200 research outputs found

    Pressure induced superconductivity in CaFe2_2As2_2

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    CaFe2_2As2_2 has been found to be exceptionally sensitive to the application of hydrostatic pressure and superconductivity has been found to exist in a narrow pressure region that appears to be at the interface between two different phase transitions. The pressure - temperature (P−TP - T) phase diagram of CaFe2_2As2_2 reveals that this stoichiometric, highly ordered, compound can be easily tuned to reveal all the salient features associated with FeAs-based superconductivity without introducing any disorder. Whereas at ambient pressure CaFe2_2As2_2 does not superconduct for T>1.8T > 1.8 K and manifests a first order structural phase transition near T≈170T \approx 170 K, the application of ∼5\sim 5 kbar hydrostatic pressure fully suppresses the resistive signature of the structural phase transition and instead superconductivity is detected for T<12T < 12 K. For P≥5.5P \ge 5.5 kbar a different transition is detected, one associated with a clear reduction in resistivity and for P>8.6P > 8.6 kbar superconductivity is no longer detected. This higher pressure transition temperature increases rapidly with increasing pressure, exceeding 300 K by P∼17P \sim 17 kbar. The low temperature, superconducting dome is centered around 5 kbar, extending down to 2.3 kbar and up to 8.6 kbar. This superconducting phase appears to exist when the low pressure transition is suppressed sufficiently, but before the high pressure transition has reduced the resistivity, and possibly the associated fluctuations, too dramatically

    Combined effects of pressure and Ru substitution on BaFe2As2

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    The ab-plane resistivity of Ba(Fe1-xRux)2As2 (x = 0.00, 0.09, 0.16, 0.21, and 0.28) was studied under nearly hydrostatic pressures, up to 7.4 GPa, in order to explore the T-P phase diagram and to compare the combined effects of iso-electronic Ru substitution and pressure. The parent compound BaFe2As2 exhibits a structural/magnetic phase transition near 134 K. At ambient pressure, progressively increasing Ru concentration suppresses this phase transition to lower temperatures at the approximate rate of ~5 K/% Ru and is correlated with the emergence of superconductivity. By applying pressure to this system, a similar behavior is seen for each concentration: the structural/magnetic phase transition is further suppressed and superconductivity induced and ultimately, for larger x Ru and P, suppressed. A detailed comparison of the T-P phase diagrams for all Ru concentrations shows that 3 GPa of pressure is roughly equivalent to 10% Ru substitution. Furthermore, due to the sensitivity of Ba(Fe1-xRux)2As2 to pressure conditions, the melting of the liquid media, 4 : 6 light mineral oil : n-pentane and 1 : 1 iso-pentane : n-pentane, used in this study could be readily seen in the resistivity measurements. This feature was used to determine the freezing curves for these media and infer their room temperature, hydrostatic limits: 3.5 and 6.5 GPa, respectively.Comment: 27 pages, 19 figure

    Thermal expansion and magnetostriction of pure and doped RAgSb2 (R = Y, Sm, La) single crystals

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    Data on temperature-dependent, anisotropic thermal expansion in pure and doped RAgSb2 (R = Y, Sm, La) single crystals are presented. Using the Ehrenfest relation and heat capacity measurements, uniaxial pressure derivatives for long range magnetic ordering and charge density wave transition temperatures are evaluated and compared with the results of the direct measurements under hydrostatic pressure. In-plane and c-axis pressure have opposite effect on the phase transitions in these materials, with in-plane effects being significantly weaker. Quantum oscillations in magnetostriction were observed for the three pure compounds, with the possible detection of new frequencies in SmAgSb2 and LaAgSb2. The uniaxial (along the c-axis) pressure derivatives of the dominant extreme orbits (beta) were evaluated for YAgSb2 and LaAgSb2

    Effect of pressure on the structural phase transition and superconductivity in (B$_{1-x}K_x)Fe_2As_2 (x = 0 and 0.45) and SrFe_2As_2 single crystals

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    The effects of pressure up to ∼20\sim 20 kbar, on the structural phase transition of SrFe2_2As2_2 and lightly Sn-doped BaFe2_2As2_2, as well as on the superconducting transition temperature and upper critical field of (Ba0.55_{0.55}K0.45_{0.45})Fe2_2As2_2 single crystals have been studied. All the transition temperatures decrease with pressure in an almost linear fashion. Under pressure, the upper critical field curve, Hc2(T)H_{c2}(T), for (Ba0.55_{0.55}K0.45_{0.45})Fe2_2As2_2 shifts down in temperature to follow the zero field TcT_c with very little change in slope. Composite P−TP - T phase diagrams for three parent compounds, AFe2_2As2_2 (A = Ba, Sr, Ca), are constructed and appear to be remarkably similar: (i) having a structural (antiferromagnetic) phase transition line with a negative slope and (ii) showing signs of the emerging superconducting state at intermediate pressures
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