319 research outputs found

    Spatial Correlation of Conduction Electrons in Metal with Complicated Geometry Of The Fermi Surface

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    The "density-density" correlation function of conduction electrons in metal is investigated. It is shown, that the asymptotic behaviour of the CF depends on the shape and the local geometry of the Fermi surface. In particular, the exponent of power law which describes the damping of Friedel oscillations at large r (-4 for an isotropic Fermi gas) is determined by local geometry of the FS. The applications of the obtained results to calculations of the CF in a metal near the electron topological transition and of the RKKY exchange integral are considered as well.Comment: 12 pages, LaTeX, 5 figures upon request (to appear in J.Phys.:CM, 1993

    Electron relaxation in metals: Theory and exact analytical solutions

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    The non-equilibrium dynamics of electrons is of a great experimental and theoretical value providing important microscopic parameters of the Coulomb and electron-phonon interactions in metals and other cold plasmas. Because of the mathematical complexity of collision integrals theories of electron relaxation often rely on the assumption that electrons are in a "quasi-equilibrium" (QE) with a time-dependent temperature, or on the numerical integration of the time-dependent Boltzmann equation. We transform the integral Boltzmann equation to a partial differential Schroedinger-like equation with imaginary time in a one-dimensional "coordinate" space reciprocal to energy which allows for exact analytical solutions in both cases of electron-electron and electron-phonon relaxation. The exact relaxation rates are compared with the QE relaxation rates at high and low temperatures.Comment: Citation list has been extended. The paper is submitted to the Physical Review

    Quantum Oscillations of Elastic Moduli and Softening of Phonon Modes in Metals

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    In this paper we present a theoretical analysis of the effect of magnetostriction on quantum oscillations of elastic constants in metals under strong magnetic fields. It is shown that at low temperatures a significant softening of some acoustic modes could occur near peaks of quantum oscillations of the electron density of states (DOS) at the Fermi surface (FS). This effect is caused by a magnetic instability of a special kind, and it can give rise to a lattice instability. We also show that the most favorable conditions for this instability to be revealed occur in metals whose Fermi surfaces include nearly cylindrical segments.Comment: 5 pages, 1 figur

    Electron-Phonon Coupling in High-Temperature Cuprate Superconductors Determined from Electron Relaxation Rates

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    We determined electronic relaxation times via pump-probe optical spectroscopy using sub-15 fs pulses for the normal state of two different cuprate superconductors.We show that the primary relaxation process is the electron-phonon interaction and extract a measure of its strength, the second moment of the Eliashberg function\lambda=800\pm200 meV^{2} for La_{1.85}Sr_{0.15}CuO_{4} and \lambda=400\pm100 meV^{2} for YBa_{2}Cu_{3}O_{6.5}. These values suggest a possible fundamental role of the electron-phonon interaction in the superconducting pairing mechanism.Comment: As published in PR

    Smearing of phase transition due to a surface effect or a bulk inhomogeneity in ferroelectric nanostructures

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    The boundary conditions, customarily used in the Landau-type approach to ferroelectric thin films and nanostructures, have to be modified to take into account that a surface of a ferroelectric (FE) is a defect of the ``field'' type. The surface (interface) field is coupled to a normal component of polarization and, as a result, the second order phase transitions are generally suppressed and anomalies in response are washed out. In FE films with a compositional (grading) or some other type of inhomogeneity, the transition into a monodomain state is suppressed, but a transition with formation of a domain structure may occur.Comment: 5 pages, 1 figure; the effective bias field is very large, the estimate is adde

    Entropy Driven Atomic Motion in Laser-Excited Bismuth

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    We introduce a thermodynamical model based on the two-temperature approach in order to fully understand the dynamics of the coherent A(1g) phonon in laser-excited bismuth. Using this model, we simulate the time evolution of (111) Bragg peak intensities measured by Fritz et al. [Science 315, 633 (2007)] in femtosecond x-ray diffraction experiments performed on a bismuth film for different laser fluences. The agreement between theoretical and experimental results is striking not only because we use fluences very close to the experimental ones but also because most of the model parameters are obtained from ab initio calculations performed for different electron temperatures

    The Origin of Anomalous Low-Temperature Downturns in the Thermal Conductivity of Cuprates

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    We show that the anomalous decrease in the thermal conductivity of cuprates below 300 mK, as has been observed recently in several cuprate materials including Pr2−x_{2-x}Cex_xCuO7−δ_{7-\delta} in the field-induced normal state, is due to the thermal decoupling of phonons and electrons in the sample. Upon lowering the temperature, the phonon-electron heat transfer rate decreases and, as a result, a heat current bottleneck develops between the phonons, which can in some cases be primarily responsible for heating the sample, and the electrons. The contribution that the electrons make to the total low-TT heat current is thus limited by the phonon-electron heat transfer rate, and falls rapidly with decreasing temperature, resulting in the apparent low-TT downturn of the thermal conductivity. We obtain the temperature and magnetic field dependence of the low-TT thermal conductivity in the presence of phonon-electron thermal decoupling and find good agreement with the data in both the normal and superconducting states.Comment: 8 pages, 5 figure

    Ab-initio calculation of all-optical time-resolved calorimetry of nanosized systems: Evidence of nanosecond-decoupling of electron and phonon temperatures

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    The thermal dynamics induced by ultrashort laser pulses in nanoscale systems, i.e. all-optical time-resolved nanocalorimetry is theoretically investigated from 300 to 1.5 K. We report ab-initio calculations describing the temperature dependence of the electron-phonon interactions for Cu nanodisks supported on Si. The electrons and phonons temperatures are found to decouple on the ns time scale at 10 K, which is two orders of magnitude in excess with respect to that found for standard low-temperature transport experiments. By accounting for the physics behind our results we suggest an alternative route for overhauling the present knowledge of the electron-phonon decoupling mechanism in nanoscale systems by replacing the mK temperature requirements of conventional experiments with experiments in the time-domain.Comment: 5 pages, 3 figures. Accepted on Physical Review B

    Evolution of the magnetic phase transition in MnO confined to channel type matrices. Neutron diffraction study

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    Neutron diffraction studies of antiferromagnetic MnO confined to MCM-41 type matrices with channel diameters 24-87 A demonstrate a continuous magnetic phase transition in contrast to a discontinuous first order transition in the bulk. The character of the magnetic transition transforms with decreasing channel diameter, showing the decreasing critical exponent and transition temperature, however the latter turns out to be above the N\'eel temperature for the bulk. This enhancement is explained within the framework of Landau theory taking into consideration the ternary interaction of the magnetic and associated structural order parameters.Comment: 6 pages pdf file, including 4 figures, uses revtex4.cl

    Quasiparticle relaxation dynamics in heavy fermion compounds

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    We present the first femtosecond studies of electron-phonon (e-ph) thermalization in heavy fermion compounds. The e-ph thermalization time tau_{ep} increases below the Kondo temperature by more than two orders of magnitude as T = 0 K is approached. Analysis using the two-temperature model and numerical simulations based on Boltzmann's equations suggest that this anomalous slowing down of the e-ph thermalization derives from the large electronic specific heat and the suppresion of scattering between heavy electrons and phonons.Comment: 4 pages, 3 figures, accepted for publication in Phys. Rev. Let
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