27,592 research outputs found
No well-defined remnant Fermi surface in Sr2CuO2Cl2
In angle-resolved photoelectron spectra of the antiferromagnetic insulators
Ca2CuO2Cl2 and Sr2CuO2Cl2 a sharp drop of the spectral intensity of the
lowest-lying band is observed along a line in k space equivalent to the Fermi
surface of the optimally doped high-temperature superconductors. This was
interpreted as a signature of the existence of a remnant Fermi surface in the
insulating phase of the high-temperature superconductors. In this paper it is
shown that the drop of the spectral intensity is not related to the spectral
function but is a consequence of the electron-photon matrix elementComment: 4 pages, 3 figure
Magnetic-Island Contraction and Particle Acceleration in Simulated Eruptive Solar Flares
The mechanism that accelerates particles to the energies required to produce
the observed high-energy impulsive emission in solar flares is not well
understood. Drake et al. (2006) proposed a mechanism for accelerating electrons
in contracting magnetic islands formed by kinetic reconnection in multi-layered
current sheets. We apply these ideas to sunward-moving flux ropes (2.5D
magnetic islands) formed during fast reconnection in a simulated eruptive
flare. A simple analytic model is used to calculate the energy gain of
particles orbiting the field lines of the contracting magnetic islands in our
ultrahigh-resolution 2.5D numerical simulation. We find that the estimated
energy gains in a single island range up to a factor of five. This is higher
than that found by Drake et al. for islands in the terrestrial magnetosphere
and at the heliopause, due to strong plasma compression that occurs at the
flare current sheet. In order to increase their energy by two orders of
magnitude and plausibly account for the observed high-energy flare emission,
the electrons must visit multiple contracting islands. This mechanism should
produce sporadic emission because island formation is intermittent. Moreover, a
large number of particles could be accelerated in each
magnetohydrodynamic-scale island, which may explain the inferred rates of
energetic-electron production in flares. We conclude that island contraction in
the flare current sheet is a promising candidate for electron acceleration in
solar eruptions.Comment: Accepted for publication in The Astrophysical Journal (2016
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Free healthy breakfasts in primary schools: A cluster randomised controlled trial of a policy intervention in Wales, UK
Objective: The present study evaluated the impact of a national school programme of universal free healthy breakfast provision in Wales, UK.
Design: A cluster randomised controlled trial with repeated cross-sectional design and a 12-month follow-up. Primary outcomes were breakfast skipping, breakfast diet and episodic memory. Secondary outcomes were frequency of eating breakfast at home and at school, breakfast attitudes, rest-of-day diet and class behaviour.
Setting: Primary schools in nine local education authority areas.
Subjects: A total of 4350 students (aged 9–11 years) at baseline and 4472 at follow-up in 111 schools.
Results: Students in intervention schools reported significantly higher numbers of healthy food items consumed at breakfast and more positive attitudes towards breakfast eating at 12 months. Parents in intervention schools reported significantly higher rates of consumption of breakfast at school and correspondingly lower rates of breakfast consumption at home. No other significant differences were found.
Conclusions: The intervention did not reduce breakfast skipping; rather, pupils substituted breakfast at home for breakfast at school. However, there were improvements in children’s nutritional intake at breakfast time, if not the rest of the day, and more positive attitudes to breakfast, which may have implications for life-course dietary behaviours. There was no impact on episodic memory or classroom behaviour, which may require targeting breakfast skippers
Submicrosecond comparisons of time standards via the Navigation Technology Satellites (NTS)
An interim demonstration was performed of the time transfer capability of the NAVSTAR GPS system using a single NTS satellite. Measurements of time difference (pseudo-range) are made from the NTS tracking network and at the participating observatories. The NTS network measurements are used to compute the NTS orbit trajectory. The central NTS tracking station has a time link to the Naval Observatory UTC (USNO,MC1) master clock. Measurements are used with the NTS receiver at the remote observatory, the time transfer value UTC (USNO,MC1)-UTC (REMOTE, VIA NTS) is calculated. Intercomparisons were computed using predicted values of satellite clock offset and ephemeus
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Synthesis and Study of Olefin Metathesis Catalysts Supported by Redox-Switchable Diaminocarbene 3 Ferrocenophanes
A redox-switchable ligand, N,N'-dimethyldiaminocarbene[3]ferrocenophane (5), was synthesized and incorporated into a series of Ir- and Ru-based complexes. Electrochemical and spectroscopic analyses of (5) Ir(CO)(2)Cl (15) revealed that 5 displayed a Tolman electronic parameter value of 2050 cm(-1) in the neutral state and 2061 cm(-1) upon oxidation. Moreover, inspection of X-ray crystallography data recorded for (5) Ir(cis,cis-1,5-cyclooctadiene)Cl (13) revealed that 5 was sterically less bulky (%V-Bur = 28.4) than other known diaminocarbene[3]ferrocenophanes, which facilitated the synthesis of (5)(PPh3)Cl2Ru-(3-phenylindenylid-1-ene) (18). Complex 18 exhibited quasi-reversible electrochemical processes at 0.79 and 0.98 V relative to SCE, which were assigned to the Fe and Ru centers in the complex, respectively, based on UV-vis and electron pair resonance spectroscopic measurements. Adding 2,3-dichloro-5,6-dicyanoquinone over the course of a ring-opening metathesis polymerization of cis, cis-1,5-cyclooctadiene catalyzed by 18 ([monomer](0)/[18](0) = 2500) reduced the corresponding rate constant of the reaction by over an order of magnitude (pre-oxidation: k(obs) = 0.045 s(-1); post-oxidation: k(obs) = 0.0012 s(-1)). Subsequent reduction of the oxidized species using decamethylferrocene restored catalytic activity (post-reduction: k(obs) = up to 0.016 s(-1), depending on when the reductant was added). The difference in the polymerization rates was attributed to the relative donating ability of the redox-active ligand (i.e., strongly donating 5 versus weakly donating 5(+)) which ultimately governed the activity displayed by the corresponding catalyst.U. S. Army Research Office W911NF-09-1-0446Chemistr
Nuclear isotope thermometry
We discuss different aspects which could influence temperatures deduced from
experimental isotopic yields in the multifragmentation process. It is shown
that fluctuations due to the finite size of the system and distortions due to
the decay of hot primary fragments conspire to blur the temperature
determination in multifragmentation reactions. These facts suggest that caloric
curves obtained through isotope thermometers, which were taken as evidence for
a first-order phase transition in nuclear matter, should be investigated very
carefully.Comment: 9 pages, 7 figure
Neutron spectroscopic factors of Ni isotopes from transfer reactions
177 neutron spectroscopic factors for nickel isotopes have been extracted by
performing a systematic analysis of the angular distributions measured from
(d,p) transfer reactions. A subset of the extracted spectroscopic factors are
compared to predictions of large-basis shell models in the full pf model space
using the GXPF1A effective interaction, and the (f5/2, p3/2, p1/2, g9/2) model
space using the JJ4PNA interaction. For ground states, the predicted
spectroscopic factors using the GXPF1A effective interaction in the full pf
model space agree very well with the experimental values, while predictions
based on several other effective interactions and model spaces are about 30%
higher than the experimental values. For low-energy excited states (<3.5 MeV),
the agreement between the extracted spectroscopic factors and shell model
calculations is not better than a factor of two.Comment: 18 pages, 4 figures, 2 tables. accepted for publication in PR
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