278 research outputs found
Dielectronic recombination data for astrophysical applications: Plasma rate-coefficients for Fe^q+ (q=7-10, 13-22) and Ni^25+ ions from storage-ring experiments
This review summarizes the present status of an ongoing experimental effort
to provide reliable rate coefficients for dielectronic recombination of highly
charged iron ions for the modeling of astrophysical and other plasmas. The
experimental work has been carried out over more than a decade at the heavy-ion
storage-ring TSR of the Max-Planck-Institute for Nuclear Physics in Heidelberg,
Germany. The experimental and data reduction procedures are outlined. The role
of previously disregarded processes such as fine-structure core excitations and
trielectronic recombination is highlighted. Plasma rate coefficients for
dielectronic recombination of Fe^q+ ions (q=7-10, 13-22) and Ni^25+ are
presented graphically and in a simple parameterized form allowing for easy use
in plasma modeling codes. It is concluded that storage-ring experiments are
presently the only source for reliable low-temperature dielectronic
recombination rate-coefficients of complex ions.Comment: submitted for publication in the International Review of Atomic and
Molecular Physics, 8 figures, 3 tables, 68 reference
Enhanced dielectronic recombination of lithium-like Ti19+ ions in external ExB fields
Dielectronic recombination(DR) of lithium-like Ti19+(1s2 2s) ions via 2s->2p
core excitations has been measured at the Heidelberg heavy ion storage ring
TSR. We find that not only external electric fields (0 <= Ey <= 280 V/cm) but
also crossed magnetic fields (30 mT <= Bz <= 80 mT) influence the DR via high-n
(2p_j nl)-Rydberg resonances. This result confirms our previous finding for
isoelectronic Cl14+ ions [Bartsch T et al, PRL 82, 3779 (1999)] that
experimentally established the sensitivity of DR to ExB fields. In the present
investigation the larger 2p_{1/2}-2p_{3/2} fine structure splitting of Ti19+
allowed us to study separately the influence of external fields via the two
series of Rydberg DR resonances attached to the 2s -> 2p_{1/2} and 2s ->
2p_{3/2} excitations of the Li-like core, extracting initial slopes and
saturation fields of the enhancement. We find that for Ey > 80 V/cm the field
induced enhancement is about 1.8 times stronger for the 2p_{3/2} series than
for the 2p_{1/2} series.Comment: 10 pages, 3 figures, to be published in Journal of Physics B, see
also http://www.strz.uni-giessen.de/~k
Near--K-edge double and triple detachment of the F- negative ion: observation of direct two-electron ejection by a single photon
Double and triple detachment of the F-(1s2 2s2 2p6) negative ion by a single
photon have been investigated in the photon energy range 660 to 1000 eV. The
experimental data provide unambiguous evidence for the dominant role of direct
photo-double-detachment with a subsequent single-Auger process in the reaction
channel leading to F2+ product ions. Absolute cross sections were determined
for the direct removal of a (1s+2p) pair of electrons from F- by the absorption
of a single photon
Single-photon single ionization of W ions: experiment and theory
Experimental and theoretical results are reported for photoionization of
Ta-like (W) tungsten ions. Absolute cross sections were measured in the
energy range 16 to 245 eV employing the photon-ion merged-beam setup at the
Advanced Light Source in Berkeley. Detailed photon-energy scans at 100 meV
bandwidth were performed in the 16 to 108 eV range. In addition, the cross
section was scanned at 50 meV resolution in regions where fine resonance
structures could be observed. Theoretical results were obtained from a
Dirac-Coulomb R-matrix approach. Photoionization cross section calculations
were performed for singly ionized atomic tungsten ions in their , =1/2, ground level and the associated
excited metastable levels with =3/2, 5/2, 7/2 and 9/2. Since the ion beams
used in the experiments must be expected to contain long-lived excited states
also from excited configurations, additional cross-section calculations were
performed for the second-lowest term, 5d^5 \; ^6{\rm S}_{J}, =5/2, and for
the F term, 5d^3 6s^2 \; ^4{\rm F}_{J}, with = 3/2, 5/2, 7/2 and 9/2.
Given the complexity of the electronic structure of W the calculations
reproduce the main features of the experimental cross section quite well.Comment: 23 pages, 7 figures, 1 table: Accepted for publication in J. Phys. B:
At. Mol. & Opt. Phy
Photoionization of tungsten ions: Experiment and theory for W5+
Experimental and theoretical cross sections are reported for single-photon single ionization of W5+ ions. Absolute measurements were conducted employing the photon-ion merged-beams technique. Detailed photon-energy scans were performed at (67 ± 10) meV resolution in the 20-160 eV range. In contrast to photoionization of tungsten ions in lower charge states, the cross section is dominated by narrow, densely-spaced resonances. Theoretical results were obtained from a Dirac-Coulomb R-matrix approach employing a basis set of 457 levels providing cross sections for photoionization of W5+ ions in the ground level as well as the and metastable excited levels. Considering the complexity of the electronic structure of tungsten ions in low charge states, the agreement between theory and experiment is satisfactory
Interference effects in the photorecombination of argonlike Sc3+ ions: Storage-ring experiment and theory
Absolute total electron-ion recombination rate coefficients of argonlike
Sc3+(3s2 3p6) ions have been measured for relative energies between electrons
and ions ranging from 0 to 45 eV. This energy range comprises all dielectronic
recombination resonances attached to 3p -> 3d and 3p -> 4s excitations. A broad
resonance with an experimental width of 0.89 +- 0.07 eV due to the 3p5 3d2 2F
intermediate state is found at 12.31 +- 0.03 eV with a small experimental
evidence for an asymmetric line shape. From R-Matrix and perturbative
calculations we infer that the asymmetric line shape may not only be due to
quantum mechanical interference between direct and resonant recombination
channels as predicted by Gorczyca et al. [Phys. Rev. A 56, 4742 (1997)], but
may partly also be due to the interaction with an adjacent overlapping DR
resonance of the same symmetry. The overall agreement between theory and
experiment is poor. Differences between our experimental and our theoretical
resonance positions are as large as 1.4 eV. This illustrates the difficulty to
accurately describe the structure of an atomic system with an open 3d-shell
with state-of-the-art theoretical methods. Furthermore, we find that a
relativistic theoretical treatment of the system under study is mandatory since
the existence of experimentally observed strong 3p5 3d2 2D and 3p5 3d 4s 2D
resonances can only be explained when calculations beyond LS-coupling are
carried out.Comment: 11 pages, 7 figures, 3 tables, Phys. Rev. A (in print), see also:
http://www.strz.uni-giessen.de/~k
K-shell photoionization of ground-state Li-like carbon ions [C]: experiment, theory and comparison with time-reversed photorecombination
Absolute cross sections for the K-shell photoionization of ground-state
Li-like carbon [C(1s2s S)] ions were measured by employing the
ion-photon merged-beams technique at the Advanced Light Source. The energy
ranges 299.8--300.15 eV, 303.29--303.58 eV and 335.61--337.57 eV of the
[1s(2s2p)P]P, [1s(2s2p)P]P and [(1s2s)S 3p]P
resonances, respectively, were investigated using resolving powers of up to
6000. The autoionization linewidth of the [1s(2s2p)P]P resonance was
measured to be meV and compares favourably with a theoretical result
of 26 meV obtained from the intermediate coupling R-Matrix method. The present
photoionization cross section results are compared with the outcome from
photorecombination measurements by employing the principle of detailed balance.Comment: 3 figures and 2 table
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