Quantum bicriticality in the heavy-fermion metamagnet YbAgGe

Bicritical points, at which two distinct symmetry-broken phases become simultaneously unstable, are typical for spin-flop metamagnetism. Interestingly, the heavy-fermion compound YbAgGe also possesses such a bicritical point (BCP) with a low temperature T_BCP ~ 0.3 K at a magnetic field of mu_0 H_BCP ~ 4.5 T. In its vicinity, YbAgGe exhibits anomalous behavior that we attribute to the influence of a quantum bicritical point (QBCP), that is close in parameter space yet can be reached by tuning T_BCP further to zero. Using high-resolution measurements of the magnetocaloric effect, we demonstrate that the magnetic Grueneisen parameter Gamma_H indeed both changes sign and diverges as required for quantum criticality. Moreover, Gamma_H displays a characteristic scaling behavior but only on the low-field side, H < H_BCP, indicating a pronounced asymmetry with respect to the critical field. We speculate that the small value of T_BCP is related to the geometric frustration of the Kondo-lattice of YbAgGe.Comment: submitted to PR

Magnetic ordering in GdNi2B2C revisited by resonant x-ray scattering: evidence for the double-q model

Recent theoretical efforts aimed at understanding the nature of antiferromagnetic ordering in GdNi2B2C predicted double-q ordering. Here we employ resonant elastic x-ray scattering to test this theory against the formerly proposed, single-q ordering scenario. Our study reveals a satellite reflection associated with a mixed-order component propagation wave vector, viz., (q_a,2q_b,0) with q_b = q_a approx= 0.55 reciprocal lattice units, the presence of which is incompatible with single-q ordering but is expected from the double-q model. A (3q_a,0,0) wave vector (i.e., third-order) satellite is also observed, again in line with the double-q model. The temperature dependencies of these along with that of a first-order satellite are compared with calculations based on the double-q model and reasonable qualitative agreement is found. By examining the azimuthal dependence of first-order satellite scattering, we show the magnetic order to be, as predicted, elliptically polarized at base temperature and find the temperature dependence of the "out of a-b plane" moment component to be in fairly good agreement with calculation. Our results provide qualitative support for the double-q model and thus in turn corroborate the explanation for the "magnetoelastic paradox" offered by this model.Comment: 8 pages, 5 figures. Submitted to Phys. Rev.

Anisotropic Hc2 of K0.8Fe1.76Se2 determined up to 60 T

The anisotropic upper critical field, Hc2(T), curves for K0.8Fe1.76Se2 are determined over a wide range of temperatures down to 1.5 K and magnetic fields up to 60 T. Anisotropic initial slopes of Hc2 ~ -1.4 T/K and -4.6 T/K for magnetic field applied along c-axis and ab-plane, respectively, were observed. Whereas the c-axis Hc2|c(T) increases quasi-linearly with decreasing temperature, the ab-plane Hc2|ab(T) shows a flattening, starting near 25 K above 30 T. This leads to a non-monotonic temperature dependence of the anisotropy parameter \gamma= Hc2|ab/Hc2|c. The anisotropy parameter is ~ 2 near Tc ~ 32 K and rises to a maximum \gamma ~ 3.6 around 27 K. For lower temperatures, \gamma decreases with T in a linear fashion, dropping to \gamma ~ 2.5 by T ~ 18 K. Despite the apparent differences between the K0.8Fe1.76Se2 and (Ba0.55K0.45)Fe2As2 or Ba(Fe0.926Co0.074)2As2, in terms of the magnetic state and proximity to an insulating state, the Hc2(T) curves are remarkably similar.Comment: slightly modified version, accepted to PRB, Rapid Communication

Effect of proton irradiation on the normal state low-energy excitations of Ba(Fe1−x_{1-x}Rhx_x)2_2As2_2 superconductors

We present a \asnmr Nuclear Magnetic Resonance (NMR) and resistivity study of the effect of 5.5 MeV proton irradiation on the optimal electron doped ($x=$ 0.068) and overdoped ($x=$ 0.107) Ba(Fe$_{1-x}$Rh$_x$)$_2$As$_2$ iron based superconductors. While the proton induced defects only mildly suppress the critical temperature and increase residual resistivity in both compositions, sizable broadening of the NMR spectra was observed in all the irradiated samples at low temperature. The effect is significantly stronger in the optimally doped sample where the Curie Weiss temperature dependence of the line width suggests the onset of ferromagnetic correlations coexisting with superconductivity at the nanoscale. 1/T$_2$ measurements revealed that the energy barrier characterizing the low energy spin fluctuations of these compounds is enhanced upon proton irradiation, suggesting that the defects are likely slowing down the fluctuations between ($0,\pi)$ and ($\pi$,0) nematic ground states.Comment: 9 pages, 9 figure

Local superconducting density of states of ErNi2B2C

We present local tunnelling microscopy and spectroscopy measurements at low temperatures in single crystalline samples of the magnetic superconductor ErNi2B2C. The electronic local density of states shows a striking departure from s-wave BCS theory with a finite value at the Fermi level, which amounts to half of the normal phase density of states.Comment: 9 pages, 3 figure

Magnetic and superconducting phase diagrams in ErNi2B2C

We present measurements of the superconducting upper critical field Hc2(T) and the magnetic phase diagram of the superconductor ErNi2B2C made with a scanning tunneling microscope (STM). The magnetic field was applied in the basal plane of the tetragonal crystal structure. We have found large gapless regions in the superconducting phase diagram of ErNi2B2C, extending between different magnetic transitions. A close correlation between magnetic transitions and Hc2(T) is found, showing that superconductivity is strongly linked to magnetism.Comment: 5 pages, 4 figure

Strong Enhancement of the Critical Current at the Antiferromagnetic Transition in ErNi2B2C Single Crystals

We report on transport and magnetization measurements of the critical current density Jc in ErNi2B2C single crystals that show strongly enhanced vortex pinning at the Neel temperature TN and low applied fields. The height of the observed Jc peak decreases with increasing magnetic field in clear contrast with that of the peak effect found at the upper critical field. We also performed the first angular transport measurements of Jc ever conducted on this compound. They reveal the correlated nature of this pinning enhancement, which we attribute to the formation of antiphase boundaries at TN.Comment: 3 figure

High-resolution x-ray diffraction study of the heavy-fermion compound YbBiPt

YbBiPt is a heavy-fermion compound possessing significant short-range antiferromagnetic correlations below a temperature of $T^{\textrm{*}}=0.7$ K, fragile antiferromagnetic order below $T_{\rm{N}}=0.4$ K, a Kondo temperature of $T_{\textrm{K}} \approx1$ K, and crystalline-electric-field splitting on the order of $E/k_{\textrm{B}}=1\,\textrm{-}\,10$ K. Whereas the compound has a face-centered-cubic lattice at ambient temperature, certain experimental data, particularly those from studies aimed at determining its crystalline-electric-field scheme, suggest that the lattice distorts at lower temperature. Here, we present results from high-resolution, high-energy x-ray diffraction experiments which show that, within our experimental resolution of $\approx6\,\textrm{-}\,10\times10^{-5}$ \AA, no structural phase transition occurs between $T=1.5$ and $50$ K. In combination with results from dilatometry measurements, we further show that the compound's thermal expansion has a minimum at $\approx18$ K and a region of negative thermal expansion for $9<T<18$ K. Despite diffraction patterns taken at $1.6$ K which indicate that the lattice is face-centered cubic and that the Yb resides on a crystallographic site with cubic point symmetry, we demonstrate that the linear thermal expansion may be modeled using crystalline-electric-field level schemes appropriate for Yb$^{3+}$ residing on a site with either cubic or less than cubic point symmetry.Comment: 7 pages, 3 figures, submitted to Phys. Rev.

Direct observation of Fe spin reorientation in single crystalline YbFe6Ge6

We have grown single crystals of YbFe6Ge6 and LuFe6Ge6 and characterized their anisotropic behaviour through low field magnetic susceptibility, field-dependent magnetization, resistivity and heat capacity measurements. The Yb+3 valency is confirmed by LIII XANES measurements. YbFe6Ge6 crystals exhibit a field-dependent, sudden reorientation of the Fe spins at about 63 K, a unique effect in the RFe6Ge6 family (R = rare earths) where the Fe ions order anti-ferromagnetically with Neel temperatures above 450 K and the R ions' magnetism appears to behave independently. The possible origins of this unusual behaviour of the ordered Fe moments in this compound are discussed.Comment: 12 pages, 8 figures, accepted in J. Phys.: Cond. Matte

Effect of electron irradiation on superconductivity in single crystals of Ba(Fe1−x_{1-x}Rux_{x})2_2As2_2 (x=x=0.24)

A single crystal of isovalently substituted Ba(Fe$_{1-x}$Ru$_{x}$)$_2$As$_2$ ($x=0.24$) was sequentially irradiated with 2.5 MeV electrons up to a maximum dose of $2.1 \times 10^{19}$ electrons/cm^2. The electrical resistivity was measured \textit{in - situ} at $T=$22 K during the irradiation and \textit{ex - situ} as a function of temperature between subsequent irradiation runs. Upon irradiation, the superconducting transition temperature, $T_c$, decreases and the residual resistivity, $\rho_0$, increases. We find that electron irradiation leads to the fastest suppression of $T_c$ compared to other types of artificially introduced disorder, probably due to the strong short-range potential of the point-like irradiation defects. A more detailed analysis within a multiband scenario with variable scattering potential strength shows that the observed $T_c$ vs. $\rho_0$ is fully compatible with $s_\pm$ pairing, in contrast to earlier claims that this model leads to a too rapid a suppression of $T_c$ with scattering