33,482 research outputs found
Prewetting transition on a weakly disordered substrate : evidence for a creeping film dynamics
We present the first microscopic images of the prewetting transition of a
liquid film on a solid surface. Pictures of the local coverage map of a helium
film on a cesium metal surface are taken while the temperature is raised
through the transition. The film edge is found to advance at constant
temperature by successive avalanches in a creep motion with a macroscopic
correlation length. The creep velocity varies strongly in a narrow temperature
range. The retreat motion is obtained only at much lower temperature,
conforming to the strong hysteresis observed for prewetting transition on a
disordered surface. Prewetting transition on such disordered surfaces appears
to give rise to dynamical phenomena similar to what is observed for domain wall
motions in 2D magnets.Comment: 7 pages, 3 figures, to be published in Euro.Phys.Let
Nonequilibrium Relaxations and Aging Effects in a Two-Dimensional Coulomb Glass
The relaxations of conductivity have been studied in the glassy regime of a
strongly disordered two-dimensional electron system in Si after a temporary
change of carrier density during the waiting time t_w. Two types of response
have been observed: a) monotonic, where relaxations exhibit aging, i.e.
dependence on history, determined by t_w and temperature; b) nonmonotonic,
where a memory of the sample history is lost. The conditions that separate the
two regimes have been also determined.Comment: 4 pages; published versioi
Building block libraries and structural considerations in the self-assembly of polyoxometalate and polyoxothiometalate systems
Inorganic metal-oxide clusters form a class of compounds that are unique in their topological and electronic versatility and are becoming increasingly more important in a variety of applications. Namely, Polyoxometalates (POMs) have shown an unmatched range of physical properties and the ability to form structures that can bridge several length scales. The formation of these molecular clusters is often ambiguous and is governed by self-assembly processes that limit our ability to rationally design such molecules. However, recent years have shown that by considering new building block principles the design and discovery of novel complex clusters is aiding our understanding of this process. Now with current progress in thiometalate chemistry, specifically polyoxothiometalates (POTM), the field of inorganic molecular clusters has further diversified allowing for the targeted development of molecules with specific functionality. This chapter discusses the main differences between POM and POTM systems and how this affects synthetic methodologies and reactivities. We will illustrate how careful structural considerations can lead to the generation of novel building blocks and further deepen our understanding of complex systems
Projective Quantum Monte Carlo Method for the Anderson Impurity Model and its Application to Dynamical Mean Field Theory
We develop a projective quantum Monte Carlo algorithm of the Hirsch-Fye type
for obtaining ground state properties of the Anderson impurity model. This
method is employed to solve the self-consistency equations of dynamical mean
field theory. It is shown that the approach converges rapidly to the ground
state so that reliable zero-temperature results are obtained. As a first
application, we study the Mott-Hubbard metal-insulator transition of the
one-band Hubbard model, reconfirming the numerical renormalization group
results.Comment: 4 pages, 4 figure
Paramagnetic reentrant effect in high purity mesoscopic AgNb proximity structures
We discuss the magnetic response of clean Ag coated Nb proximity cylinders in
the temperature range 150 \mu K < T < 9 K. In the mesoscopic temperature
regime, the normal metal-superconductor system shows the yet unexplained
paramagnetic reentrant effect, discovered some years ago [P. Visani, A. C.
Mota, and A. Pollini, Phys. Rev. Lett. 65, 1514 (1990)], superimposing on full
Meissner screening. The logarithmic slope of the reentrant paramagnetic
susceptibility chi_para(T) \propto \exp(-L/\xi_N) is limited by the condition
\xi_N=n L, with \xi_N=\hbar v_F/2 \pi k_B T, the thermal coherence length and
n=1,2,4. In wires with perimeters L=72 \mu m and L=130 \mu m, we observe
integer multiples n=1,2,4. At the lowest temperatures, \chi_para compensates
the diamagnetic susceptibility of the \textit{whole} AgNb structure.Comment: 4 pages, 4 figures (color
Prolific pair production with high-power lasers
Prolific electron-positron pair production is possible at laser intensities
approaching 10^{24} W/cm^2 at a wavelength of 1 micron. An analysis of electron
trajectories and interactions at the nodes (B=0) of two counter-propagating,
circularly polarised laser beams shows that a cascade of gamma-rays and pairs
develops. The geometry is generalised qualitatively to linear polarisation and
laser beams incident on a solid target.Comment: 4 pages, 1 figure, minor revisions, accepted for publication in
Physical Review Letter
Molecular transport and flow past hard and soft surfaces: Computer simulation of model systems
The properties of polymer liquids on hard and soft substrates are
investigated by molecular dynamics simulation of a coarse-grained bead-spring
model and dynamic single-chain-in-mean-field (SCMF) simulations of a soft,
coarse-grained polymer model. Hard, corrugated substrates are modelled by an
FCC Lennard-Jones solid while polymer brushes are investigated as a
prototypical example of a soft, deformable surface. From the molecular
simulation we extract the coarse-grained parameters that characterise the
equilibrium and flow properties of the liquid in contact with the substrate:
the surface and interface tensions, and the parameters of the hydrodynamic
boundary condition. The so-determined parameters enter a continuum description
like the Stokes equation or the lubrication approximation.Comment: 41 pages, 13 figure
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