264 research outputs found
Evidence for the coexistence of low-dimensional magnetism and long-range order in Ca3CoRhO6
We report the results of neutron powder diffraction studies on the spin-chain
compound Ca3CoRhO6 in the temperature range 3 to 293 K. Bragg peaks due to
magnetic ordering start appearing below about 100 K. The most interesting
observation is that there is a diffuse magnetic peak superimposed over the
strongest magnetic Bragg peak. The diffuse magnetic intensity is observed below
as well above 100 K. This finding provides a new insight into the physics of
this compound as though the low-dimensional magnetic interaction coexists with
long range magnetic order - a novel situation among quasi one-dimensional
oxides.Comment: accepted by Eur. Phys. Let
Stability of geometrically frustrated magnetic state of Ca3CoRhO6 to applications of positive and negative pressure
The influence of negative chemical pressure induced by gradual replacement of
Ca by Sr as well as of external pressure (up to 10 kbar) on the magnetism of
Ca3CoRhO6 has been investigated by magnetization studies. It is found that the
solid solution, Ca(3-x)Sr(x)CoRhO6, exists at least till about x= 1.0 without
any change in the crystal structure. Apart from insensitivity of the spin-chain
feature to volume expansion, the characteristic features of geometrical
frustration interestingly appear at the same temperatures for all compositions,
in sharp contrast to the response to Y substitution for Ca (reported
previously). Interestingly, huge frequency dependence of ac susceptibility
known for the parent compound persists for all compositions. We do not find a
change in the properties under external pressure. The stability of the magnetic
anomalies of this compound to the volume change (about 4%) is puzzling
Crystal Field, Magnetic Anisotropy and Excitations in Rare-Earth Hexaborides
We clarify the role of crystalline electric field (CEF) induced magnetic
anisotropy in the ground state and spin-wave spectrum of cubic rare-earth
materials with dominating isotropic magnetic exchange interactions. In
particular we study the hexaboride NdB_6 which is shown to exhibit strong
spin-quadrupolar coupling. The CEF scheme is analyzed and a non-collinear
magnetization response is found. The spin orientation in the
antiferromagnetically ordered ground-state is identified. Moreover, the spin
excitations are evaluated and in agreement with inelastic neutron scattering a
suppression of one of the two magnetic modes in the strong-coupling regime is
predicted.Comment: 4 pages, 1 eps-figur
The magnetic order of GdMn2Ge2 studied by neutron diffraction and x ray resonant magnetic scattering
Interpocket polarization model for magnetic structures in rare-earth hexaborides
The origin of peculiar magnetic structures in cubic rare-earth (R)
hexaborides RB_6 is traced back to their characteristic band structure. The
three sphere-like Fermi surfaces induce interpocket polarization of the
conduction band as a part of a RKKY-type interaction. It is shown for the
free-electron-like model that the interpocket polarization gives rise to a
broad maximum in the intersite interaction I(q) around q=(1/4,1/4,1/2) in the
Brillouin zone. This maximum is consistent with the superstructure observed in
R=Ce, Gd and Dy. The wave-number dependence of I(q) is independently extracted
from analysis of the spin-wave spectrum measured for NdB_6. It is found that
I(q) obtained from fitting the data has a similarly to that derived by the
interpocket polarization model, except that the absolute maximum now occurs at
(0,0,1/2) in consistency with the A-type structure. The overall shape of I(q)
gives a hint toward understanding an incommensurate structure in PrB_6 as well.Comment: 5 pages, 3 figures, submitted to J.Phys.Soc.Jp
Highly Dispersive Spin Excitations in the Chain Cuprate Li2CuO2
We present an inelastic neutron scattering investigation of Li2CuO2 detecting
the long sought quasi-1D magnetic excitations with a large dispersion along the
CuO2-chains studied up to 25 meV. The total dispersion is governed by a
surprisingly large ferromagnetic (FM) nearest-neighbor exchange integral
J1=-228 K. An anomalous quartic dispersion near the zone center and a
pronounced minimum near (0,0.11,0.5) r.l.u. (corresponding to a spiral
excitation with a pitch angle about 41 degree point to the vicinity of a 3D
FM-spiral critical point. The leading exchange couplings are obtained applying
standard linear spin-wave theory. The 2nd neighbor inter-chain interaction
suppresses a spiral state and drives the FM in-chain ordering below the Ne'el
temperature. The obtained exchange parameters are in agreement with the results
for a realistic five-band extended Hubbard Cu 3d O 2p model and L(S)DA+U
predictions.Comment: 6 pages, 4 figures, submitted to Europhys. Let
Elastic Properties and Magnetic Phase Diagrams of Dense Kondo Compound Ce0.75La0.25B6
We have investigated the elastic properties of the cubic dense Kondo compound
Ce0.75La0.25B6 by means of ultrasonic measurements. We have obtained magnetic
fields vs temperatures (H-T) phase diagrams under magnetic fields along the
crystallographic [001], [110] and [111] axes. An ordered phase IV showing the
elastic softening of c44 locates in low temperature region between 1.6 and 1.1
K below 0.7 T in all field directions. The phase IV shows an isotropic nature
with regard to the field directions, while the antiferro-magnetic phase III
shows an anisotropic character. A remarkable softening of c44 and a spontaneous
trigonal distortion εyz+εzx+εxy recently reported by Akatsu et
al. [J. Phys. Soc. Jpn. 72 (2003) 205] in the phase IV favor a ferro-quadrupole
(FQ) moment of Oyz+Ozx+Oxy induced by an octupole ordering.Comment: 9 figures, Strongly Correlated Electron
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