30,062 research outputs found

    Field-free molecular orientation by THz laser pulses at high temperature

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    We investigate to which extend a THz laser pulse can be used to produce field-free molecular orientation at high temperature. We consider laser pulses that can be implemented with the state of the art technology and we show that the efficiency of the control scheme crucially depends on the parameters of the molecule. We analyze the temperature effects on molecular dynamics and we demonstrate that, for some molecules, a noticeable orientation can be achieved at high temperature.Comment: 13 pages, 7 figure

    Malmheden's theorem revisited

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    In 1934 H. Malmheden discovered an elegant geometric algorithm for solving the Dirichlet problem in a ball. Although his result was rediscovered independently by Duffin 23 years later, it still does not seem to be widely known. In this paper we return to Malmheden's theorem, give an alternative proof of the result that allows generalization to polyharmonic functions and, also, discuss applications of his theorem to geometric properties of harmonic measures in balls in Euclidean spaces

    Photoassociation adiabatic passage of ultracold Rb atoms to form ultracold Rb_2 molecules

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    We theoretically explore photoassociation by Adiabatic Passage of two colliding cold ^{85}Rb atoms in an atomic trap to form an ultracold Rb_2 molecule. We consider the incoherent thermal nature of the scattering process in a trap and show that coherent manipulations of the atomic ensemble, such as adiabatic passage, are feasible if performed within the coherence time window dictated by the temperature, which is relatively long for cold atoms. We show that a sequence of ~2*10^7 pulses of moderate intensities, each lasting ~750 ns, can photoassociate a large fraction of the atomic ensemble at temperature of 100 microkelvin and density of 10^{11} atoms/cm^3. Use of multiple pulse sequences makes it possible to populate the ground vibrational state. Employing spontaneous decay from a selected excited state, one can accumulate the molecules in a narrow distribution of vibrational states in the ground electronic potential. Alternatively, by removing the created molecules from the beam path between pulse sets, one can create a low-density ensemble of molecules in their ground ro-vibrational state.Comment: RevTex, 23 pages, 9 figure

    Overlapping resonances in the control of intramolecular vibrational redistribution

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    Coherent control of bound state processes via the interfering overlapping resonances scenario [Christopher et al., J. Chem. Phys. 123, 064313 (2006)] is developed to control intramolecular vibrational redistribution (IVR). The approach is applied to the flow of population between bonds in a model of chaotic OCS vibrational dynamics, showing the ability to significantly alter the extent and rate of IVR by varying quantum interference contributions.Comment: 10 pages, 7 figure

    Incomplete Photonic Bandgap as Inferred from the Speckle Pattern of Scattered Light Waves

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    Motivated by recent experiments on intensity correlations of the waves transmitted through disordered media, we demonstrate that the speckle pattern from disordered photonic crystal with incomplete band-gap represents a sensitive tool for determination the stop-band width. We establish the quantitative relation between this width and the {\em angualar anisotropy} of the intensity correlation function.Comment: 6 pages, 3 figure

    Automatic structures, rational growth and geometrically finite hyperbolic groups

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    We show that the set SA(G)SA(G) of equivalence classes of synchronously automatic structures on a geometrically finite hyperbolic group GG is dense in the product of the sets SA(P)SA(P) over all maximal parabolic subgroups PP. The set BSA(G)BSA(G) of equivalence classes of biautomatic structures on GG is isomorphic to the product of the sets BSA(P)BSA(P) over the cusps (conjugacy classes of maximal parabolic subgroups) of GG. Each maximal parabolic PP is a virtually abelian group, so SA(P)SA(P) and BSA(P)BSA(P) were computed in ``Equivalent automatic structures and their boundaries'' by M.Shapiro and W.Neumann, Intern. J. of Alg. Comp. 2 (1992) We show that any geometrically finite hyperbolic group has a generating set for which the full language of geodesics for GG is regular. Moreover, the growth function of GG with respect to this generating set is rational. We also determine which automatic structures on such a group are equivalent to geodesic ones. Not all are, though all biautomatic structures are.Comment: Plain Tex, 26 pages, no figure

    Generic Quantum Ratchet Accelerator with Full Classical Chaos

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    A simple model of quantum ratchet transport that can generate unbounded linear acceleration of the quantum ratchet current is proposed, with the underlying classical dynamics fully chaotic. The results demonstrate that generic acceleration of quantum ratchet transport can occur with any type of classical phase space structure. The quantum ratchet transport with full classical chaos is also shown to be very robust to noise due to the large linear acceleration afforded by the quantum dynamics. One possible experiment allowing observation of these predictions is suggested.Comment: 4 pages, 4 figure

    Implementing Quantum Gates by Optimal Control with Doubly Exponential Convergence

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    We introduce a novel algorithm for the task of coherently controlling a quantum mechanical system to implement any chosen unitary dynamics. It performs faster than existing state of the art methods by one to three orders of magnitude (depending on which one we compare to), particularly for quantum information processing purposes. This substantially enhances the ability to both study the control capabilities of physical systems within their coherence times, and constrain solutions for control tasks to lie within experimentally feasible regions. Natural extensions of the algorithm are also discussed.Comment: 4+2 figures; to appear in PR

    A Semi-classical calculus of correlations

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    The method of passive imaging in seismology has been developped recently in order to image the earth crust from recordings of the seismic noise. This method is founded on the computation of correlations of the seismic noise. In this paper, we give an explicit formula for this correlation in the "semi-classical" regime. In order to do that, we define the power spectrum of a random field as the ensemble average of its Wigner measure, this allows phase-space computations: the pseudo-differential calculus and the ray theory. This way, we get a formula for the correlation of the seismic noise in the semi-classcial regime with a source noise which can be localized and non homogeneous. After that, we show how the use of surface guided waves allows to image the earth crust.Comment: To appear in a special issue "Imaging and Monitoring with Seismic Noise" of the series "Comptes Rendus G\'eosciences", from the French "Acad\'emie des sciences
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