2,891 research outputs found

    Visualizing plasmon-exciton polaritons at the nanoscale using electron microscopy

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    Polaritons are compositional light-matter quasiparticles that have recently enabled remarkable breakthroughs in quantum and nonlinear optics, as well as in material science. Despite the enormous progress, however, a direct nanometer-scale visualization of polaritons has remained an open challenge. Here, we demonstrate that plasmon-exciton polaritons, or plexcitons, generated by a hybrid system composed of an individual silver nanoparticle and a few-layer transition metal dichalcogenide can be spectroscopically mapped with nanometer spatial resolution using electron energy loss spectroscopy in a scanning transmission electron microscope. Our experiments reveal important insights about the coupling process, which have not been reported so far. These include nanoscale variation of Rabi splitting and plasmon-exciton detuning, as well as absorption-dominated extinction signals, which in turn provide the ultimate evidence for the plasmon-exciton hybridization in the strong coupling regime. These findings pioneer new possibilities for in-depth studies of polariton-related phenomena with nanometer spatial resolution

    Origin of Spin Incommensurability in Hole-doped S=1 Y2−xCaxBaNiO5\rm Y_{2-x}Ca_x Ba Ni O_5 Chains

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    Spin incommensurability has been recently experimentally discovered in the hole-doped Ni-oxide chain compound Y2−xCaxBaNiO5\rm Y_{2-x}Ca_x Ba Ni O_5 (G. Xu {\it al.}, Science {\bf 289}, 419 (2000)). Here a two orbital model for this material is studied using computational techniques. Spin IC is observed in a wide range of densities and couplings. The phenomenon originates in antiferromagnetic correlations ``across holes'' dynamically generated to improve hole movement, as it occurs in the one-dimensional Hubbard model and in recent studies of the two-dimensional extended t-J model. The close proximity of ferromagnetic and phase-separated states in parameter space are also discussed.Comment: RevTex, 4 pages, 4 figures (eps
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