57 research outputs found

    Laser induced electron diffraction: a tool for molecular orbital imaging

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    We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show that the electron recollision process taking place after an initial tunnel ionization stage results in quantum interference patterns in the energy resolved photo-electron signals. If the molecule is initially aligned perpendicular to the field polarization, the position and relative heights of the associated fringes can be related to the molecular geometrical and orbital structure, using a simple inversion algorithm which takes into account the symmetry of the initial molecular orbital from which the ionized electron is produced. We show that it is possible to extract inter-atomic distances in the molecule from an averaged photon-electron signal with an accuracy of a few percents

    Electron-energy bunching in laser-driven soft recollisions

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    We introduce soft recollisions in laser-matter interaction. They are characterized by the electron missing the ion upon recollision in contrast to the well-known head-on collisions responsible for high-harmonic generation or above-threshold ionization. We demonstrate analytically that soft recollisions can cause a bunching of photo-electron energies through which a series of low-energy peaks emerges in the electron yield along the laser polarization axis. This peak sequence is universal, it does not depend on the binding potential, and is found below an excess energy of one fifth of the ponderomotive energy.Comment: 4 pages, 3 figures, 1 tabl

    Ultrafast Molecular Imaging by Laser Induced Electron Diffraction

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    We address the feasibility of imaging geometric and orbital structure of a polyatomic molecule on an attosecond time-scale using the laser induced electron diffraction (LIED) technique. We present numerical results for the highest molecular orbitals of the CO2 molecule excited by a near infrared few-cycle laser pulse. The molecular geometry (bond-lengths) is determined within 3% of accuracy from a diffraction pattern which also reflects the nodal properties of the initial molecular orbital. Robustness of the structure determination is discussed with respect to vibrational and rotational motions with a complete interpretation of the laser-induced mechanisms

    Multiphoton radiative recombination of electron assisted by laser field

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    In the presence of an intensive laser field the radiative recombination of the continuum electron into an atomic bound state generally is accompanied by absorption or emission of several laser quanta. The spectrum of emitted photons represents an equidistant pattern with the spacing equal to the laser frequency. The distribution of intensities in this spectrum is studied employing the Keldysh-type approximation, i.e. neglecting interaction of the impact electron with the atomic core in the initial continuum state. Within the adiabatic approximation the scale of emitted photon frequencies is subdivided into classically allowed and classically forbidden domains. The highest intensities correspond to emission frequencies close to the edges of classically allowed domain. The total cross section of electron recombination summed over all emitted photon channels exhibits negligible dependence on the laser field intensity.Comment: 14 pages, 5 figures (Figs.2-5 have "a" and "b" parts), Phys.Rev.A accepted for publication. Fig.2b is presented correctl

    Many Body Correlation Corrections to Superconducting Pairing in Two Dimensions.

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    We demonstrate that in the strong coupling limit (the superconducting gap Δ\Delta is as large as the chemical potential μ\mu), which is relevant to the high-TcT_c superconductivity, the correlation corrections to the gap and critical temperature are about 10\% of the corresponding mean field approximation values. For the weak coupling (Δμ\Delta \ll \mu) the correlation corrections are very large: of the order of 100\% of the corresponding mean field values.Comment: LaTeX 12 page

    Adiabatic Theory of Electron Detachment from Negative Ions in Two-Color Laser Field

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    Negative ion detachment in bichromatic laser field is considered within the adiabatic theory. The latter represents a recent modification of the famous Keldysh model for multiphoton ionization which makes it quantitatively reliable. We calculate angular differential detachment rates, partial rates for particular ATD (Above Threshold Detachment) channels and total detachment rates for the Hydrogen ion in a bichromatic field with 1:3 frequency ratio and various phase differences. Reliability of the present, extremely simple approach is testified by comparison with much more elaborate earlier calculations.Comment: 22 pages, 6 Postscript figure

    Landau mapping and Fermi liquid parameters of the 2D t-J model

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    We study the momentum distribution function n(k) in the 2D t-J model on small clusters by exact diagonalization. We show that n(k) can be decomposed systematically into two components with Bosonic and Fermionic doping dependence. The Bosonic component originates from the incoherent motion of holes and has no significance for the low energy physics. For the Fermionic component we exlicitely perform the one-to-one Landau mapping between the low lying eigenstates of the t-J model clusters and those of an equivalent system of spin-1/2 quasiparticles. This mapping allows to extract the quasiparticle dispersion, statistics, and Landau parameters. The results show conclusively that the 2D t-J model for small doping is a Fermi liquid with a `small' Fermi surface and a moderately strong attractive interaction between the quasiparticles.Comment: Revtex file, 5 pages with 5 embedded eps-files, hardcopies of figures (or the entire manuscript) can be obtained by e-mail request to: [email protected]

    Recent Developments in Precision Electroweak Physics

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    Developments in precision electroweak physics in the two years since the symposium are briefly summarized.Comment: Update on recent developments, prepared for the publication of the Proceedings of Alberto Sirlin Symposium, New York University, October 2000. 10 pages, 1 figur

    Antiferromagnetic and van Hove Scenarios for the Cuprates: Taking the Best of Both Worlds

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    A theory for the high temperature superconductors is proposed. Holes are spin-1/2, charge e, quasiparticles strongly dressed by spin fluctuations. Based on their dispersion, it is claimed that the experimentally observed van Hove singularities of the cuprates are likely originated by antiferromagnetic (AF) correlations. From the two carriers problem in the 2D t-J model, an effective Hamiltonian for holes is defined with %no free parameters. This effective model has superconductivity in the dx2y2{\rm d_{x^2-y^2}} channel, a critical temperature Tc100K{\rm T_c \sim 100K} at the optimal hole density, x=0.15{\rm x=0.15}, and a quasiparticle lifetime linearly dependent with energy. Other experimental results are also quantitativelyquantitatively reproduced by the theory.Comment: 12 pages, 4 figures (on request), RevTeX (version 3.0), preprint NHMF

    Two-hole problem in the t-J model: A canonical transformation approach

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    The t-J model in the spinless-fermion representation is studied. An effective Hamiltonian for the quasiparticles is derived using canonical transformation approach. It is shown that the rather simple form of the transformation generator allows to take into account effect of hole interaction with the short-range spin waves and to describe the single-hole groundstate. Obtained results are very close to ones of the self-consistent Born approximation. Further accounting for the long-range spin-wave interaction is possible on the perturbative basis. Both spin-wave exchange and an effective interaction due to minimization of the number of broken antiferromagnetic bonds are included in the effective quasiparticle interaction. Two-hole bound state problem is solved using Bethe-Salpeter equation. The only d-wave bound state is found to exist in the region of 1< (t/J) <5. Combined effect of the pairing interactions of both types is important to its formation. Discussion of the possible relation of the obtained results to the problem of superconductivity in real systems is presented.Comment: 19 pages, RevTeX, 12 postscript figure
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