4 research outputs found
Green Light Photoelectrocatalysis with Sulfur-Doped Carbon Nitride: Using Triazole-Purpald for Enhanced Benzylamine Oxidation and Oxygen Evolution Reactions
- Author
- Publication venue
- Publication date
- 01/01/2023
- Field of study
Get PDFMaterials dictate carbon neutral industrial chemical processes. Visible-light photoelectrocatalysts from abundant resources will play a key role in exploiting solar irradiation. Anionic doping via pre-organization of precursors and further co-polymerization creates tuneable semiconductors. Triazole derivative-purpald, an unexplored precursor with sulfur (S) container, combined in different initial ratios with melamine during one solid-state polycondensation with two thermal steps yields hybrid S-doped carbon nitrides (C3N4). The series of S-doped/C3N4-based materials show enhanced optical, electronic, structural, textural, and morphological properties and exhibit higher performance in organic benzylamine photooxidation, oxygen evolution, and similar energy storage (capacitor brief investigation). 50M-50P exhibits the highest photooxidation conversion (84 +/- 3%) of benzylamine to imine at 535 nm - green light for 48 h, due to a discrete shoulder (approximate to 700) nm, high sulfur content, preservation of crystal size, new intraband energy states, structural defects by layer distortion, and 10-16 nm pores with arbitrary depth. This work innovates by studying the concomitant relationships between: 1) the precursor decomposition while C3N4 is formed, 2) the insertion of S impurities, 3) the S-doped C3N4 property-activity relationships, and 4) combinatorial surface, bulk, structural, optical, and electronic characterization analysis. This work contributes to the development of disordered long-visible-light photocatalysts for solar energy conversion and storage
Correction: Nitrogen-doped carbons prepared from eutectic mixtures as metal-free oxygen reduction catalysts
- Author
- Publication venue
- 'Royal Society of Chemistry (RSC)'
- Publication date
- 01/01/2018
- Field of study
No full textThe authors regret the omission of an Acknowledgements section in the original manuscript. The Acknowledgements section should be as below. Acknowledgements. This study was supported by MINECO (Project Numbers MAT2012-34811 and MAT2015-68639-R). N. L.-S. acknowledges MINECO for a FPI contract. The Royal Society of Chemistry apologises for these errors and any consequent inconvenience to authors and readers
Body mass index and complications following major gastrointestinal surgery: a prospective, international cohort study and meta-analysis
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- Publication venue
- Publication date
- 01/01/2018
- Field of study
No full textAim: Previous studies reported conflicting evidence on the effects of obesity on outcomes after gastrointestinal surgery. The aims of this study were to explore the relationship of obesity with major postoperative complications in an international cohort and to present a meta-analysis of all available prospective data.
Methods: This prospective, multicentre study included adults undergoing both elective and emergency gastrointestinal resection, reversal of stoma or formation of stoma. The primary end-point was 30-day major complications (Clavien-Dindo Grades III-V). A systematic search was undertaken for studies assessing the relationship between obesity and major complications after gastrointestinal surgery. Individual patient meta-analysis was used to analyse pooled results.
Results: This study included 2519 patients across 127 centres, of whom 560 (22.2%) were obese. Unadjusted major complication rates were lower in obese vs normal weight patients (13.0% vs 16.2%, respectively), but this did not reach statistical significance (P = 0.863) on multivariate analysis for patients having surgery for either malignant or benign conditions. Individual patient meta-analysis demonstrated that obese patients undergoing surgery for malignancy were at increased risk of major complications (OR 2.10, 95% CI 1.49-2.96, P < 0.001), whereas obese patients undergoing surgery for benign indications were at decreased risk (OR 0.59, 95% CI 0.46-0.75, P < 0.001) compared to normal weight patients.
Conclusions: In our international data, obesity was not found to be associated with major complications following gastrointestinal surgery. Meta-analysis of available prospective data made a novel finding of obesity being associated with different outcomes depending on whether patients were undergoing surgery for benign or malignant disease
Body mass index and complications following major gastrointestinal surgery: a prospective, international cohort study and meta‐analysis
- Author
- A A Adebayo
- A A Gonzalez Ruiz
- A A Khetarpal
- A A Thevathasan
- A A Zhang
- A Abdulmajid
- A Abid
- A Adlan
- A Ahmad
- A Akdogan
- A Al-Mousawi
- A Al-Nasser
- A Al-Robeye
- A Ali
- A Aljbour
- A Amajuoyi
- A Ang
- A Anilkumar
- A Arezzo
- A Arrigo
- A Aslanyan
- A Asma
- A Asmadi
- A Atayi
- A Aytekin
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- A B Bolat
- A Badran
- A Bakhsh
- A Baldwin
- A Batho
- A Bell
- A Benevento
- A Bhangu
- A Borrellas
- A Brogan
- A Broyd
- A Burgess
- A C D Smith
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- A C van der Hoeven
- A Cammarota
- A Campion
- A Capozzolo
- A Charania
- A Chhabra
- A Chung
- A Coates
- A Cody
- A Collins
- A Costa
- A Cotton
- A Craig-McQuaide
- A Croall
- A Curran
- A D Greenhalgh
- A D Hacioglu
- A D Henson
- A D Semana
- A D Wood
- A Daoub
- A Decorato
- A Delport
- A Demirci
- A Dhanji
- A Díaz Padillo
- A Doshi
- A Duffy
- A Durr
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- A E Cardwell
- A E Gezen
- A E Lim
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- N Palanivail
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- N Pujol-Cano
- N Punjabi
- N Rajan
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- N Seneviratne
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- N Yildirim
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- O Al-Obaedi
- O Altintas
- O Amin
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- O D Thompson
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- O F Toto
- O Firat
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- O J Cundy
- O K Vernon
- O Kopac
- O Kurklu
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- O O'Carroll
- O Ogunleye
- O Parker
- O Prys-Jones
- O Sitta
- O Sotona
- O Spence
- O Taskin
- O Uzun
- O Ziff
- P A Schmidt
- P Alberti Delgado
- P Aonzo
- P Avery
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- P Buakuma
- P C Copley
- P C Hurst
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- P Checcacci
- P Ciano
- P Collins
- P Coyne
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- P D Jewell
- P De Nardi
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- P Diaz-Jover
- P Dube
- P E Gonzalez de Chaves
- P Erdogan
- P Fergurson
- P G Horgan
- P Gaskell
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- P H Khaing
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- P Higgins
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- P Innocenti
- P J Choi
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- P W Stather
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- R A O'Loughlin
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- R D Obute
- R Dawar
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- S A Graus
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- S Angelov
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- S B Husnoo
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- S Quill
- S Qureshi
- S R Kosasih
- S R Mizan
- S Rabinthiran
- S Rashid
- S Rees
- S Rinkoff
- S Rogers
- S S Talukdar
- S S Yildiz
- S S Yurdaor
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- S Suresh
- S T Marchal
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- S Trecarten
- S Turaga
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- S Venturini
- S Verma
- S Vivekanantham
- S W McLure
- S Wadanamby
- S Wang
- S X Poo
- S Yaman
- S Yauw
- S Yıgman
- S Yildiz
- S Yilmaz
- S Yoganathan
- S Z Kuiper
- S Zope
- T Akcaoglu
- T Ankarali
- T Arif
- T Axelson
- T Bergara
- T Bloomfield
- T C Hoskins
- T Caliskan
- T Clifford
- T D Pinkney
- T de Mees
- T Dogra
- T Dosa
- T Dušek
- T E Glover
- T Elkatroushi
- T Erel
- T Ersoy
- T Fautz
- T Filipescu
- T Goldsmith
- T Kane
- T Khan
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- T Lewis
- T Lo
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- T M P Fung
- T M Schulz
- T M Van Heumen
- T Nelli
- T Oakley
- T P Bemand
- T P Pezas
- T Patel
- T Pitts-Tucker
- T R Barrow
- T R van Elst
- T Raghvani
- T Ramtoola
- T Rangan
- T Reakes
- T Reeves
- T Rob
- T Ross
- T S Deliktas
- T S L Yeoh
- T S Oudman
- T Sale
- T Sarvanandan
- T Schok
- T Sivrikaya
- T Sorah
- T Spencer
- T Tharmachandirar
- T Vable
- T van Engelenburg
- T W Tilston
- T Ward
- T Wilson
- T Yang
- T Yildiz
- T Yilmaz
- T Zengin
- U Arslan
- U Ashfaq
- U Cengiz
- U Datta
- U de Andres Olabarria
- U Hayat
- U Karabacak
- U Khan
- U Onsal
- U Qureshi
- U S Mohamed
- U Sajjad
- U Seyhan
- U Topal
- U White
- V A J I M van Rijckevorsel
- V Agarwal
- V Anakwenze
- V Balian
- V Barone
- V C Isler
- V C Wing
- V Charavanamuttu
- V Dominguez-Prieto
- V Elangovan
- V Farina
- V Gilissen
- V Gupta
- V Laterza
- V M Duran Muñoz-Cruzado
- V M T van Verschuer
- V Manvydas
- V Mirdavoudi
- V Morandi
- V Narwani
- V Navayogaarajah
- V Ozben
- V Paraoan
- V Patel
- V Pattapola
- V Portugal Porras
- V Raghuvir
- V Raina
- V Rampulla
- V Robertson
- V Sari
- V Shatkar
- V Simon Frapolli
- V Soria Aledo
- V Teng
- V Thirumal
- V Tosun
- V Wong
- W A Bemelman
- W A Gatfield
- W Bolton
- W C Soon
- W Cymes
- W Dean
- W Din
- W English
- W Goh
- W H Steup
- W Ho
- W Hogendoorn
- W J A Sedee
- W J Dronkers
- W J H J Meijerink
- W Leung
- W Liew
- W Loke
- W M U Van Grevenstein
- W M Wynell-Mayow
- W P M Van Dijck
- W W Chaudhry
- X Chen
- X F Gonzalez-Argente
- X Monzonis Hernandez
- Y Buyukkarabacak
- Y Cao
- Y Devabalan
- Y E Alim
- Y Eggen
- Y Embury-Young
- Y Endo
- Y F Dennis
- Y Gozubuyuk
- Y Gunaydin
- Y H Soo
- Y H Tan
- Y I Z Acherman
- Y Kelesoglu
- Y Liew
- Y Maheswaran
- Y N Löwensteyn
- Y N Neo
- Y N Suleman
- Y Narang
- Y P Mogan
- Y R Willems
- Y S Mugurtay
- Y Sinha
- Y Tan
- Y Taşçı
- Y Yalcin
- Z A Saglam
- Z Abbas
- Z Afzal
- Z Al-Nasser
- Z B Ekinci
- Z Gok
- Z H Sam
- Z H Siddiqui
- Z Kazmi
- Z Khonat
- Z Momoh
- Z O B B Soylemez
- Z O Belibagli
- Z P Polat
- Z Parinisi
- Z R Bakewell
- Z S Demirci
- Z Yazkan
- Publication venue
- Publication date
- 01/01/2018
- Field of study
No full textAim Previous studies reported conflicting evidence on the effects of obesity on outcomes after gastrointestinal surgery. The aims of this study were to explore the relationship of obesity with major postoperative complications in an international cohort and to present a meta-analysis of all available prospective data.Methods This prospective, multicentre study included adults undergoing both elective and emergency gastrointestinal resection, reversal of stoma or formation of stoma. The primary end-point was 30-day major complications (Clavien-Dindo Grades III-V). A systematic search was undertaken for studies assessing the relationship between obesity and major complications after gastrointestinal surgery. Individual patient meta-analysis was used to analyse pooled results.Results This study included 2519 patients across 127 centres, of whom 560 (22.2%) were obese. Unadjusted major complication rates were lower in obese vs normal weight patients (13.0% vs 16.2%, respectively), but this did not reach statistical significance (P = 0.863) on multivariate analysis for patients having surgery for either malignant or benign conditions. Individual patient meta-analysis demonstrated that obese patients undergoing surgery for malignancy were at increased risk of major complications (OR 2.10, 95% CI 1.49-2.96, P < 0.001), whereas obese patients undergoing surgery for benign indications were at decreased risk (OR 0.59, 95% CI 0.46-0.75, P < 0.001) compared to normal weight patients.Conclusions In our international data, obesity was not found to be associated with major complications following gastrointestinal surgery. Meta-analysis of available prospective data made a novel finding of obesity being associated with different outcomes depending on whether patients were undergoing surgery for benign or malignant disease
