156 research outputs found
Metallic ground state and glassy transport in single crystalline URhGe: Enhancement of disorder effects in a strongly correlated electron system
We present a detailed study of the electronic transport properties on a
single crystalline specimen of the moderately disordered heavy fermion system
URhGe. For this material, we find glassy electronic transport in a
single crystalline compound. We derive the temperature dependence of the
electrical conductivity and establish metallicity by means of optical
conductivity and Hall effect measurements. The overall behavior of the
electronic transport properties closely resembles that of metallic glasses,
with at low temperatures an additional minor spin disorder contribution. We
argue that this glassy electronic behavior in a crystalline compound reflects
the enhancement of disorder effects as consequence of strong electronic
correlations.Comment: 5 pages, 4 figures, accepted for publication in PR
Giant spin canting in the S = 1/2 antiferromagnetic chain [CuPM(NO3)2(H2O)2]n observed by 13C-NMR
We present a combined experimental and theoretical study on copper pyrimidine
dinitrate [CuPM(NO3)2(H2O)2]n, a one-dimensional S = 1/2 antiferromagnet with
alternating local symmetry. From the local susceptibility measured by NMR at
the three inequivalent carbon sites in the pyrimidine molecule we deduce a
giant spin canting, i.e., an additional staggered magnetization perpendicular
to the applied external field at low temperatures. The magnitude of the
transverse magnetization, the spin canting of 52 degrees at 10 K and 9.3 T and
its temperature dependence are in excellent agreement with exact
diagonalization calculations.Comment: 5 pages, 6 Postscript figure
Quantum critical dynamics of a S = 1/2 antiferromagnetic Heisenberg chain studied by 13C-NMR spectroscopy
We present a 13C-NMR study of the magnetic field driven transition to
complete polarization of the S=1/2 antiferromagnetic Heisenberg chain system
copper pyrazine dinitrate Cu(C_4H_4N_2)(NO_3)_2 (CuPzN). The static local
magnetization as well as the low-frequency spin dynamics, probed via the
nuclear spin-lattice relaxation rate 1/T_1, were explored from the low to the
high field limit and at temperatures from the quantum regime (k_B T << J) up to
the classical regime (k_B T >> J). The experimental data show very good
agreement with quantum Monte Carlo calculations over the complete range of
parameters investigated. Close to the critical field, as derived from static
experiments, a pronounced maximum in 1/T_1 is found which we interpret as the
finite-temperature manifestation of a diverging density of zero-energy magnetic
excitations at the field-driven quantum critical point.Comment: 5 pages, 4 figure
Spectroscopic study of the magnetic ground state of NbFe
We have investigated single crystals and polycrystals from the series
NbFe, by electron spin resonance,
muon spin relaxation and M\"ossbauer spectroscopy. Our data establish that at
lowest temperatures all samples exhibit bulk magnetic order. Slight Fe-excess
induces low-moment ferromagnetism, consistent with bulk magnetometry (), Nb--rich and stoichiometric NbFe display spin
density wave order with small magnetic moment amplitudes of the order . This provides microscopic evidence for a
modulated magnetic state on the border of ferromagnetism in NbFe.Comment: 7 pages, 9 figure
Field-induced coupled superconductivity and spin density wave order in the Heavy Fermion compound CeCoIn5
The high field superconducting state in CeCoIn5 has been studied by
transverse field muon spin rotation measurements with an applied field parallel
to the crystallographic c-axis close to the upper critical field Hc2 = 4.97 T.
At magnetic fields >= 4.8 T the muon Knight shift is enhanced and the
superconducting transition changes from second order towards first order as
predicted for Pauli-limited superconductors. The field and temperature
dependence of the transverse muon spin relaxation rate sigma reveal
paramagnetic spin fluctuations in the field regime from 2 T < H < 4.8 T. In the
normal state close to Hc2 correlated spin fluctuations as described by the self
consistent renormalization theory are observed. The results support the
formation of a mode-coupled superconducting and antiferromagnetically ordered
phase in CeCoIn5 for H directed parallel to the c-axis.Comment: 5 paes, 4 figure
Magnetoelastic and structural properties of azurite Cu3(CO3)2(OH)2 from neutron scattering and muon spin rotation
Azurite, Cu3(CO3)2(OH)2, has been considered an ideal example of a
one-dimensional (1D) diamond chain antiferromagnet. Early studies of this
material imply the presence of an ordered antiferromagnetic phase below K while magnetization measurements have revealed a 1/3 magnetization
plateau. Until now, no corroborating neutron scattering results have been
published to confirm the ordered magnetic moment structure. We present recent
neutron diffraction results which reveal the presence of commensurate magnetic
order in azurite which coexists with significant magnetoelastic strain. The
latter of these effects may indicate the presence of spin frustration in zero
applied magnetic field. Muon spin rotation, SR, reveals an onset of
short-range order below 3K and confirms long-range order below .Comment: 5 pages, 4 figures, PHYSICAL REVIEW B 81, 140406(R) (2010
Antiferromagnetic Dimers of Ni(II) in the S=1 Spin-Ladder Na_2Ni_2(C_2O_4)_3(H_2O)_2
We report the synthesis, crystal structure and magnetic properties of the S=1
2-leg spin-ladder compound Na_2Ni_2(C_2O_4)_3(H_2O)_2. The magnetic properties
were examined by magnetic susceptibility and pulsed high field magnetization
measurements. The magnetic excitations have been measured in high field high
frequency ESR. Although the Ni(II) ions form structurally a 2-leg ladder, an
isolated dimer model consistently describes the observations very well. The
analysis of the temperature dependent magnetization data leads to a magnetic
exchange constant of J=43 K along the rungs of the ladder and an average value
of the g-factor of 2.25. From the ESR measurements, we determined the single
ion anisotropy to D=11.5 K. The validity of the isolated dimer model is
supported by Quantum Monte Carlo calculations, performed for several ratios of
interdimer and intradimer magnetic exchange and taking into account the
experimentally determined single ion anisotropy. The results can be understood
in terms of the different coordination and superexchange angles of the oxalate
ligands along the rungs and legs of the 2-leg spin ladder.Comment: 8 pages, 10 figure
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