements done in a scanning transmission electron microscope (STEM) which exhibit linear dispersive modes separated by 50 meV energy gaps up to 250 meV in optimally doped Bi-2212. Our observations show similarities with the fluctuating stripes as predicted by Zaanen
Diamond deposition on modified silicon substrates: Making diamond atomic force microscopy tips for nanofriction experiments
Fine-crystalline diamond particles are grown on standard Si atomic force microscopy tips, using hot filament-assisted chemical vapor deposition. To optimize the conditions for diamond deposition, first a series of experiments is carried out using silicon substrates covered by point-topped pyramids as obtained by wet chemical etching. The apexes and the edges of the silicon pyramids provide favorable sites for diamond nucleation and growth. The investigation of the deposited polycrystallites is done by means of optical microscopy, scanning electron microscopy and micro-Raman spectroscopy. The resulting diamond-terminated tips are tested in ultra high vacuum using contact-mode atomic force microscope on a stepped surface of sapphire showing high stability, sharpness, and hardnes
Ordered vacancy network induced by the growth of epitaxial graphene on Pt(111)
We have studied large areas of (v3×v3)R30° graphene commensurate with a Pt(111) substrate. A combination of experimental techniques with ab initio density functional theory indicates that this structure is related to a reconstruction at the Pt surface, consisting of an ordered vacancy network formed in the outermost Pt layer and a graphene layer covalently bound to the Pt substrate. The formation of this reconstruction is enhanced if low temperatures and polycyclic aromatic hydrocarbons are used as molecular precursors for epitaxial growth of the graphene layers
Room-temperature ferromagnetism in graphite driven by 2D networks of point defects
Ferromagnetism in carbon-based materials is appealing for both applications
and fundamental science purposes because carbon is a light and bio-compatible
material that contains only s and p electrons in contrast to traditional
ferromagnets based on 3d or 4f electrons. Here we demonstrate direct evidence
for ferromagnetic order locally at defect structures in highly oriented
pyrolytic graphite (HOPG) with magnetic force microscopy and in bulk
magnetization measurements at room temperature. Magnetic impurities have been
excluded as the origin of the magnetic signal after careful analysis supporting
an intrinsic magnetic behavior of carbon. The observed ferromagnetism has been
attributed to originate from unpaired electron spins localized at grain
boundaries of HOPG. Grain boundaries form two-dimensional arrays of point
defects, where their spacing depends on the mutual orientation of two grains.
Depending on the distance between these point defects, scanning tunneling
spectroscopy of grain boundaries showed two intense split localized states for
small distances between defects (< 4 nm) and one localized state at the Fermi
level for large distances between defects (> 4 nm).Comment: 19 pages, 5 figure
Development of a Near-Field Magneto-Optical Microscopy for Studying Ultrafast Magnetization Dynamics
Polymer waveguides with optimized overlap integral for modal dispersion phase-matching
Modal dispersion phase-matched second harmonic generation is demonstrated in new poled polymer waveguide geometries with a nonlinear optical core consisting of two side-chain polymers with different glass transition temperatures. After poling above and between the respective glass transitions, the sign of the nonlinear optical coefficient is reversed in the two polymers, thereby improving the overlap integral. Conversion efficiencies up to 7%/W cm(2) were achieved in the first experiments
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