Controlling the nature of a charged impurity in a bath of Feshbach dimers

We theoretically study the dynamics of a trapped ion that is immersed in an ultracold gas of weakly bound atomic dimers created by a Feshbach resonance. Using quasi-classical simulations, we find a crossover from dimer dissociation to molecular ion formation depending on the binding energy of the dimers. The location of the crossover strongly depends on the collision energy and the time-dependent fields of the Paul trap. Deeply bound dimers lead to fast molecular ion formation, with rates approaching the Langevin collision rate $\Gamma'_\text{L}\approx4.8\times10^{-9}\,$cm$^3$s$^{-1}$. The kinetic energies of the created molecular ions have a median below $1\,$mK, such that they will stay confined in the ion trap. We conclude that interacting ions and Feshbach molecules may provide a novel approach towards the creation of ultracold molecular ions with applications in precision spectroscopy and quantum chemistry.Comment: 9 pages and 12 figures including appendice

Observation of a Strong Atom-Dimer Attraction in a Mass-Imbalanced Fermi-Fermi Mixture

We investigate a mixture of ultracold fermionic $^{40}$K atoms and weakly bound $^{6}$Li$^{40}$K dimers on the repulsive side of a heteronuclear atomic Feshbach resonance. By radio-frequency spectroscopy we demonstrate that the normally repulsive atom-dimer interaction is turned into a strong attraction. The phenomenon can be understood as a three-body effect in which two heavy $^{40}$K fermions exchange the light $^{6}$Li atom, leading to attraction in odd partial-wave channels (mainly p-wave). Our observations show that mass imbalance in a fermionic system can profoundly change the character of interactions as compared to the well-established mass-balanced case

Lifetime of Feshbach dimers in a Fermi-Fermi mixture of 6^6Li and 40^{40}K

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